胺基改性微/介孔材料吸附CO_2研究进展
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摘要
化学嫁接法或物理浸渍法胺基改性微/介孔复合材料结合了化学吸附与物理吸附的优点,是一种潜在的CO_2吸附剂。主要论述了胺基改性微孔分子筛、介孔分子筛以及微/介孔复合材料在不同条件下对CO2的捕获效果,并对比了它们的相关性能,对未来新材料的研究方向进行了展望。
Combining the advantages of chemical and physical adsorption,the amine modified micro/mesoporous composite material produced by chemical grafting or physical impregnation method is a potential CO_2 adsorbent.The capture properties of microporous molecular sieves,mesoporous molecular sieves and micro/mesoporous composite materials after amine modification under different conditions on CO_2 were mainly discussed.And their relevant performance was compared.The prospect of some new materials was proposed and a new direction was provided for future research.
Combining the advantages of chemical and physical adsorption,the amine modified micro/mesoporous composite material produced by chemical grafting or physical impregnation method is a potential CO_2 adsorbent.The capture properties of microporous molecular sieves,mesoporous molecular sieves and micro/mesoporous composite materials after amine modification under different conditions on CO_2 were mainly discussed.And their relevant performance was compared.The prospect of some new materials was proposed and a new direction was provided for future research.
引文
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[3]Su F S,Lu C,Kuo S C,et al.Adsorption of CO2on aminefunctionalized Y-type zeolites[J].Energy&Fuels,2010,24(2):1441-1448.
[4]Lee C H,Hyeon D H,Jung H,et al.Effects of pore structure and PEI impregnation on carbon dioxide adsorption by ZSM-5zeolites[J].Journal of Industrial&Engineering Chemistry,2015,23:251-256.
[5]Bhagiyalakshmi M,Yun L J,Anuradha R,et al.Utilization of rice husk ash as silica source for the synthesis of mesoporous silicas and their application to CO2 adsorption through TREN/TEPA grafting[J].Journal of Hazardous Materials,2010,175(1/2/3):928-938.
[6]Wang W L,Xiao J,Wei X L,et al.Development of a new clay supported polyethylenimine composite for CO2capture[J].Applied Energy,2014,113(6):334-341.
[7]Sanz R,Calleja G,Arencibia A,et al.CO2capture with poreexpanded MCM-41 silica modified with amino groups by double functionalization[J].Microporous&Mesoporous Materials,2015,209:165-171.
[8]Yue M B,Sun L B,Cao Y,et al.Promoting the CO2adsorption in the amine-containing SBA-15by hydroxyl group[J].Microporous&Mesoporous Materials,2008,114(1/2/3):74-81.
[9]Xu X C,Song C S,Andrésen J M,et al.Preparation and characterization of novel CO2“molecular basket”adsorbents based on polymer-modified mesoporous molecular sieve MCM-41[J].Microporous&Mesoporous Materials,2003,62(1/2):29-45.
[10]Wei J W,Shi J J,Pan H,et al.Adsorption of carbon dioxide on organically functionalized SBA-16[J].Microporous&Mesoporous Materials,2008,116(1/2/3):394-399.
[11]Matsumoto A,Sasaki T.Thermal stability and hydrophobicity of mesoporous silica FSM-16[J].Colloids&Surfaces A:Physicochemical&Engineering Aspects,2002,203(1/2/3):185-193.
[12]史晶金,刘亚敏,陈杰,等.氨基功能化SBA-16对CO2的动态吸附特性[J].物理化学学报,2010,26(11):3023-3029.
[13]Son W J,Choi J S,Ahn W S.Adsorptive removal of carbon dioxide using polyethyleneimine-loaded mesoporous silica materials[J].Microporous&Mesoporous Materials,2008,113(1):31-40.
[14]Xu X C,Song C S,Andresen J M,et al.Novel polyethylenimine-modified mesoporous molecular sieve of MCM-41type as high-capacity adsorbent for CO2capture[J].Energy&Fuels,2002,16(6):1463-1469.
[15]Liu Y M,Shi J J,Chen J,et al.Dynamic performance of CO2adsorption with tetraethylenepentamine-loaded KIT-6[J].Microporous&Mesoporous Materials,2010,134(1/2/3):16-21.
[16]Liu Y M,Ye Q,Shen M,et al.Carbon dioxide capture by functionalized solid amine sorbents with simulated flue gas conditions[J].Environmental Science&Technology,2011,45(13):5710-5716.
[17]Kishor R,Ghoshal A K.APTES grafted ordered mesoporous silica KIT-6for CO2 adsorption[J].Chemical Engineering Journal,2014,262:882-890.
[18]Gartmann N,Schütze C,Ritter H,et al.The effect of water on the functionalization of mesoporous silica with 3-aminopropyltriethoxysilane[J].Journal of Physical Chemistry Letters,2009,1(1):379-382.
[19]Kishor R,Ghoshal A K.N1-(3-trimethoxysilylpropyl)diethylenetriamine grafted KIT-6for CO2/N2 selective separation[J].RSC Advances,2015,6(2):898-909.
[20]Zelenk V,Badanicov M,Halamov D,et al.Amine-modified ordered mesoporous silica:effect of pore size on carbon dioxide capture[J].Chemical Engineering Journal,2008,144(2):336-342.
[21]Santos S C G,Pedrosa A M G,Souza M J B,et al.Carbon dioxide adsorption on micro-mesoporous composite materials of ZSM-12/MCM-48type:the role of the contents of zeolite and functionalized amine[J].Materials Research Bulletin,2015,70:663-672.
[22]Zhou J H,Zhao H L,Li J X,et al.CO2capture on micro/mesoporous composites of(zeolite A)/(MCM-41)with Ca2+located:computer simulation and experimental studies[J].Solid State Sciences,2013,24(10):107-114.
[23]孔童童,王霞,郭庆杰.新型多级微/介孔固态胺吸附剂的制备及其CO2吸附性能研究[J].燃料化学学报,2015,43(12):1389-1497.
[24]Liu X W,Gao F,Xu J,et al.Zeolite@mesoporous silica-supported-amine hybrids for the capture of CO2in the presence of water[J].Microporous&Mesoporous Materials,2015,222:113-119.