红外波段水汽连续吸收研究进展
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摘要
水汽连续吸收广泛存在于红外波段,对于地球辐射平衡和遥感探测有着重要的意义.一般水汽连续吸收的研究大多处于中红外窗口区域,而在吸收谱带内和近红外窗口区域的研究较少.目前,水汽连续吸收的机理仍然是一个有争议的课题.简要阐述了现有理论及计算模型的发展历史和研究现状,介绍了几种实验测量方法的原理、优点与不足,并对水汽连续吸收的发展进行了展望.
The infrared spectrum of water vapor is made up of strongly absorbing bands and many transparent windows between these bands. The water vapour continuum in these same spectral regions is of particular importance for the Earth's radiation budget and for remote sensing techniques that exploit these windows.Historically, most attention has focused on the mid-infrared atmospheric window, but there have been many fewer reports within bands and in the near-infrared spectral region. In addition, the causes of the continuum remain a subject of controversy. The history and recent developments of the causes of the continuum and calculation models were reviewed briefly. The advantages and disadvantages of several experimental methods were discussed. The possible future directions were given.
The infrared spectrum of water vapor is made up of strongly absorbing bands and many transparent windows between these bands. The water vapour continuum in these same spectral regions is of particular importance for the Earth's radiation budget and for remote sensing techniques that exploit these windows.Historically, most attention has focused on the mid-infrared atmospheric window, but there have been many fewer reports within bands and in the near-infrared spectral region. In addition, the causes of the continuum remain a subject of controversy. The history and recent developments of the causes of the continuum and calculation models were reviewed briefly. The advantages and disadvantages of several experimental methods were discussed. The possible future directions were given.
引文
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[15]Ma Q,Tipping R H,Leforestier C.Temperature dependences of mechanisms responsible for the water-vapor continuum absorption.I.Far wings of allowed lines[J].The Journal of Chemical Physics,2008,128(12):124313.
[16]Bogdanova J V,Rodimova O B.Line shape in far wings and water vapor absorption in a broad temperature interval[J].Journal of Quantitative Spectroscopy and Radiative Transfer,2010,111(15):2298-2307.
[17]Baranov Y I,Lafferty W J.The water vapour self-and water-nitrogen continuum absorption in the 1000 and 2500 cm~(-1)atmospheric windows[J].Philosophical Transactions of the Royal Society A:Mathematical,Physical and Engineering Sciences,2012,370(1968):2578-2589.
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[25]Bignell K,Saiedy F,Sheppard P A.On the atmospheric infrared continuum[J].Journal of the Optical Society of America,1963,53(4):466-479.
[26]Fomin V V,Tvorogov S D.Formation of the far wings contour of spectral lines broadened by a foreign gas;analysis of exponential decrease of continuous absorption beyond the band head of the4.3μm band of CO_2[J].Applied Optics,1973,12(3):584-589.
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[30]Fano U.Pressure broadening as a prototype of relaxation[J].Physicai Review,1963,131(1):259.
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[33]Ma Q,Tipping R H.A far wing line shape theory and its application to the water continuum absorption in the infrared region.I[J].The Journal of Chemical Physics,1991,95(9):6290-6301.
[34]Ma Q,Tipping R H.A far wing line shape theory and its application to the foreign-broadened water continuum absorption.Ⅲ[J].The Journal of Chemical Physics,1992,97(2):818-828.
[35]Ma Q,Tipping R H.The averaged density mar trix in the coordinate representation:application to the calculation of the far-wing line shapes for H_2O[J].The Journal of Chemical Physics,1999,111(13):5909-5921.
[36]Ma Q,Tipping R H.The frequency detuning correction and the asymmetry of line shapes:the far wings of H_2OH_2O[J].The Journal of Chemical Physics,2002,110(10):4102-4115.
[37]Cormier J G,Ciurylo R,Drummond J R.Cavity ringdown spectroscopy measurements of the infrared water vapor continuum[J].The Journal of Chemical Physics,2002,118(3):1030-1034.
[38]Bogdanova J V,Rodimova O B.Line shape in far wings and water vapor absorption in a broad temperature interval[J].Journal of Quantitative Spectroscopy and Radiative Transfer,2010,111(15):2298-2307.
[39]Klimeshina T E,Rodimova O B.Temperature dependence of the water vapor continuum absorption in the 3~5μm spectral region[J].Journal of Quantitative Spectroscopy and Radiative Transfer,2013,119:77-83.
[40]Penner S S,Varanasi P.Spectral absorption coefficients in the pure rotation spectrum of water vapor[J].Journal of Quantitative Spectroscopy and Radiative Transfer,1967,7(4):687-690.
[41]Varanasi P,Chou S,Penner S S.Absorption coefficients for water vapor in the 600~1000 cm~(-1)region[J],Journal of Quantitative Spectroscopy and Radiative Transfer,1968,8(8):1537-1541.
[42]Bignell K J.The water-vapour infrared continuum[J].Quarterly Journal of the Royal Meteorological Society,1970,96(409):390-403.
[43]Aref'ev V N,Dianov-Klokov V I,Radionov V F,et al.Laboratory measurements of attenuation of CO_2 laser radiation by pure water vapor[J].Optics and Spectroscopy,1975,39(5):560-561.
[44]Aref'ev V N,Dianov-Klokov V I.Attenuation of10.6μm radiation by water vapor and the role of(H_2O)_2 dimers[J].Optics and Spectroscopy,1977,42:488-492.
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