碳热还原氮化法制备氮化铝的研究进展
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摘要
氮化铝陶瓷在热、电、光和力学等方面具有优良的综合性能,是理想的基板材料和电子封装材料,碳热还原法制备氮化铝粉末是实现氮化铝粉末商业化生产的重要方法。综述了国内外采用碳热还原法制备氮化铝粉末的工艺和反应机理的研究进展,并对未来研究方向进行了展望。
Aluminum nitride ceramics are the ideal substrate materials and electronic packaging materials due to their excellent comprehensive performances in thermal,electrical,optical and mechanical aspects. The carbothermal reduction method is an important commercial production method for AlN powder. The research progresses of AlN powders prepared by the carbothermal reduction method at home and abroad were reviewed from the aspects of process and rection mechanism,and the future research direction was prospected.
Aluminum nitride ceramics are the ideal substrate materials and electronic packaging materials due to their excellent comprehensive performances in thermal,electrical,optical and mechanical aspects. The carbothermal reduction method is an important commercial production method for AlN powder. The research progresses of AlN powders prepared by the carbothermal reduction method at home and abroad were reviewed from the aspects of process and rection mechanism,and the future research direction was prospected.
引文
[1]王柳燕,张宁.氮化铝粉体制备技术的研究现状与展望[J].粉末冶金工业,2008,18(3):42.
[2]姚园林,李慧琴,韩晓星.稀土掺杂ZnVO基压敏陶瓷的研究进展[J].金属功能材料,2016,23(4):53.
[3]黄莉萍,黄熊璋,符锡仁,等.氮化铝粉末的制备[J].硅酸盐学报,1986(3):78.
[4]姜珩.氮化铝粉末的制备研究[D].北京:北京有色金属研究总院,2012.
[5] QI S,MAO X,LI X,et al. Synthesis of AlN hexagonal bipyramids by carbothermal reduction nitridation[J]. Materials Letters,2016,174:167.
[6]谭俊,张勇,吴迪,等.自蔓延高温合成法合成金属陶瓷功能梯度材料研究进展[J].材料导报,2013,27(17):79.
[7]宋旭波,郭志刚,郑捷,等.化学气相沉积法合成氮化铝纳米材料[C]//中国化学会学术年会.北京:2006.
[8]邹清,马鸿雁.氮化铝的研究进展[J].化学研究与应用,2004(1):11.
[9] WANG Q,CUI W,GE Y,et al. Preparation of spherical AlN granules directly by carbothermal reduction-nitridation method[J]. Journal of the American Ceramic Society,2015,98(2):392.
[10] Lefort P,Billy M. Mechanism of AlN formation through the carbothermal reduction of Al2O3in a flowing N2atmosphere[J].Journal of the American Ceramic Society,2010,76(9):2295.
[11] Baik Y,Shanker K,Mcdermid J R,et al. Carbothermal synthesis of aluminum nitride using sucrose[J]. Journal of the American Ceramic Society,2010,77(8):2165.
[12]秦明礼,杜学丽,李帅,等.沉淀前驱物制备AIN陶瓷粉末[J].中国有色金属学报,2005,15(12):1974.
[13] Tsuge A,Inoue H,Kasori M,et al. Raw material effect on AIN powder synthesis from Al2O3,carbothermal reduction[J]. Journal of Materials Science,1990,25(5):2359.
[14]刘新宽,马明亮,周敬恩.高能球磨对碳热还原合成氮化铝的作用[J].兵器材料科学与工程,1999,22(3):23.
[15] Ramesh Peelamedu D,Rao Kalva J. Microwave-assisted synthesis of aluminum nitride[J]. Advanced Materials,2010,7(2):177.
[16]肖劲,周峰,陈燕彬.微波碳热还原法制备氮化铝粉末的工艺研究[J].无机材料学报,2009,4(4):755.
[17] Ide T,Komeya K,Meguro T,et al. Synthesis of Al N powder by carbothermal reduction-nitridation of various Al2O3powders with Ca F2[J]. Key Engineering Materials,2010,159/160(11):71.
[18]傅崇说.有色冶金原理[M]. 2版.北京:冶金工业出版社,2007.
[19] YU J K,Ueno S,LI H X,et al. Improvement of graphitization of isotropic carbon by Al2O3,formed from aluminium chelate compound[J]. Journal of the European Ceramic Society,1999,19(16):2843.
[20] Hirai N,Miwa T. Formation of aluminum nitride by carbothermic reduction of alumina in a flowing nitrogen atmosphere[J].Nippon Kinzoku Gakkaishi,1989,53(13):1053.
[21]张正权,金永中,杨林,等.碳/氮源对碳热还原(Ti,W)(C,N,B)固溶体粉末合成的影响[J].粉末冶金工业,2017,27(6):8.
[22] Suehiro T,Tatami J,Meguro T,et al. Aluminum nitride fibers synthesized from alumina fibers using gas-reduction-nitridation method[J]. Journal of the American Ceramic Society,2010,85(3):715.
[23]匡加才,张长瑞,周新贵,等.不同铝源对碳热还原法合成氮化铝粉末的影响[J].宇航材料工艺,2003,33(5):44.
[24]魏颖娜,魏恒勇,赵冬梅,等.基于非水解sol-gel法的碳热还原氮化合成氮化铝超细粉体[J].功能材料,2013,44(17):2546.
[25] Joo H U,Jung W S. Conversion of basic dicarboxylate Al(III)complexes to aluminum carbide under a flow of argon[J]. Journal of Alloys&Compounds,2008,465(1/2):265.
[2]姚园林,李慧琴,韩晓星.稀土掺杂ZnVO基压敏陶瓷的研究进展[J].金属功能材料,2016,23(4):53.
[3]黄莉萍,黄熊璋,符锡仁,等.氮化铝粉末的制备[J].硅酸盐学报,1986(3):78.
[4]姜珩.氮化铝粉末的制备研究[D].北京:北京有色金属研究总院,2012.
[5] QI S,MAO X,LI X,et al. Synthesis of AlN hexagonal bipyramids by carbothermal reduction nitridation[J]. Materials Letters,2016,174:167.
[6]谭俊,张勇,吴迪,等.自蔓延高温合成法合成金属陶瓷功能梯度材料研究进展[J].材料导报,2013,27(17):79.
[7]宋旭波,郭志刚,郑捷,等.化学气相沉积法合成氮化铝纳米材料[C]//中国化学会学术年会.北京:2006.
[8]邹清,马鸿雁.氮化铝的研究进展[J].化学研究与应用,2004(1):11.
[9] WANG Q,CUI W,GE Y,et al. Preparation of spherical AlN granules directly by carbothermal reduction-nitridation method[J]. Journal of the American Ceramic Society,2015,98(2):392.
[10] Lefort P,Billy M. Mechanism of AlN formation through the carbothermal reduction of Al2O3in a flowing N2atmosphere[J].Journal of the American Ceramic Society,2010,76(9):2295.
[11] Baik Y,Shanker K,Mcdermid J R,et al. Carbothermal synthesis of aluminum nitride using sucrose[J]. Journal of the American Ceramic Society,2010,77(8):2165.
[12]秦明礼,杜学丽,李帅,等.沉淀前驱物制备AIN陶瓷粉末[J].中国有色金属学报,2005,15(12):1974.
[13] Tsuge A,Inoue H,Kasori M,et al. Raw material effect on AIN powder synthesis from Al2O3,carbothermal reduction[J]. Journal of Materials Science,1990,25(5):2359.
[14]刘新宽,马明亮,周敬恩.高能球磨对碳热还原合成氮化铝的作用[J].兵器材料科学与工程,1999,22(3):23.
[15] Ramesh Peelamedu D,Rao Kalva J. Microwave-assisted synthesis of aluminum nitride[J]. Advanced Materials,2010,7(2):177.
[16]肖劲,周峰,陈燕彬.微波碳热还原法制备氮化铝粉末的工艺研究[J].无机材料学报,2009,4(4):755.
[17] Ide T,Komeya K,Meguro T,et al. Synthesis of Al N powder by carbothermal reduction-nitridation of various Al2O3powders with Ca F2[J]. Key Engineering Materials,2010,159/160(11):71.
[18]傅崇说.有色冶金原理[M]. 2版.北京:冶金工业出版社,2007.
[19] YU J K,Ueno S,LI H X,et al. Improvement of graphitization of isotropic carbon by Al2O3,formed from aluminium chelate compound[J]. Journal of the European Ceramic Society,1999,19(16):2843.
[20] Hirai N,Miwa T. Formation of aluminum nitride by carbothermic reduction of alumina in a flowing nitrogen atmosphere[J].Nippon Kinzoku Gakkaishi,1989,53(13):1053.
[21]张正权,金永中,杨林,等.碳/氮源对碳热还原(Ti,W)(C,N,B)固溶体粉末合成的影响[J].粉末冶金工业,2017,27(6):8.
[22] Suehiro T,Tatami J,Meguro T,et al. Aluminum nitride fibers synthesized from alumina fibers using gas-reduction-nitridation method[J]. Journal of the American Ceramic Society,2010,85(3):715.
[23]匡加才,张长瑞,周新贵,等.不同铝源对碳热还原法合成氮化铝粉末的影响[J].宇航材料工艺,2003,33(5):44.
[24]魏颖娜,魏恒勇,赵冬梅,等.基于非水解sol-gel法的碳热还原氮化合成氮化铝超细粉体[J].功能材料,2013,44(17):2546.
[25] Joo H U,Jung W S. Conversion of basic dicarboxylate Al(III)complexes to aluminum carbide under a flow of argon[J]. Journal of Alloys&Compounds,2008,465(1/2):265.