摘要
二维过渡金属碳/氮化物(MXene)是2011年发现的一类结构新颖、性质独特的层状纳米材料,目前已被广泛应用于能源存储以及环境治理等领域. MXene材料拥有较大的比表面积、丰富的活性吸附位点、良好的亲水性以及可控的层间距,并且这类纯无机材料表现出优异的抗辐照性能以及良好的导热性能,因此是容纳放射性元素与重金属离子的理想载体.本文归纳总结了近年来MXene材料的可控制备及其对放射性元素和重金属离子的去除研究进展,对相关的实验技术手段、吸附行为与相互作用机理进行了系统梳理,此外还对该领域的发展趋势进行了展望.
Two-dimensional transition metal carbide/nitride(MXene) is a class of new layered nanomaterial discovered in 2011. Due to the novel structure and unique characteristics, MXene-based materials have been widely explored in the applications of energy storage and environmental remediation fields. MXene materials have the advantages of large specific surface areas, abundant active adsorption sites, good hydrophilicity and controllable layer space, and such purely inorganic materials also exhibit excellent radiation resistance and thermal conductivity, thus can be considered as ideal candidates for the sequestration of radioactive element and heavy metal ions. Herein we review the research progress in the controllable preparation of MXene materials and their removal performance for radionuclides and heavy metal ions in the past five years. The related experimental techniques, adsorption behaviors and interaction mechanisms have been systematically summarized. The prospective investigation trends and possible directions in this field are also proposed and discussed.
引文
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