废树脂湿法氧化减容处理技术路线及问题探讨
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摘要
从废树脂湿法氧化处理技术的优势出发,分析比较了国内外湿法氧化处理技术的发展和研究现状,设计了废树脂湿法氧化减容及水泥固化处理技术路线,探讨了该处理技术的关键技术问题。
After briefing on the advantages of wet oxidation technology,the paper analyzes and compares the advances of wet oxidation technology domestic and aboard. A technical route of wet oxidation and cemented solidification of spent resin for volume reduction is then proposed with discussions on key issues.
After briefing on the advantages of wet oxidation technology,the paper analyzes and compares the advances of wet oxidation technology domestic and aboard. A technical route of wet oxidation and cemented solidification of spent resin for volume reduction is then proposed with discussions on key issues.
引文
[1]范智文.放射性废物树脂水泥固化体性能[D].北京:清华大学,2003.
[2]郭喜良,冯文东,高帅,等.放射性废物用高整体容器监管政策研究[R].中国辐射防护研究院,2012.
[3]裴勇,潘跃龙.高整体容器在我国放射性废物管理中的应用分析[J].核动力工程,2012,33(03):125-128.
[4]刘志勇,游兆金,康云鼎,等.秦山核电基地放射性废物最小化技术路线探讨[C]//第三届两岸放射性废物管理研讨会会议论文集.成都,2013.
[5]程娟,李全伟.放射性废树脂氧化分解处理技术[J].同位素,2012,25(2):124-128.
[6]罗上庚.废离子交换树脂的优化处理[J].核科学与工程,2003,23(3):165-171.
[7]Ma Jiahai,Song Wenjing,Chen Chuncheng,et al.Fenton degradation of organic compounds promoted by dyes under visible irradiation[J].Environ Sci Technol,2005,39:5 810-5 815.
[8]Bibler NE,Orebaugh EG.Iron-catalysed dissolution of polystyrenesulfonate cation-exchange resin in hydrogen peroxide[J].Ind Eng Chem Prod Res Dev,1976,15:136.
[9]Miyamoto T,Motoyama M,Shibuya M.Development of wet-oxidation treatment system for filter backwash sludge and ion exchange resins[C].WM’03 conference,Tucson,Arizona(USA),2003.
[10]Gunale TL,Mahajani VV,Wattal PK,et al.Studies in liquid phase mineralization of cation exchange resin by a hybrid process of Fenton dissolution followed by wet oxidation[J].Chemical Engineering Journal,2009,148:371
[11]Hwan-Young Kim,In-Tae Kim,Gi-Hong Kim,et al.Wet oxidation of mixed resins by a modified Fenton’s reaction with an electrochemical potential[J].J Ind Eng Chem,2007,13(05):665-668.
[12]Srinivas C,Sugilal G,Wattal PK.Management of spent organic ion-exchange resins by photochemical oxidation[C].WM’03conference,Tucson,Arizona(USA),2003.
[13]Twissel MA,Holt NS.Wet oxidation of organic radioactive waste[R].Nuclear Science and Technology,EUR16776,European Commission,1996:17-25.
[14]蹇兴超,云桂春.放射性废离子交换树脂的过氧化氢湿法催化氧化技术研究[J].辐射防护,1993,13(3):203-210.
[15]李庆瑞.核二厂低放射性废弃物管理成效与精进简报[C]//2011年两岸核电管理研讨会.北京,2011.
[16]陈义平,田景光,罗任瀚,等.湿式氧化暨高效率固化系统之建置[C]//第三届两岸放射性废物管理研讨会会议论文集.成都,2013.
[17]梁志荣,吴玉生,刘学军.芬顿氧化法预处理放射性废离子交换树脂[J].核化学与放射化学,2007,29(2):71-74.
[2]郭喜良,冯文东,高帅,等.放射性废物用高整体容器监管政策研究[R].中国辐射防护研究院,2012.
[3]裴勇,潘跃龙.高整体容器在我国放射性废物管理中的应用分析[J].核动力工程,2012,33(03):125-128.
[4]刘志勇,游兆金,康云鼎,等.秦山核电基地放射性废物最小化技术路线探讨[C]//第三届两岸放射性废物管理研讨会会议论文集.成都,2013.
[5]程娟,李全伟.放射性废树脂氧化分解处理技术[J].同位素,2012,25(2):124-128.
[6]罗上庚.废离子交换树脂的优化处理[J].核科学与工程,2003,23(3):165-171.
[7]Ma Jiahai,Song Wenjing,Chen Chuncheng,et al.Fenton degradation of organic compounds promoted by dyes under visible irradiation[J].Environ Sci Technol,2005,39:5 810-5 815.
[8]Bibler NE,Orebaugh EG.Iron-catalysed dissolution of polystyrenesulfonate cation-exchange resin in hydrogen peroxide[J].Ind Eng Chem Prod Res Dev,1976,15:136.
[9]Miyamoto T,Motoyama M,Shibuya M.Development of wet-oxidation treatment system for filter backwash sludge and ion exchange resins[C].WM’03 conference,Tucson,Arizona(USA),2003.
[10]Gunale TL,Mahajani VV,Wattal PK,et al.Studies in liquid phase mineralization of cation exchange resin by a hybrid process of Fenton dissolution followed by wet oxidation[J].Chemical Engineering Journal,2009,148:371
[11]Hwan-Young Kim,In-Tae Kim,Gi-Hong Kim,et al.Wet oxidation of mixed resins by a modified Fenton’s reaction with an electrochemical potential[J].J Ind Eng Chem,2007,13(05):665-668.
[12]Srinivas C,Sugilal G,Wattal PK.Management of spent organic ion-exchange resins by photochemical oxidation[C].WM’03conference,Tucson,Arizona(USA),2003.
[13]Twissel MA,Holt NS.Wet oxidation of organic radioactive waste[R].Nuclear Science and Technology,EUR16776,European Commission,1996:17-25.
[14]蹇兴超,云桂春.放射性废离子交换树脂的过氧化氢湿法催化氧化技术研究[J].辐射防护,1993,13(3):203-210.
[15]李庆瑞.核二厂低放射性废弃物管理成效与精进简报[C]//2011年两岸核电管理研讨会.北京,2011.
[16]陈义平,田景光,罗任瀚,等.湿式氧化暨高效率固化系统之建置[C]//第三届两岸放射性废物管理研讨会会议论文集.成都,2013.
[17]梁志荣,吴玉生,刘学军.芬顿氧化法预处理放射性废离子交换树脂[J].核化学与放射化学,2007,29(2):71-74.