湖相富有机质泥质白云岩生排烃模拟及其对页岩油勘探的启示
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摘要
富有机质湖相白云质泥岩、泥质白云岩及其贫有机质粉砂岩、白云岩夹层是我国陆相盆地页岩油勘探的重要领域,但目前针对湖相富有机质白云质泥岩或泥质白云岩在近地质条件下的生排烃一体化模拟研究尚属空白.以典型低熟富有机质泥质白云岩为例,开展了近地质条件下的生排烃一体化模拟实验,揭示了其呈现四阶段生排烃演化模式.结果表明,Ro≤0.74%时为缓慢生油伴生烃气、排油能力有限阶段,0.74%排油能力逐渐增高阶段,0.84%排油阶段,1.30% The organic-rich lacustrine dolomitic mudstone,argillaceous dolomite,organic-poor siltstone and dolomite interlayer are important areas for shale oil exploration in terrestrial basins in China.However,the research on the integration of hydrocarbon generation,expulsion and hydrocarbon accumulation in the lacustrine organic-rich dolomitic mudstone or argillaceous dolomite under near geological conditions is still blank.An integrate experiment of hydrocarbon generation and expulsion simulation from argillaceous dolomite rich in organic matter under near geological condition in confined systems,has been carried out with typical lower mature organic-rich argillaceous dolomite.The four-stage of hydrocarbon generation and expulsion evolution mod-el is revealed.The results show that the first stage is characterized by relatively slow oil generation associated hydrocarbon gases and by limited ability of oil expulsion when Rois≤0.74%.The second stage is characterized by rapid oil generation associated hydrocarbon gases and with incremental ability of oil expulsion when Rois in the range of 0.74%-0.84%.The third stage is characterized by hydrocarbon gas generation associated oil and oil initial cracking,and by oil expulsion effectively at 0.84%1.30%.And the retained oil is mainly occurred as adsorption phase with organic matter at Ro<0.68%,and mainly occurred as free phase within micron to nano-scale pores and microfractures in mineral matrix of argillaceous dolomite at 0.68%≤Ro≤2.00%.The range of thermal maturity for favorable shale oil exploration within lacustrine dolomite measures,is proposed at 0.84%-1.30%,on the basis of the results of simulation of hydrocarbon generation and expulsion for lacustrine organic-rich argillaceous dolomite,integrated with geological conditions and exploring economic benefit.
引文
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Guan,D.F.,Xu,X.H.,Li,Z.M.,et al.,2014.Hydrocarbon Generation Theory of Source Rocks in Confined System and Application.Petroleum Industry Press,Beijing,49-63(in Chinese).
Jarvie,D.M.,2012.Shale Resource Systems for Oil and Gas:Part 2-Shale-Oil Resource Systems.In:Breyer,J.A.,ed.,Shale Reservoirs-Giant Resources for the 21st Century.AAPG Memoir,97:89-119.https://doi.org/10.1306/13321447m973489
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Li,J.J.,Shi,Y.L.,Zhang,X.W.,et al.,2014.Control Factors of Enrichment and Producibility of Shale Oil:A Case Study of Biyang Depression.Earth Science,39(7):848-857(in Chinese with English abstract).https://doi.org/10.3799/dqkx.2014.079
Li,L.,Xu,G.S.,Wang,W.,et al.,2007.Accumulation Patterns of the Oil Reservoirs in the Daerqi Area,Baiyinchagan Sag,Inner Mongol,China.Journal of Chengdu University of Technology(Science&Technology Edition),34(3):277-284(in Chinese with English abstract).
Li,M.W.,Li,Z.M.,Li,Z.,et al.,2015.Formation and Occurrence Mechanism of Continental Shale Oil.Wuxi Research Institute of Petroleum Geology,SINOPEC,Wuxi(in Chinese).
Li,Z.M.,Zheng,L.J.,Ma,Z.L.,et al.,2011.Simulation of Source Rock for Hydrocarbon Generation and Expulsion in Finite Space and Its Significance.Petroleum Geology&Experiment,33(5):447-451,459(in Chinese with English abstract).
Lu,S.F.,Huang,W.B.,Chen,F.W.,et al,2012.Classification and Evaluation Criteria of Shale Oil and Gas Resources:Discussion and Application.Petroleum Exploration and Development,39(2):249-256(in Chinese with English abstract).
Ma,S.P.,Luo,C.S.,Tian,C.T.,et al.,2012.HydrocarbonGenerating Characteristics of Lacustrine Carbonate Rocks.Journal of Chengdu University of Technology(Science&Technology Edition),39(6):583-587(in Chinese with English abstract).
Ma,S.P.,Sun,D.,Zhang,X.B.,et al.,2011.The Study of Hydrocarbon Generation Kinetics in Lower Cretaceous Lacustrine Source Rocks,Qingxi Depression,Jiuxi Basin.Natural Gas Geoscience,22(2):219-223(in Chinese with English abstract).
Ma,Z.L.,Zheng,L.J.,Li,Z.M.,2012.The Thermocompression Simulation Experiment of Source Rock Hydrocarbon Generation and Expulsion in Formation Porosity.Acta Sedimentologica Sinica,30(5):955-963(in Chinese with English abstract).
Ma,Z.L.,Zheng,L.J.,Qin,J.Z.,et al.,2011.Hydrocarbon Generation and Expulsion Caused by Pressure Difference between Source Rock and Reservoir during Basin Subsiding and Uplifting.Petroleum Geology&Experiment,33(4):402-407(in Chinese with English abstract).
Pang,X.Q.,1995.Theory and Application of the Hydrocarbon Expulsion Threshold Controlling Petroleum Distribution.Petroleum Industry Press,Beijing,34-56(in Chinese).
Pepper,A.S.,Corvi,P.J.,1995.Simple Kinetic Models of Petroleum Formation.Part I:Oil and Gas Generation from Kerogen.Marine and Petroleum Geology,12(3):291-319.https://doi.org/10.1016/0264-8172(95)98381-e
Que,Y.Q.,Zheng,L.J.,Cheng,Q.Q.,et al.,2015.Vitrinite Reflectance Correction of Residues in Organic Matter Pyrolysis Simulation Experiments.Petroleum Geology&Experiment,37(4):506-511,517(in Chinese with English abstract).
Ritter,U.,2003.Solubility of Petroleum Compounds in Kerogen:Implications for Petroleum Expulsion.Organic Geochemistry,34(3):319-326.https://doi.org/10.1016/s0146-6380(02)00245-0
Shao,H.S.,Huang,X.Z.,Yan,C.F.,et al.,2002.Conditions for the Formation of Immature Oil in Lacustrine Carbonate Rocks in Biyang Depression.Geochimica,31(3):266-272(in Chinese with English abstract).
Stainforth,J.G.,2009.Practical Kinetic Modeling of Petroleum Generation and Expulsion.Marine and Petroleum Geology,26(4):552-572.https://doi.org/10.1016/j.marpetgeo.2009.01.006
Tan,Y.M.,Feng,J.H.,Jin,G.X.,et al.,2003.Geochemical Characteristics and Physical Features of Daerqi Oilfield,Baiyinchagan Depression.Geochimica,32(3):271-281(in Chinese with English abstract).
Tu,J.Q.,Chen,J.P.,Zhang,D.J.,et al.,2012.A Petrographic Classification of Macerals in Lacustrine Carbonate Source Rocks and Their Organic Petrological Characteristics:A Case Study on Jiuxi Basin,NW China.Acta Petrologica Sinica,28(3):917-926(in Chinese with English abstract).
Wang,G.L.,Wang,T.G.,Zhang,L.Y.,2007.Hydrocarbon Generation Characteristics for Lacustrine Carbonate Source Rocks in Bonan Sag of Jiyang Depression.Acta Petrolei Sinica,28(2):62-68(in Chinese with English abstract).
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Xiong,Y.,Cheng,K.M.,Ma,L.Y.,2006.Hydrocarbon Generation of Lower Cretaceous Lacustrine Carbonate in Jiuxi Depression.Petroleum Exploration and Development,33(6):687-691(in Chinese with English abstract).
Yan,Y.H.,Zou,Y.R.,Qu,Z.Y.,et al.,2015.Experimental Study on Hydrocarbon Retention-Expulsion of Es4 Formation Source Rock in the Dongying Depression.Geochimica,44(1):79-86(in Chinese with English abstract).
Yang,Z.M.,Wang,Q.,Shi,J.A.,et al.,2003.Controls on the Enrichment of Oil Pools in Qingxi Sag,Jiuxi Basin.Acta Sedimentologica Sinica,21(4):695-701(in Chinese with English abstract).
Yao,Y.,Wang,G.,Li,L.,et al.,2017.The Reservoir Heterogeneity Characteristics and Affecting Factors of Tight Lacustrine Dolomite Reservoirs.Earth Science,42(12):2327-2335(in Chinese with English abstract).https://doi.org/10.3799/dqkx.2017.145
Zhang,J.C.,Lin,L.M.,Li,Y.X.,et al.,2012.Classification and Evaluation of Shale Oil.Earth Science Frontiers,19(5):322-331(in Chinese with English abstract).
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