过硫酸盐活化技术的研究进展
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摘要
阐述了国内外活化过硫酸盐的技术如过渡金属活化、热活化、紫外光活化、活性炭活化的研究进展,简述了新型的碳纳米管活化、复合活化方式,并提出了过硫酸盐活化技术存在的问题和该技术的发展方向。
This paper introduces mainly the research progresses on persulfate activation technologies such as transition metal activation,hot activation,UV activation,and activated carbon activation at home and abroad and describes new types of activation technologies such as carbon nanotube activation and some multiplex activation technologies.Finally,this paper points out the existing deficiencies of the persulfate activation technologies and gives prospects for the development direction.
This paper introduces mainly the research progresses on persulfate activation technologies such as transition metal activation,hot activation,UV activation,and activated carbon activation at home and abroad and describes new types of activation technologies such as carbon nanotube activation and some multiplex activation technologies.Finally,this paper points out the existing deficiencies of the persulfate activation technologies and gives prospects for the development direction.
引文
[1]孙怡,于利亮,黄浩斌,等.高级氧化技术处理降解有机废水的研发趋势及实用化进展[J].化工学报,2017,68(5):1743-1756.
[2]Zhang B T,Zhang Y Q,Huang S B,et al.Sulfate radical and its application in decontamination technologies[J].Critical Reviews in Environmental Science and Technology,2015,45:1756-1800.
[3]Tang X,Hashmi M Z,Zeng B,et al.Application of iron-activated persulfate oxidation for the degradation of PCBs in soil[J].Chemical Engineering Journal,2015,279:673-680.
[4]姚宁波,李学艳,李青松,等.Fe(Ⅱ)活化过硫酸盐去除水中三氯生[J].环境工程学报,2016,10(9):4737-4744.
[5]Liang C,Clifford J Bruell,Michael C Marley,et al.Persulfate oxidation for in situ remediation of TCEⅡactivated by chelated ferrous ion[J].Chemosphere,2004,55(9):1225-1233.
[6]阳海,黎源,徐淼,等.Fe2+/S2O2-8/EDTA体系中自由基离子对啶虫脒的氧化降解[J].环境科学研究,2014,27(3):321-327.
[7]刘占孟,占鹏,李静,等.零价铁活化过硫酸盐处理渗滤液生化尾水[J].中国给水排水,2016,32(9):112-115.
[8]Liang Haiyun,Zhang Yongqing,Huang Shaobin,et al.Oxidative degradation of p-chloroaniline by copper oxidate activated persulfate[J].Chemical Engineering Journal,2013,218:384-391.
[9]朱思瑞,高乃云,鲁仙,等.热激活过硫酸盐氧化降解水中双酚A[J].中国环境科学,2017,37(1):188-194.
[10]Nick Zrinyi,Anh Le-Tuan Pham.Oxidation of benzoic acid by heatactivated persulfate:Effect of temperature on transformation pathway and product distribution[J].Water Research,2017,120:43-51.
[11]张萍萍,葛建华,郭学涛,等.热活化过硫酸盐降解联苯胺的研究[J].水处理技术,2016,42(3):65-68,75.
[12]Huang Kunchang,Zhao Zhiqiang,George E Hoag,et al.Degradation of volatile organic compounds with thermally activated persulfate oxidation[J].Chemosphere,2005,61:551-560.
[13]祁承都,刘希涛,郑文娟.微波加热活化过硫酸盐降解水中五氯酚的研究[A]//清华大学持久性有机污染物研究中心.持久性有机污染物论坛2012暨第七届持久性有机污染物全国学术研讨会论文集[C].天津:清华大学持久性有机污染物研究中心,2012:284-285.
[14]Lin Yating,Liang Chenju,Chen Jiunhua.Feasibility study of ultraviolet activated persulfate oxidation of phenol[J].Chemosphere,2011,82:1168-1172.
[15]Luo Congwei,Jiang Jin,Ma Jun,et al.Oxidation of the odorous compound 2,4,6-trichloroanisole by UV activated persulfate:Kinetics,products,and pathways[J].Water Research,2016,96:12-21.
[16]Wang Chiwei,Liang Chenju.Oxidative degradation of TMAH solution with UV persulfate activation[J].Chemical Engineering Journal,2014,254:472-478.
[17]郭佑罗,高乃云,关小红,等.紫外激活过硫酸盐降解水中双氯芬酸钠[J].哈尔滨工业大学学报,2017,49(8):65-70.
[18]Gao Yuqiang,Gao Naiyun,Deng Yang,et al.Ultraviolet(UV)light-activated persulfate oxidation of sulfamethazine in water[J].Chemical Engineering Journal,2012,195-196:248-253.
[19]张海璇,刘娟,欧桦瑟.紫外-过硫酸盐降解水中环丙沙星动力学和效果[J].水处理技术,2017,43(5):43-47.
[20]Wang Zongping,Chen Yiqun,Xie Pengchao,et al.Removal of Microcystis aeruginosa by UV-activated persulfate:Performance and characteristics[J].Chemical Engineering Journal,2016,300:245-253.
[21]杨梅梅,周少奇,刘聃,等.活性炭催化过硫酸钠降解金橙G动力学[J].环境科学,2013,34(3):962-967.
[22]杨世迎,杨鑫,邵雪停,等.活性炭激活过硫酸盐水处理技术操作方式的影响[A]//2010中国环境科学学会学术年会论文集(第三卷)[C].上海:中国环境科学学会,2010:2999-3002.
[23]王宇轩,王应军,方明珠.活性炭负载Cu O催化过硫酸盐去除活性艳红X-3B染料[J].环境工程学报,2016,10(1):230-236.
[24]李志军.负载Fe(Ⅱ)颗粒性活性炭活化过硫酸盐处理老龄垃圾渗滤液的研究[D].长沙:湖南大学,2016.
[25]陈家斌,魏成耀,房聪,等.碳纳米管活化过二硫酸盐降解偶氮染料酸性橙7[J].中国环境科学,2016,36(12):3618-3524.
[26]朱英良,万金泉,马邕文,等.电化学协同过硫酸盐法氧化处理橙黄G染料废水[J].水处理技术,2016,42(8):48-51,56.
[27]唐海,李洋,汤同欢,等.Cu O/UV/过硫酸盐体系深度降解印染废水[J].中国给水排水,2016,32(19):89-94.
[28]万金泉,濮梦婕,马邕文,等.PS高级氧化-离子沉淀-V型砂滤组合工艺深度处理AO7染料废水应用研究[J].环境工程学报,2016,10(3):1138-1144.
[29]王蔚,张洛红,杨阿敏,等.混凝-热活化过硫酸盐氧化预处理乳化液废水[J].西安工程大学学报,2016,30(6):767-771.
[30]Fang Jingyun,Shang Chii.Bromate formation from bromide oxidation by the UV/persulfate process[J].Environmental Science and Technology,2012,46:8976-8983.
[2]Zhang B T,Zhang Y Q,Huang S B,et al.Sulfate radical and its application in decontamination technologies[J].Critical Reviews in Environmental Science and Technology,2015,45:1756-1800.
[3]Tang X,Hashmi M Z,Zeng B,et al.Application of iron-activated persulfate oxidation for the degradation of PCBs in soil[J].Chemical Engineering Journal,2015,279:673-680.
[4]姚宁波,李学艳,李青松,等.Fe(Ⅱ)活化过硫酸盐去除水中三氯生[J].环境工程学报,2016,10(9):4737-4744.
[5]Liang C,Clifford J Bruell,Michael C Marley,et al.Persulfate oxidation for in situ remediation of TCEⅡactivated by chelated ferrous ion[J].Chemosphere,2004,55(9):1225-1233.
[6]阳海,黎源,徐淼,等.Fe2+/S2O2-8/EDTA体系中自由基离子对啶虫脒的氧化降解[J].环境科学研究,2014,27(3):321-327.
[7]刘占孟,占鹏,李静,等.零价铁活化过硫酸盐处理渗滤液生化尾水[J].中国给水排水,2016,32(9):112-115.
[8]Liang Haiyun,Zhang Yongqing,Huang Shaobin,et al.Oxidative degradation of p-chloroaniline by copper oxidate activated persulfate[J].Chemical Engineering Journal,2013,218:384-391.
[9]朱思瑞,高乃云,鲁仙,等.热激活过硫酸盐氧化降解水中双酚A[J].中国环境科学,2017,37(1):188-194.
[10]Nick Zrinyi,Anh Le-Tuan Pham.Oxidation of benzoic acid by heatactivated persulfate:Effect of temperature on transformation pathway and product distribution[J].Water Research,2017,120:43-51.
[11]张萍萍,葛建华,郭学涛,等.热活化过硫酸盐降解联苯胺的研究[J].水处理技术,2016,42(3):65-68,75.
[12]Huang Kunchang,Zhao Zhiqiang,George E Hoag,et al.Degradation of volatile organic compounds with thermally activated persulfate oxidation[J].Chemosphere,2005,61:551-560.
[13]祁承都,刘希涛,郑文娟.微波加热活化过硫酸盐降解水中五氯酚的研究[A]//清华大学持久性有机污染物研究中心.持久性有机污染物论坛2012暨第七届持久性有机污染物全国学术研讨会论文集[C].天津:清华大学持久性有机污染物研究中心,2012:284-285.
[14]Lin Yating,Liang Chenju,Chen Jiunhua.Feasibility study of ultraviolet activated persulfate oxidation of phenol[J].Chemosphere,2011,82:1168-1172.
[15]Luo Congwei,Jiang Jin,Ma Jun,et al.Oxidation of the odorous compound 2,4,6-trichloroanisole by UV activated persulfate:Kinetics,products,and pathways[J].Water Research,2016,96:12-21.
[16]Wang Chiwei,Liang Chenju.Oxidative degradation of TMAH solution with UV persulfate activation[J].Chemical Engineering Journal,2014,254:472-478.
[17]郭佑罗,高乃云,关小红,等.紫外激活过硫酸盐降解水中双氯芬酸钠[J].哈尔滨工业大学学报,2017,49(8):65-70.
[18]Gao Yuqiang,Gao Naiyun,Deng Yang,et al.Ultraviolet(UV)light-activated persulfate oxidation of sulfamethazine in water[J].Chemical Engineering Journal,2012,195-196:248-253.
[19]张海璇,刘娟,欧桦瑟.紫外-过硫酸盐降解水中环丙沙星动力学和效果[J].水处理技术,2017,43(5):43-47.
[20]Wang Zongping,Chen Yiqun,Xie Pengchao,et al.Removal of Microcystis aeruginosa by UV-activated persulfate:Performance and characteristics[J].Chemical Engineering Journal,2016,300:245-253.
[21]杨梅梅,周少奇,刘聃,等.活性炭催化过硫酸钠降解金橙G动力学[J].环境科学,2013,34(3):962-967.
[22]杨世迎,杨鑫,邵雪停,等.活性炭激活过硫酸盐水处理技术操作方式的影响[A]//2010中国环境科学学会学术年会论文集(第三卷)[C].上海:中国环境科学学会,2010:2999-3002.
[23]王宇轩,王应军,方明珠.活性炭负载Cu O催化过硫酸盐去除活性艳红X-3B染料[J].环境工程学报,2016,10(1):230-236.
[24]李志军.负载Fe(Ⅱ)颗粒性活性炭活化过硫酸盐处理老龄垃圾渗滤液的研究[D].长沙:湖南大学,2016.
[25]陈家斌,魏成耀,房聪,等.碳纳米管活化过二硫酸盐降解偶氮染料酸性橙7[J].中国环境科学,2016,36(12):3618-3524.
[26]朱英良,万金泉,马邕文,等.电化学协同过硫酸盐法氧化处理橙黄G染料废水[J].水处理技术,2016,42(8):48-51,56.
[27]唐海,李洋,汤同欢,等.Cu O/UV/过硫酸盐体系深度降解印染废水[J].中国给水排水,2016,32(19):89-94.
[28]万金泉,濮梦婕,马邕文,等.PS高级氧化-离子沉淀-V型砂滤组合工艺深度处理AO7染料废水应用研究[J].环境工程学报,2016,10(3):1138-1144.
[29]王蔚,张洛红,杨阿敏,等.混凝-热活化过硫酸盐氧化预处理乳化液废水[J].西安工程大学学报,2016,30(6):767-771.
[30]Fang Jingyun,Shang Chii.Bromate formation from bromide oxidation by the UV/persulfate process[J].Environmental Science and Technology,2012,46:8976-8983.