层状双金属氢氧化物在电催化中的应用
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摘要
在能源紧张和环境问题突出的今天,开发可再生的清洁能源和储能装置已引起研究者们的广泛关注。电催化及其催化材料在新能源开发和使用中起着举足轻重的作用。而二维层状材料因其具有较高的比表面积和独特的电子特性可作为很好的电极材料,在电催化和储能中应用广泛。其中,层状双金属氢氧化物(layered double hydroxides,LDHs)以其典型的层状结构特征,且价格低廉、合成方法简单并易于功能化、组成易于调控、结构可裁剪等优点在电催化及催化材料的制备中具有很好的发展前景。本文主要从LDHs作为阳极析氧反应(oxygen evolution reaction,OER)催化剂、电催化剂载体以及作为制备电催化剂的前驱体三个方面综述了层状双金属氢氧化物应用于电催化材料的研究进展,对调控LDHs材料的电子结构、形貌、界面相互作用以及与贵金属催化剂之间的协同催化等提高其催化性能作了相关阐述,并对以LDHs为前驱体制备电催化剂作了简要阐述。最后,对LDHs应用于电催化所存在的问题及前景进行了展望。
The development of renewable clean energy and energy storage devices has attracted extensive attention because of bad condition of energy shortages and harsh environmental problems. Electrocatalytic reaction and catalyst materials play vital roles in the process of catalysis. Two dimensional layered materials have been widely used as electrode materials in electrocatalysis and energy storage devices thanks to their high specific surface area and unique electronic properties. Among them,layered double hydroxides( LDHs) have a good development prospect in the electrocatalysis process and preparation of catalyst materials due to their typical layered structure and unique advantages such as lowprice,easy to be prepared and functionalized,good tunability in the composition and structure,etc. This reviewsummarizes the research progress of LDHs applied in catalyst for oxygen evolution reaction( OER),catalyst supporter and used as precursor to prepare electrocatalyst.Especially,we discusse the recent advances in tuning LDHs including electronic structure,morphology,interface interaction and synergetic catalytic effect with noble metal catalyst to improve the catalytic performance. In addition,we briefly describe the preparation of electrocatalysts using LDHs as precursors. Finally,the current difficulties and future research directions of LDHs are also discussed to give an outlook of their prospect in electrocatalysis.
The development of renewable clean energy and energy storage devices has attracted extensive attention because of bad condition of energy shortages and harsh environmental problems. Electrocatalytic reaction and catalyst materials play vital roles in the process of catalysis. Two dimensional layered materials have been widely used as electrode materials in electrocatalysis and energy storage devices thanks to their high specific surface area and unique electronic properties. Among them,layered double hydroxides( LDHs) have a good development prospect in the electrocatalysis process and preparation of catalyst materials due to their typical layered structure and unique advantages such as lowprice,easy to be prepared and functionalized,good tunability in the composition and structure,etc. This reviewsummarizes the research progress of LDHs applied in catalyst for oxygen evolution reaction( OER),catalyst supporter and used as precursor to prepare electrocatalyst.Especially,we discusse the recent advances in tuning LDHs including electronic structure,morphology,interface interaction and synergetic catalytic effect with noble metal catalyst to improve the catalytic performance. In addition,we briefly describe the preparation of electrocatalysts using LDHs as precursors. Finally,the current difficulties and future research directions of LDHs are also discussed to give an outlook of their prospect in electrocatalysis.
引文
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