选择性油水分离材料
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摘要
水是人类赖以生存的基础,其重要性不言而喻。但是,当前水环境日益恶化,水污染日益加重,尤其是石油泄漏和有机污染物肆意排放给环境和生态系统造成了不可挽回的损害。因此,高效油水分离已成为亟待解决的问题。当前主要通过物理吸附、化学分散以及生物降解等方法进行油污清理;化学分散和生物降解法易对海洋环境造成二次污染,而物理吸附具有易于回收及无污染等优点。本文综述了近年来物理过滤和物理吸附油水分离材料的研究现状及尚待解决的难点,同时也展望了该领域未来研究的热点及发展方向。
Water resource is a prerequisite for the survival of human beings with a self-evident importance. In recent years, water environment continues to deteriorate and water pollution is becoming more and more severe, oil spillages and indiscriminate discharge of organic pollutants cause serious and irrecoverable damages to environment and ecosystems, and the way for effective separation of oil-water mixture is becoming an urgent problem. The frequently-used methods for oil/water separation are physical adsorption, chemical dispersion and biodegradation, in which chemical adsorption and biodegradation methods usually cause secondary pollution to the marine environment; and the physical adsorption material has the advantages of easily collection, pollution-free and so on. This article summarizes the research status of physical filtration and physical adsorption materials for oil/water separation, some related difficulties that remain to be solved are pointed out and its future researching focus and developing directions are proposed.
Water resource is a prerequisite for the survival of human beings with a self-evident importance. In recent years, water environment continues to deteriorate and water pollution is becoming more and more severe, oil spillages and indiscriminate discharge of organic pollutants cause serious and irrecoverable damages to environment and ecosystems, and the way for effective separation of oil-water mixture is becoming an urgent problem. The frequently-used methods for oil/water separation are physical adsorption, chemical dispersion and biodegradation, in which chemical adsorption and biodegradation methods usually cause secondary pollution to the marine environment; and the physical adsorption material has the advantages of easily collection, pollution-free and so on. This article summarizes the research status of physical filtration and physical adsorption materials for oil/water separation, some related difficulties that remain to be solved are pointed out and its future researching focus and developing directions are proposed.
引文
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[2] Ivshina I B, Kuyukina M S, Krivoruchko A V, Elkin A A, Makarov S O, Cunningham C J, Peshkur T A, Atlas R M, Philp J C. Environmental Science Processes & Impacts, 2015, 17(7): 1201.
[3] Nisticò R, Franzoso F, Cesano F, Scarano D, Magnacca G, Parolo M E, Carlos L. ACS Sustainable Chemistry & Engineering, 2017, 5(1): 793.
[4] Li Y, Zhang Z, Wang M, Men X, Xue Q. Journal of Materials Chemistry A, 2017, 5(10): 5077.
[5] Ge J, Zhao H Y, Zhu H W, Huang J, Shi L A, Yu S H. Advanced Materials, 2016, 28(47): 10459.
[6] Ma Q, Cheng H, Fane A G, Wang R, Zhang H. Small, 2016, 12(16): 2186.
[7] Xia B B, Liu H T, Fan Y N, Chen T C, Chen C, Wang B. Materials & Design, 2017, 135:51.
[8] Wang Z, Guo Z. Chemical Communications, 2017, 53(4): 12990.
[9] Wang K, Wang Z, Dong Y, Zhang S, Li J. Polymers, 2017, 9(8): 347.
[10] Tang X, Shen C, Zhu W, Zhang S, Xu Y, Yang Y, Gao M, Dong F. RSC Advances, 2017, 7(48): 30495.
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[12] Chen L, Guo Z, Liu W. Journal of Materials Chemistry A, 2017, 5(28): 14480.
[13] 詹晓力(Zhan X L), 金碧玉(Jin B Y), 张庆华(Zhang Q H), 陈丰秋(Chen F Q). 化学进展(Progress in Chemistry), 2018, 1: 87.
[14] Zhang T, Kong L, Dai Y, Yue X, Rong J, Qiu F, Pan J. Chemical Engineering Journal, 2017, 309:7.
[15] Li H, Yu S, Han X. Chemical Engineering Journal, 2016, 283:1443.
[16] Ebihara Y, Ota R, Noriki T, Shimojo M, Kajikawa K. Scientific Reports, 2015, 5:15992.
[17] Lai C Y, Tang T C, Amadei C A, Marsden A J, Verdaguer A, Wilson N, Chiesa M. Carbon, 2014, 80:784.
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[27] Saththasivam J, Yiming W, Wang K, Jin J, Liu Z. Scientific Reports, 2018, 8(1): 7418.
[28] Kong L H, Chen X H, Yu L G, Wu Z S, Zhang P Y. ACS Appl Mater Interfaces, 2015, 7(4): 2616.
[29] Gao X, Zhou J, Du R, Xie Z, Deng S, Liu R, Liu Z, Zhang J. Advanced Materials, 2016, 28(1): 168.
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[32] Xu Z, Wang L, Yu C, Li K, Tian Y, Jiang L. Advanced Functional Materials, 2018, 28(5): 1703970.
[33] Lv W, Mei Q, Xiao J, Du M, Zheng Q. Advanced Functional Materials, 2017, 27(48): 1704293.
[34] Yang Y, Li X, Zheng X, Chen Z, Zhou Q, Chen Y. Advanced Materials, 2018, 30(9).
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[41] Wang C F, Tzeng F S, Chen H G, Chang C J. Langmuir the ACS Journal of Surfaces & Colloids, 2012, 28(26): 10015.
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[43] Yang J, Zhang Z, Xu X, Zhu X, Men X, Zhou X. Journal of Materials Chemistry, 2012, 22(7): 2834.
[44] Zhang F, Zhang W B, Shi Z, Wang D, Jin J, Jiang L. Advanced Materials, 2013, 25(30): 4192.
[45] Liu X, Ge L, Li W, Wang X, Li F. ACS Appl Mater Interfaces, 2015, 7(1): 791.
[46] Chen Q, Yu Z, Li F, Yang Y, Pan Y, Peng Y, Yang X, Zeng G. Journal of Chemical Technology and Biotechnology, 2018, 93(3): 761.
[47] Lee W, Ahn Y. Bulletin of the Korean Chemical Society, 2017, 38(12): 1503.
[48] Wang J, Chen Y. Journal of Applied Polymer Science, 2015, 132(39): 42614.
[49] Li J, Yan L, Zhao Y, Zha F, Wang Q, Lei Z. Physical Chemistry Chemical Physics, 2015, 17(9): 6451.
[50] Wang B, Li J, Wang G, Liang W, Zhang Y, Shi L, Guo Z, Liu W. ACS Appl Mater Interfaces, 2013, 5(5): 1827.
[51] Zhang W, Shi Z, Zhang F, Liu X, Jin J, Jiang L. Advanced Materials, 2013, 25(14): 2071.
[52] Chen B, Ma Q, Tan C, Lim T T, Huang L, Zhang H. Small, 2015, 11(27): 3319.
[53] Reddy D H K, Yun Y S. Coordination Chemistry Reviews, 2016, 315: 90.
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[59] Duan C, Zhu T, Guo J, Wang Z, Liu X, Wang H, Xu X, Jin Y, Zhao N, Xu J. ACS Applied Materials & Interfaces, 2015, 7(19): 10475.
[60] Wang B, Liu Y, Zhang Y, Guo Z, Zhang H, Xin J H, Zhang L. Advanced Materials Interfaces, 2015, 2(13): 1500234.
[61] Ning C, Qian L, Jin L, Yong W, Bai Y, Szunerits S, Boukherroub R. Chemical Engineering Journal, 2017, 326: 17.
[62] Wan W, Lin Y, Prakash A, Zhou Y. Journal of Materials Chemistry A, 2016, 4(48): 18687.
[63] Shen Y, Li L, Xiao K, Xi J. ACS Sustainable Chemistry & Engineering, 2016, 4(4): 2351.
[64] Gupta S, Tai N H. Journal of Materials Chemistry A, 2016, 4(5): 1550.
[65] Fard A K, Rhadfi T, Mckay G, Al-Marri M, Abdala A, Hilal N, Hussien M A. Chemical Engineering Journal, 2016, 293: 90.
[66] Cao X, Zang L, Bu Z, Sun L, Guo D, Wang C. Journal of Materials Chemistry A, 2016, 4(27): 10479.
[67] Ma W, Zhang Q, Hua D, Xiong R, Zhao J, Rao W, Huang S, Zhan X, Chen F, Huang C. RSC Advances, 2016, 6(16): 12868.
[68] Shuai Q, Yang X, Luo Y, Tang H, Luo X, Tan Y, Ma M. Materials Chemistry & Physics, 2015, 162: 94.
[69] Ruan C, Ai K, Li X, Lu L. Angew. Chem. Int. Ed., 2014, 126(22): 5662.
[70] Ge J, Shi L A, Wang Y C, Zhao H Y, Yao H B, Zhu Y B, Zhang Y, Zhu H W, Wu H A, Yu S H. Nature Nanotechnology, 2017, 12(5): 434.
[71] Ge J, Ye Y D, Yao H B, Zhu X, Wang X, Wu L, Wang J L, Ding H, Yong N, He L H. Angewandte Chemie International Edition, 2014, 53(14): 3612.
[72] Bi H, Xie X, Yin K, Zhou Y, Wan S, Ruoff R, Sun L. Journal of Materials Chemistry A, 2014, 2(6): 1652.
[73] Sun H, Xu Z, Gao C. Advanced Materials, 2013, 25(18): 2554.
[74] Li Y Q, Samad Y A, Polychronopoulou K, Alhassan S M, Liao K. ACS Sustainable Chemistry & Engineering, 2014, 2(6): 1492.
[75] Bi H, Yin Z, Cao X, Xie X, Tan C, Huang X, Chen B, Chen F, Yang Q, Bu X. Advanced Materials, 2013, 25(41): 5916.