凹凸棒土-稻壳活性炭复合滤料与陶粒滤料对水中亚甲基蓝的吸附性能研究
|
摘要
用以凹凸棒土为主要原料制备的凹凸棒土-稻壳活性炭复合滤料和陶粒滤料分别对亚甲基蓝进行吸附实验。研究了温度、pH值、吸附时间和2种滤料投加量对亚甲基蓝吸附性的影响,并对2种不同滤料的吸附性能进行比较。实验数据表明,凹凸棒土-稻壳活性炭复合滤料在大多数外界条件下对亚甲基蓝的吸附率都高于陶粒滤料,对于亚甲基蓝吸附效果更好。
The adsorption experiments on methylene blue were carried out on the composite filter media mainly composed of attapulgite clay-rice husk activated carbon composite filter and the ceramic particle filter.The effects of temperature,pH value,adsorption time and the dosage of two kinds of media on the adsorption of methylene blue were studied.The adsorption properties of two different media were compared.The experimental data show that the attraction rate of attapulgite clay-rice husk activated carbon composite filter media is higher than that of ceramic particle filter under most external conditions,and the adsorption effect on methylene blue is better.
The adsorption experiments on methylene blue were carried out on the composite filter media mainly composed of attapulgite clay-rice husk activated carbon composite filter and the ceramic particle filter.The effects of temperature,pH value,adsorption time and the dosage of two kinds of media on the adsorption of methylene blue were studied.The adsorption properties of two different media were compared.The experimental data show that the attraction rate of attapulgite clay-rice husk activated carbon composite filter media is higher than that of ceramic particle filter under most external conditions,and the adsorption effect on methylene blue is better.
引文
[1]郑为升,王海玲,朱兆连,等.新型凹凸棒土颗粒吸附剂对亚甲基蓝和刚果红的吸附研究[J].工业安全与环保,2016,42(12):59-62.
[2]车晓冬,丁竹红,胡祈,等.微波加热硝酸氧化改性稻壳基生物质炭对Pb(Ⅱ)和亚甲基蓝的吸附作用[J].农业环境科学学报,2016,35(9):1 773-1 780.
[3]王郑.我国微污染水源水处理技术研究进展[J].工业水处理,2012,32(10):1-3.
[4]贾佳祺,李坤权,陆凯,等.微波活化中孔酸性生物质炭对亚甲基蓝的吸附行为与机理[J].环境工程学报,2014,8(3):909-916.
[5]王郑,仲米贵,黄雷,等.聚合氯化铝-壳聚糖复合絮凝剂对活性蓝19的脱色研究[J].工业水处理,2017,37(9):21-25.
[6]常春,刘天琪,王瑀婷,等.水热法制备玉米叶基生物炭对亚甲基蓝的吸附性能研究[J].环境科学学报,2017,37(7):2 680-2 692.
[7]王郑,仲米贵,黄雷,等.聚合氯化铝9壳聚糖复合絮凝剂对腐殖酸的絮凝特性研究[J].环境工程,2017,35(10):61-65.
[8]徐继红,穆新科,洪思明,等.木质素基水凝胶对亚甲基蓝染料的吸附性能[J].环境工程学报,2015,9(10):4 877-4 822.
[9]王郑,程星星,黄雷,等.催化臭氧化技术在水处理中的应用研究进展[J].应用化工,2017,46(6):1 214-1217.
[10]Wang Z,Zhong M G,Wan J F,et al.Development of attapulgite composite ceramsite/quartz sand double-layer biofilter for micropolluted drinking source water purification[J].International Journal of Environmental Science and Technology,2016,13(3):825-834.
[11]宋娟,李晓晖,宁喜斌.壳聚糖质活性炭对亚甲基蓝的吸附性能研究[J].应用化工,2014,43(8):1 446-1 452.
[12]刘娟丽,曹天鹏,李佳.秸秆生物质炭的活化制备及其对亚甲基蓝的吸附研究[J].水处理技术,2015,41(9):53-60.
[13]王郑,仲米贵,黄雷,等.聚合氯化铝-壳聚糖复合絮凝剂的制备及其铝形态分布[J].科学技术与工程,2017,17(20):194-200.
[14]王丰喜,倪佩军,刘张敏,等.硅质壳及硅藻土对亚甲基蓝吸附性能比较[J].环境工程学报,10(4):1 693-1 698.
[15]马宏飞,李晨晨,李薇,等.高岭土对亚甲基蓝的吸附性能和等温吸附模型研究[J].应用化工,2016,45(3):496-500.
[16]王郑,徐海强,徐晶晶,等.凹凸棒土烧结滤料对酸性红88吸附性能研究[J].应用化工,2014,43(4):616-620.
[17]吕琳琳,姜效军,刁全平,等.改性榛壳对水中孔雀石绿和亚甲基蓝吸附性能的研究[J].应用化工,2017,46(7):1 343-1 350.
[18]邹德靓,陈庆国,杨平,等.改性贻贝壳对亚甲基蓝的吸附去除研究[J].环境科学与技术,2014,37(12):214-252.
[19]陈莉,司慧,靳峰,等.改性甘薯渣对亚甲基蓝的吸附特性及吸附机制[J].环境工程学报,2016,10(8):4 278-4 283.
[20]夏天明,王营茹.改性稻壳吸附柱处理亚甲基蓝废水试验研究[J].环境科学与技术,2014,37(120):417-421.
[21]王欣,陈元涛,张炜,等.改性埃洛石材料的制备及其对亚甲基蓝吸附行为的研究[J].分析测试学报,2016,35(6):729-733.
[22]Wang Z.Efficient adsorption of dibutyl phthalate from aqueous solution by activated carbon developed from phoenix leaves[J].Environmental Science and Technology,2015,12(6),1 923-1 932.
[23]马清亮,廖俊杰,纵瑞涵,等.粉煤灰-聚丙烯酸复合微凝胶对亚甲基蓝的吸附探究[J].硅酸盐通报,2016,35(2):380-391.
[24]马文清,赫文芳,王雲生,等.磁性埃洛石复合材料的制备及其对亚甲基蓝吸附性能研究[J].硅酸盐通报,36(1):242-248.
[25]Wang Z,Chen L.Adsorption characteristics of dibutyl phthalate from aqueous solution using ginkgo leaves-activated carbon by chemical activation with zinc chloride[J].Desalination and Water Treatment,2015,54(7):1 969-1 980.
[26]黎强,周少奇,李夫振,等.不同方法处理飞灰对亚甲基蓝的吸附性能[J].环境工程学报,2015,9(1):367-373.
[27]Wang Z,Zhong MG,Chen L.Coal-based granular activated carbon loaded with Mn O2as an efficient adsorbent for removing formaldehyde from aqueous solution[J].Desalination and Water Treatment,2016,57(28):13 225-13 235.
[28]孙续兵,吴彩文,何柏琼.柠檬皮渣对亚甲基蓝吸附性能研究[J].工业用水与废水,2014,45(6):62-66.
[2]车晓冬,丁竹红,胡祈,等.微波加热硝酸氧化改性稻壳基生物质炭对Pb(Ⅱ)和亚甲基蓝的吸附作用[J].农业环境科学学报,2016,35(9):1 773-1 780.
[3]王郑.我国微污染水源水处理技术研究进展[J].工业水处理,2012,32(10):1-3.
[4]贾佳祺,李坤权,陆凯,等.微波活化中孔酸性生物质炭对亚甲基蓝的吸附行为与机理[J].环境工程学报,2014,8(3):909-916.
[5]王郑,仲米贵,黄雷,等.聚合氯化铝-壳聚糖复合絮凝剂对活性蓝19的脱色研究[J].工业水处理,2017,37(9):21-25.
[6]常春,刘天琪,王瑀婷,等.水热法制备玉米叶基生物炭对亚甲基蓝的吸附性能研究[J].环境科学学报,2017,37(7):2 680-2 692.
[7]王郑,仲米贵,黄雷,等.聚合氯化铝9壳聚糖复合絮凝剂对腐殖酸的絮凝特性研究[J].环境工程,2017,35(10):61-65.
[8]徐继红,穆新科,洪思明,等.木质素基水凝胶对亚甲基蓝染料的吸附性能[J].环境工程学报,2015,9(10):4 877-4 822.
[9]王郑,程星星,黄雷,等.催化臭氧化技术在水处理中的应用研究进展[J].应用化工,2017,46(6):1 214-1217.
[10]Wang Z,Zhong M G,Wan J F,et al.Development of attapulgite composite ceramsite/quartz sand double-layer biofilter for micropolluted drinking source water purification[J].International Journal of Environmental Science and Technology,2016,13(3):825-834.
[11]宋娟,李晓晖,宁喜斌.壳聚糖质活性炭对亚甲基蓝的吸附性能研究[J].应用化工,2014,43(8):1 446-1 452.
[12]刘娟丽,曹天鹏,李佳.秸秆生物质炭的活化制备及其对亚甲基蓝的吸附研究[J].水处理技术,2015,41(9):53-60.
[13]王郑,仲米贵,黄雷,等.聚合氯化铝-壳聚糖复合絮凝剂的制备及其铝形态分布[J].科学技术与工程,2017,17(20):194-200.
[14]王丰喜,倪佩军,刘张敏,等.硅质壳及硅藻土对亚甲基蓝吸附性能比较[J].环境工程学报,10(4):1 693-1 698.
[15]马宏飞,李晨晨,李薇,等.高岭土对亚甲基蓝的吸附性能和等温吸附模型研究[J].应用化工,2016,45(3):496-500.
[16]王郑,徐海强,徐晶晶,等.凹凸棒土烧结滤料对酸性红88吸附性能研究[J].应用化工,2014,43(4):616-620.
[17]吕琳琳,姜效军,刁全平,等.改性榛壳对水中孔雀石绿和亚甲基蓝吸附性能的研究[J].应用化工,2017,46(7):1 343-1 350.
[18]邹德靓,陈庆国,杨平,等.改性贻贝壳对亚甲基蓝的吸附去除研究[J].环境科学与技术,2014,37(12):214-252.
[19]陈莉,司慧,靳峰,等.改性甘薯渣对亚甲基蓝的吸附特性及吸附机制[J].环境工程学报,2016,10(8):4 278-4 283.
[20]夏天明,王营茹.改性稻壳吸附柱处理亚甲基蓝废水试验研究[J].环境科学与技术,2014,37(120):417-421.
[21]王欣,陈元涛,张炜,等.改性埃洛石材料的制备及其对亚甲基蓝吸附行为的研究[J].分析测试学报,2016,35(6):729-733.
[22]Wang Z.Efficient adsorption of dibutyl phthalate from aqueous solution by activated carbon developed from phoenix leaves[J].Environmental Science and Technology,2015,12(6),1 923-1 932.
[23]马清亮,廖俊杰,纵瑞涵,等.粉煤灰-聚丙烯酸复合微凝胶对亚甲基蓝的吸附探究[J].硅酸盐通报,2016,35(2):380-391.
[24]马文清,赫文芳,王雲生,等.磁性埃洛石复合材料的制备及其对亚甲基蓝吸附性能研究[J].硅酸盐通报,36(1):242-248.
[25]Wang Z,Chen L.Adsorption characteristics of dibutyl phthalate from aqueous solution using ginkgo leaves-activated carbon by chemical activation with zinc chloride[J].Desalination and Water Treatment,2015,54(7):1 969-1 980.
[26]黎强,周少奇,李夫振,等.不同方法处理飞灰对亚甲基蓝的吸附性能[J].环境工程学报,2015,9(1):367-373.
[27]Wang Z,Zhong MG,Chen L.Coal-based granular activated carbon loaded with Mn O2as an efficient adsorbent for removing formaldehyde from aqueous solution[J].Desalination and Water Treatment,2016,57(28):13 225-13 235.
[28]孙续兵,吴彩文,何柏琼.柠檬皮渣对亚甲基蓝吸附性能研究[J].工业用水与废水,2014,45(6):62-66.