基于微弧氧化和电化学沉积在纯Ti基体表面制备FHAP/MAO复合涂层的腐蚀行为和力学性能（英文）
|
摘要
采用微弧氧化和电化学沉积(ED)技术在工业纯钛(CPTi)表面沉积氟掺杂羟基磷灰石(FHAP)/微弧氧化(MAO)复合涂层。并在Hsnk’s溶液中对未涂覆的CPTi基材和涂覆的样品进行电化学耐腐蚀性测试。研究了MAO界面层对涂层微观结构,力学性能和电化学性能的影响。结果表明,HAP/Ti,FHAP/Ti和FHAP/MAO/Ti复合涂层样品在模拟Hank’s溶液中提高了CPTi基体的耐腐蚀性能。然而,力学性能测试表明,与具有MAO界面层的FHAP/Ti涂层的结合强度(18.1 MPa)相比,FHAP/Ti涂层的结合强度较差(10.7 MPa)。此外,FHAP/MAO/Ti涂层的接触角约为35.8°,这更有利于促进细胞附着和增殖。
A fluorine-doped hydroxyapatite(FHAP)/micro-arc oxidation(MAO) composite coating was deposited on commercially pure titanium(CPTi) surface through micro-arc oxidation and electrochemical deposition(ED) technique. Simulative Hank's solution was used to test the electrochemical corrosion resistance of uncoated CPTi substrate and coated samples. The effect of MAO interface layer on the micro-structure, mechanical property, and electrochemical property of the coating was studied. Results show that the deposited HAP/Ti, FHAP/Ti and FHAP/MAO/Ti coating samples dramatically improve the anticorrosion of the CPTi substrate in the simulative Hank's solution. However, the mechanical properties testing shows that FHAP/Ti coating has a poor bonding strength of 10.7 MPa compared to FHAP/Ti coating with a MAO interface layer(18.1 MPa). Furthermore, the contact angle of the FHAP/MAO/Ti coating with deionized water is approximately 35.8°, which is more beneficial to promoting cell attachment and proliferation.
A fluorine-doped hydroxyapatite(FHAP)/micro-arc oxidation(MAO) composite coating was deposited on commercially pure titanium(CPTi) surface through micro-arc oxidation and electrochemical deposition(ED) technique. Simulative Hank's solution was used to test the electrochemical corrosion resistance of uncoated CPTi substrate and coated samples. The effect of MAO interface layer on the micro-structure, mechanical property, and electrochemical property of the coating was studied. Results show that the deposited HAP/Ti, FHAP/Ti and FHAP/MAO/Ti coating samples dramatically improve the anticorrosion of the CPTi substrate in the simulative Hank's solution. However, the mechanical properties testing shows that FHAP/Ti coating has a poor bonding strength of 10.7 MPa compared to FHAP/Ti coating with a MAO interface layer(18.1 MPa). Furthermore, the contact angle of the FHAP/MAO/Ti coating with deionized water is approximately 35.8°, which is more beneficial to promoting cell attachment and proliferation.
引文
1 Bai Y,Park I S,Lee S J et al.Applied Surface Science[J],2011,257(15):7010
2 Koch C F,Johnson S,Kumar D et al.Materials Science&Engineering C[J],2007,27(3):484
3 Blind O,Klein L H,Dailey B et al.Dental Materials[J],2005,21(11):1017
4 Xie J,Meng X,Zhou Z et al.Materials Letters[J],2013,110:57
5 García F,Arias J L,Mayor B et al.Journal of Biomedical Materials Research[J],1998,43(1):69
6 Tong W,Yang Z,Zhang X et al.Journal of Biomedical Materials Research[J],1998,40(3):407
7 Song Y,Zhang S,Li J et al.Acta Biomaterialia[J],2010,6(5):1736
8 Wang J,Chao Y,Wan Q et al.Acta Biomaterialia[J],2009,5(5):1798
9 Heimann R B.Surface&Coatings Technology[J],2006,201(5):2012
10 Uhlmann D R,Suratwala T,Davidson K et al.Journal of Non-Crystalline Solids[J],1997,218(97):113
11 Alicja K,Ma?gorzata K,Grzegorz D et al.Electrochimica Acta[J],2016,204:294
12 Bakhsheshi-Rad H R,Hamzah E,Daroonparvar M et al.Vacuum[J],2014,110:127
13 Xu J L,Khor K A,Gu Y W et al.Biomaterials[J],2005,26(15):2197
14 Frayssinet P,Hardy D,Rouquet N et al.Biomaterials[J],1992,13(10):668
15 Mohan L,Durgalakshmi D,Geetha M et al.Ceramics International[J],2012,38(4):3435
16 Fazel M,Salimijazi H R,Golozar M A et al.Applied Surface Science[J],2015,324:751
17 Bakhsheshi-Rad H R,Hamzah E,Ebrahimi-Kahrizsangi R et al.Vacuum[J],2016,125:185
18 Gnedenkov S V,Sinebryukhov S L,Mashtalyar D V et al.Vacuum[J],2015,120:107
19 Rokosz K,Hryniewicz T,Raaen S.International Journal of Advanced Manufacturing Technology[J],2015,85(9):2425
20 ASTM international.Standard Test Method for Adhesion or Cohesion Strength of Thermal Spray Coatings,ASTM C663-01[S].Philadelphia:West Conshohocken,2001
21 He Daihua,Liu P,Liu X et al.Journal of Wuhan University of Technology-Mater Sci Ed[J],2014,29(2):398
22 Sternitzke V,Kaegi R,Audinot J N et al.Environmental Science&Technology[J],2012,46(2):802
23 Montazeri M,Dehghanian C,Shokouhfar M et al.Applied Surface Science[J],2011,257(16):7268
24 Gu Y,Chen L,Yue W et al.Journal of Alloys&Compounds[J],2016,664:770
25 Zhao Y,Wei L,Yi P et al.International Journal of Hydrogen Energy[J],2016,41(2):1142
26 Zomorodian A,Garcia M P,Moura S T et al.Acta Biomaterialia[J],2013,9(10):8660
27 Grips V K W,Selvi V E,Barshilia H C et al.Electrochimica Acta[J],2006,51(17):3461
28 Bakhsheshi-Rad H R,Hamzah E,Ismail A F et al.Journal of Alloys&Compounds[J],2015,648:1067
29 Zoltowski P.Journal of Electroanalytical Chemistry[J],1998,443(1):149
30 Bakhsheshi-Rad H R,Hamzah E,Daroonparvar M et al.Transactions of Nonferrous Metals Society of China[J],2014,24(8):2516
31 He D H,Wang P,Liu P et al.Surface&Coatings Technology[J],2015,277:203
32 Gibson L,Ashby M.Cellular Solids Structure and Properties[M].Sydney:Pergamon Press,1988
33 Lee H U,Jeong Y S,Park S Y et al.Current Applied Physics[J],2009,9(2):528
34 Kunzler T P,Drobek T,Schuler M et al.Biomaterials[J],2007,28(13):2175
35 Bakhsheshi-Rad H R,Hamzah E,Ismail A F et al.Ceramics International[J],2016,42(10):11 941
36 Gopi D,Karthika A,Rajeswari D et al.Rsc Advances[J],2014,66:34 751
2 Koch C F,Johnson S,Kumar D et al.Materials Science&Engineering C[J],2007,27(3):484
3 Blind O,Klein L H,Dailey B et al.Dental Materials[J],2005,21(11):1017
4 Xie J,Meng X,Zhou Z et al.Materials Letters[J],2013,110:57
5 García F,Arias J L,Mayor B et al.Journal of Biomedical Materials Research[J],1998,43(1):69
6 Tong W,Yang Z,Zhang X et al.Journal of Biomedical Materials Research[J],1998,40(3):407
7 Song Y,Zhang S,Li J et al.Acta Biomaterialia[J],2010,6(5):1736
8 Wang J,Chao Y,Wan Q et al.Acta Biomaterialia[J],2009,5(5):1798
9 Heimann R B.Surface&Coatings Technology[J],2006,201(5):2012
10 Uhlmann D R,Suratwala T,Davidson K et al.Journal of Non-Crystalline Solids[J],1997,218(97):113
11 Alicja K,Ma?gorzata K,Grzegorz D et al.Electrochimica Acta[J],2016,204:294
12 Bakhsheshi-Rad H R,Hamzah E,Daroonparvar M et al.Vacuum[J],2014,110:127
13 Xu J L,Khor K A,Gu Y W et al.Biomaterials[J],2005,26(15):2197
14 Frayssinet P,Hardy D,Rouquet N et al.Biomaterials[J],1992,13(10):668
15 Mohan L,Durgalakshmi D,Geetha M et al.Ceramics International[J],2012,38(4):3435
16 Fazel M,Salimijazi H R,Golozar M A et al.Applied Surface Science[J],2015,324:751
17 Bakhsheshi-Rad H R,Hamzah E,Ebrahimi-Kahrizsangi R et al.Vacuum[J],2016,125:185
18 Gnedenkov S V,Sinebryukhov S L,Mashtalyar D V et al.Vacuum[J],2015,120:107
19 Rokosz K,Hryniewicz T,Raaen S.International Journal of Advanced Manufacturing Technology[J],2015,85(9):2425
20 ASTM international.Standard Test Method for Adhesion or Cohesion Strength of Thermal Spray Coatings,ASTM C663-01[S].Philadelphia:West Conshohocken,2001
21 He Daihua,Liu P,Liu X et al.Journal of Wuhan University of Technology-Mater Sci Ed[J],2014,29(2):398
22 Sternitzke V,Kaegi R,Audinot J N et al.Environmental Science&Technology[J],2012,46(2):802
23 Montazeri M,Dehghanian C,Shokouhfar M et al.Applied Surface Science[J],2011,257(16):7268
24 Gu Y,Chen L,Yue W et al.Journal of Alloys&Compounds[J],2016,664:770
25 Zhao Y,Wei L,Yi P et al.International Journal of Hydrogen Energy[J],2016,41(2):1142
26 Zomorodian A,Garcia M P,Moura S T et al.Acta Biomaterialia[J],2013,9(10):8660
27 Grips V K W,Selvi V E,Barshilia H C et al.Electrochimica Acta[J],2006,51(17):3461
28 Bakhsheshi-Rad H R,Hamzah E,Ismail A F et al.Journal of Alloys&Compounds[J],2015,648:1067
29 Zoltowski P.Journal of Electroanalytical Chemistry[J],1998,443(1):149
30 Bakhsheshi-Rad H R,Hamzah E,Daroonparvar M et al.Transactions of Nonferrous Metals Society of China[J],2014,24(8):2516
31 He D H,Wang P,Liu P et al.Surface&Coatings Technology[J],2015,277:203
32 Gibson L,Ashby M.Cellular Solids Structure and Properties[M].Sydney:Pergamon Press,1988
33 Lee H U,Jeong Y S,Park S Y et al.Current Applied Physics[J],2009,9(2):528
34 Kunzler T P,Drobek T,Schuler M et al.Biomaterials[J],2007,28(13):2175
35 Bakhsheshi-Rad H R,Hamzah E,Ismail A F et al.Ceramics International[J],2016,42(10):11 941
36 Gopi D,Karthika A,Rajeswari D et al.Rsc Advances[J],2014,66:34 751