金属-有机骨架及其功能材料在食品和水有害物质预处理中的应用
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摘要
食品安全问题是关系人民生命健康和经济社会和谐发展的重大问题。食品类样品残存的痕量有毒有害物质对人体健康产生潜在危害。因此,需要高效的吸附材料用于食品类样品预处理及检测。金属-有机骨架材料(metal-organic frameworks, MOFs)是一类新型的多孔功能材料,具有高孔隙度、高比表面积、结构可设计与调控、孔径可调及良好的化学和热稳定性等优点。MOFs的早期研究主要集中在结构及功能化设计方面,近年来MOFs及其功能材料在各领域的潜在应用逐渐成为新的研究热点。MOFs具有高度发达的孔隙结构,易通过功能化改变材料表面性质,不同的金属元素和配体种类,以及配位方式的多样化特性,极大地丰富固相萃取的固定相材料种类。尤其是在复杂基质样品预处理中,MOFs及其功能材料表现出强富集能力、强抗基质干扰能力、优异的选择性以及环境友好等优势。本文综述了近几年MOFs及其功能材料在食品和水样品中有害物质预处理方面的研究进展,并对这类材料应用在食品安全分析方面的发展进行了展望。
Food safety has received great attention due to its close connectivity with people's health and the harmonious development of national economy and society. Trace amount of toxic and harmful compounds in food and water are potentially harmful to human health. Excellent adsorbent and efficient extraction have received more and more attention in food safety detection. Metal-organic frameworks(MOFs) are an emerging class of porous functional materials with high porosity, large surface area, easy structural design, adjustable pore size, as well as acceptable chemical and thermal stability. In the past, the research on MOFs mainly focused on the structural design. Recently, more and more attention has been focused on applications of MOFs in food safety analysis. Meanwhile, their high porosity, tunable surface functionalities, various metal and ligands, as well as diverse coordination modes make MOFs promising as adsorption material for SPE. The merits of MOFs and their functional materials, in particular, are high enrichment, excellent matrix interference resistance, good selectivity, and environmentally-friendly development. Interesting research of MOFs and their functional materials in the pretreatment of food and water samples are summarized.
Food safety has received great attention due to its close connectivity with people's health and the harmonious development of national economy and society. Trace amount of toxic and harmful compounds in food and water are potentially harmful to human health. Excellent adsorbent and efficient extraction have received more and more attention in food safety detection. Metal-organic frameworks(MOFs) are an emerging class of porous functional materials with high porosity, large surface area, easy structural design, adjustable pore size, as well as acceptable chemical and thermal stability. In the past, the research on MOFs mainly focused on the structural design. Recently, more and more attention has been focused on applications of MOFs in food safety analysis. Meanwhile, their high porosity, tunable surface functionalities, various metal and ligands, as well as diverse coordination modes make MOFs promising as adsorption material for SPE. The merits of MOFs and their functional materials, in particular, are high enrichment, excellent matrix interference resistance, good selectivity, and environmentally-friendly development. Interesting research of MOFs and their functional materials in the pretreatment of food and water samples are summarized.
引文
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[72] Liu H L, Mu L, Chen X M, Wang J, Wang S, Sun B G. J. Agric. Food Chem., 2017, 65: 986.
[73] Liu X L, Wang C, Wu Q H, Wang Z. J. Sep. Sci., 2015, 38: 3928.
[74] Chang N, Gu Z Y, Yan XP. J. Am. Chem. Soc., 2010, 132:13645.
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