电催化氧化技术处理含盐有机废水研究进展
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摘要
介绍了电催化氧化技术在实际工业废水处理中的优势,对其反应原理进行了概述。总结了电催化氧化技术在石油、制药、造纸行业废水和含氨氮类有机废水处理中的研究进展,指出:电催化氧化技术未来的主要研究方向为研发新型电催化阳极材料;开发高效电解反应器;探索电催化氧化技术与其他处理工艺组合联用。
The advantages of electro-catalytic oxidation technology in actual industrial wastewater treatment are introduced and the reaction principle is outlined. The progresses in electro-catalytic oxidation technology for treatment of petroleum wastewater,pharmaceutical wastewater,papermaking wastewater and ammonia nitrogen wastewater are summarized. Furthermore,it is pointed out that the future research directions of electro-catalytic oxidation technology are as follows:developing new catalytic anode materials and ef?cient electrolytic reactor,and combining the electrocatalytic oxidation technology with other treatment processes.
The advantages of electro-catalytic oxidation technology in actual industrial wastewater treatment are introduced and the reaction principle is outlined. The progresses in electro-catalytic oxidation technology for treatment of petroleum wastewater,pharmaceutical wastewater,papermaking wastewater and ammonia nitrogen wastewater are summarized. Furthermore,it is pointed out that the future research directions of electro-catalytic oxidation technology are as follows:developing new catalytic anode materials and ef?cient electrolytic reactor,and combining the electrocatalytic oxidation technology with other treatment processes.
引文
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[27]DAGHRIR R,DROGUI P,TSHBANGU J.Efficient treatment of domestic wastewater by electrochemical oxidation process using bored doped diamond anode[J].Sep Purif Technol,2014,131:79-83.
[28]DONG H,SU H M,CHEN Z,et al.Fabrication of electrochemically reduced graphene oxide modified gas diffusion electrode for in-situ electrochemical advanced oxidation process under mild conditions[J].Electrochim Acta,2016,222:1501-1509.
[29]GARCíA-MORALES M A,ROA-MORALES G,BARRERA-DíAZ C,et al.Synergy of electrochemical oxidation using boron-doped diamond(BDD)electrodes and ozone(O3)in industrial wastewater treatment[J].Electrochem Commun,2013,27:34-37.
[2]周栋,俞彬,耿翠玉.O3-H2O2催化氧化技术深度处理石化含盐废水[J].化工环保,2018,38(2):202-206.
[3]NIDHEESH P V,ZHOU M H,OTURAN M A.An overview on the removal of synthetic dyes from water by electrochemical advanced oxidation processes[J].Chemosphere,2018,197:210-215.
[4]JING Y,CHAPLIN B P.A mechanistic study of the validity of using hydroxyl radical probes to characterize electrochemical advanced oxidation processes[J].Environ Sci Technol,2017,51(4):2355-2365.
[5]FANG C,MEGHARAJ M,NAIDU R.Electrochemical advanced oxidation processes(EAOP)to degrade per-and polyfluoroalkyl substances(PFASs)[J].J Adv Oxid Technol,2017,20(2):45-56.
[6]GARCIA-SEGURA S,OCON J D,CHONG M N.Electrochemical oxidation remediation of real wastewater effluents:a review[J].Process Saf Environ Prot,2018,113:48-67.
[7]YAVUZ Y,SAVA?KOPARAL A,??üTVERENüB.Treatment of petroleum refinery wastewater by electrochemical methods[J].Desalination,2010,258(1/3):201-205.
[8]阚连宝,丁思棋,宋亚瑞,等.电催化氧化法处理含油污水的实验研究[J].森林工程,2017,33(4):49-54.
[9]GARGOURI B,GARGOURI O D,GARGOURI B,et al.Application of electrochemical technology for removing petroleum hydrocarbons from produced water using lead dioxide and boron-doped diamond electrodes[J].Chemosphere,2014,117:309-315.
[10]DOMINGUEZ J R,GONZALEZ T,PALO P,et al.Electrochemical degradation of a real pharmaceutical effluent[J].Water Air Soil Pollut,2012,223(5):2685-2694.
[11]DA SILVA A J C,DOS SANTOS E V,DE OLIVEIRAMORAIS C C,et al.Electrochemical treatment of fresh,brine and saline produced water generated by petrochemical industry using Ti/IrO2-Ta2O5 and BDD in flow reactor[J].Chem Eng J,2013,233:47-55.
[12]夏伊静.高效金属掺杂PbO2电极的制备及用于降解典型制药废水的研究[D].杭州:浙江工业大学,2016.
[13]MOOK W T,CHAKRABARTI M H,AROUA M K,et al.Removal of total ammonia nitrogen(TAN),nitrate and total organic carbon(TOC)from aquaculture wastewater using electrochemical technology:a review[J].Desalination,2012,285(3):1-13.
[14]OUARDA Y,TIWARI B,AZA?S A,et al.Synthetic hospital wastewater treatment by coupling submerged membrane bioreactor and electrochemical advanced oxidation process:kinetic study and toxicity assessment[J].Chemosphere,2018,193:160-169.
[15]刘峻峰,黄琳琳,李姗姗,等.电催化氧化对制药废水二级出水的深度处理效能[J].环境工程学报,2016,10(11):6269-6274.
[16]LI X L,XU H,YAN W,et al.Electrocatalytic degradation of aniline by Ti/Sb-SnO2,Ti/Sb-SnO2/Pb3O4and Ti/Sb-SnO2/PbO2 anodes in different electrolytes[J].J Electroanal Chem,2016,775:43-51.
[17]徐丽丽,施汉昌,陈金銮.Ti/RuO2-TiO2-IrO2-SnO2电极电解氧化含氨氮废水[J].环境科学,2007,28(9):2009-2013.
[18]李锦景.复极性三维电极反应器预处理焦化废水的试验研究[D].合肥:安徽工业大学,2016.
[19]AOUDJ S,KHELIFA A,DROUICHE N,et al.Electrocoagulation process applied to wastewater containing dyes from textile industry[J].Chem Eng Process,2010,49(11):1176-1182.
[20]CHATZISYMEON E,XEKOUKOULOTAKIS N P,COZ A,et al.Electrochemical treatment of textile dyes and dyehouse effluents[J].J Hazard Mater,2006,137(2):998-1007.
[21]MALPASS G R,MIWA D W,MORTARI D A,et al.Decolorisation of real textile waste using electrochemical techniques:effect of the chloride concentration[J].Water Res,2007,41(13):2969-2977.
[22]杨蕴哲,杨卫身,杨凤林,等.电化学法处理高含盐活性艳蓝KN-R废水的研究[J].化工环保,2005,25(3):178-181.
[23]CHEN J M,XIA Y J,DAI Q Z.Electrochemical degradation of chloramphenicol with a novel Al doped PbO2 electrode:performance,kinetics and degradation mechanism[J].Electrochim Acta,2015,165:277-287.
[24]CHANWORRAWOOT K,HUNSOM M.Treatment of wastewater from pulp and paper mill industry by electrochemical methods in membrane reactor[J].JEnviron Manage,2012,113:399-406.
[25]EL-ASHTOUKHY E S Z,AMIN N K,ABDELWA-HAB O.Treatment of paper mill effluents in a batchstirred electrochemical tank reactor[J].Chem Eng J,2009,146(2):205-210.
[26]雷庆铎,刘依林,谷启源,等.电催化氧化预处理焦化废水的实验研究[J].工业水处理,2014,34(4):51-54.
[27]DAGHRIR R,DROGUI P,TSHBANGU J.Efficient treatment of domestic wastewater by electrochemical oxidation process using bored doped diamond anode[J].Sep Purif Technol,2014,131:79-83.
[28]DONG H,SU H M,CHEN Z,et al.Fabrication of electrochemically reduced graphene oxide modified gas diffusion electrode for in-situ electrochemical advanced oxidation process under mild conditions[J].Electrochim Acta,2016,222:1501-1509.
[29]GARCíA-MORALES M A,ROA-MORALES G,BARRERA-DíAZ C,et al.Synergy of electrochemical oxidation using boron-doped diamond(BDD)electrodes and ozone(O3)in industrial wastewater treatment[J].Electrochem Commun,2013,27:34-37.