Al-P系晶种合金的研究与应用
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摘要
对铝硅活塞合金用Al-P系列晶种合金的制备方法、组织特点、应用原理和细化作用等方面进行了系统介绍。在介绍铝硅活塞用Al-P晶种合金研究进展的同时,提出了面临的挑战和机遇,从而进一步推动该领域内晶种合金的发展。
This paper systematically introduces the fabrication methods, typical structures, applied principles and refining effects of Al-P series master alloys which have extensive applications in Al-Si piston alloys. Meanwhile, the confronted challenges and opportunities at current situations are put forward for driving the development of master alloys in this field.
This paper systematically introduces the fabrication methods, typical structures, applied principles and refining effects of Al-P series master alloys which have extensive applications in Al-Si piston alloys. Meanwhile, the confronted challenges and opportunities at current situations are put forward for driving the development of master alloys in this field.
引文
[1]李言祥.材料加工原理[M].北京:清华大学出版社,2005.LI Yan-xiang.Principle of Material Processing[M].Beijing:Tsinghua University Press,2005.
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[5]张蓉,黄太文,刘林.过共晶Al-Si合金熔体中初生硅生长特性[J].中国有色金属学报,2004,14(2):262-266.ZHANG Rong,HUANG Tai-wen,LIU Lin.Growth Characterization of Primary Si in Hypereutectic Al-Si alloy[J].Chinese Journal of Nonferrous Metals,2004,14(2):262-266.
[6]HERNáNDEZ F C Robles,SOKOLOWSKI J H.Comparison Among Chemical and Electromagnetic Stirring and Vibration Melt Treatments for Al-Si Hypereutectic Alloys[J].Journal of Alloys and Compounds,2006,426(1/2):205-212.
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[17]HO C R,CANTOR B.Heterogeneous Nucleation of Solidification of Si in Al-Si and Al-Si-P Alloys[J].Acta Metallurgica et Materialia,1995,43(8):3231-3246.
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[19]杨伏良,甘卫平,陈招科.高硅铝合金几种常见制备方法及其细化机理[J].材料导报,2005,19(5):42-45.YANG Fu-liang,GAN Wei-ping,CHEN Zhao-ke.Several Preparation Methods and Refinement Mechanism of High-Si Aluminium Alloys[J].Materials Review,2005,19(5):42-45.
[20]王泽华,毛协民,张金龙,等.Sr-PM复合变质过共晶铝硅合金[J].特种铸造及有色合金,2005,25(4):241-243.WANG Ze-hua,MAO Xie-min,ZHANG Jin-long,et al.Complex Modification of Hypereutectic Al-Si Alloy by Sr-PM[J].Special Casting&Nonferrous Alloys,2005,25(4):241-243.
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[22]武玉英,刘相法,刘相俊,等.低熔点Cu-P基中间合金及其变质效果[J].特种铸造及有色合金,2004(3):69-70.WU Yu-ying,LIU Xiang-fa,LIU Xiang-jun,et al.A Low Melting Point Cu-P Based Master Alloy and Its Modification Efficiency[J].Special Casting&Nonferrous Alloys,2004(3):69-70.
[23]WOLFGANG S.A New Method for the Refinement of Primary Si of Hypereutectic Al-Si Alloys in Direct Chill and Ingot Casting[J].Light Metals,1993:815-820.
[24]赵永治,高泽生.过共晶Al-Si合金连续铸造中初晶硅细化的新方法[J].轻合金加工技术,1995,23(10):5-8.ZHAO Yong-zhi,GAO Ze-sheng.A New Method for Refinement of Silicon in the Continuous Casting of Eutectic Al-Si Alloy[J].Light Alloy Fabrication Technology,1995,23(10):5-8.
[25]王德满,郑子樵,石春生,等.熔铸法生产的磷变质剂对过共晶铝-硅合金组织和性能的影响[J].轻合金加工技术,1995,23(9):9-12.WANG De-man,ZHENG Zi-qiao,SHI Chun-sheng,et al.The Influence of Phosphorus Metamorphic Agent on the Microstructure and Properties of Eutectic Al-Si Alloy[J].Light Alloy Fabrication Technology,1995,23(9):9-12.
[26]王德满,赵海英,孙兆霞,等.一种新型过共晶Al-Si合金变质剂[J].轻金属,1997(7):50-53.WANG De-man,ZHAO Hai-ying,SUN Zhao-xia,et al.A New Modifier for Hypereutectic Al-Si Alloy[J].Light Metals,1997(7):50-53.
[27]KYFFIN W J,RAINFORTH W M,JONES H.The Formation of Aluminum Phosphide in Aluminum Melt Treated with an Al-Fe-P Inoculant Addition[J].Zeitschrift für Metallkunde,2001,92(4):396-398.
[28]KYFFIN W J,RAINFORTH W M,JONES H.Effect of Phosphorus Additions on the Spacing between Primary Silicon Particles in a Bridgman Solidified Hypereutectic Al-Si Alloy[J].Journal of Materials Science,2001,36(11):2667-2672.
[29]刘相法,齐广慧,韩延峰,等.Al-P中间合金变质剂在Al-Si活塞合金中的应用[J].内燃机配件,2001(6):14-17.LIU Xiang-fa,QI Guang-hui,HAN Yan-feng,et al.Application of Al-P Master Alloy in Al-Si Piston Alloy[J].Internal Combustion Engine Parts,2001(6):14-17.
[30]QIN J Y,ZUO Min,GU T,et al.The Featured Local Structural Units in Liquid Al80Si15P5 Alloy and Their Relationship with Si Modification[J].Journal of Alloys and Compounds,2010,492(1/2):525-528.
[31]朱向镇.Al-Si-X-P熔体中Al-P团簇演变行为与化学稳定性的研究[D].济南:山东大学,2016.ZHU Xiang-zhen.Study of Evolution and Chemistry Stability of Al-P Clusters in Al-Si-X-P melt[D].Jinan:Doctoral Dissertation of Shandong University,2009.
[32]ZHU X,JIANG W,LI M,et al.The Effect of Mg Adding Order on the Liquid Structure and Solidified Microstructure of the Al-Si-Mg-P Alloy:An Experiment and ab Initio Study[J].Metals,2015,5(1):40-51.
[33]乔进国.Al-P-Si中间合金及其变质处理技术的研究[D].济南:山东大学,2005.QIAO Jin-guo.Study of Al-P-Si Master Alloy and Its Modification Treatment[D].Jinan:Master's Dissertation of Shandong University,2005.
[34]ZUO Min,LIU Xiang-fa.Twin Growth Mechanism of Al P Hexagonal Platelets in an Al-Si Melt[J].Crystal Growth&Design,2010,10:2443-2446.
[35]刘相法,侯静,李冲,等.一种铝-镁-磷中间合金及其制备方法:中国,ZL201110264218.4[P].LIU Xiang-fa,HOU Jing,LI Chong,et al.An Al-Mg-PIntermediate Alloy and Its Preparation Method:China,ZL201110264218.4[P].
[36]侯静.Al-P中间合金对含Si镁合金细化与变质行为的研究[D].济南:山东大学,2012.HOU Jing.Study of Refinement and Modification Effect of Al-P Master Alloy on Magnesium Alloy with Si Containing[D].Jinan:Master's Dissertation of Shandong University,2012.
[37]刘相法,左敏,姜琨,等.一种铝-锆-磷中间合金及其制备方法:中国,ZL200910016834.0[P].LIU Xiang-fa,ZUO Min,JIANG Kun,et al.An Al-Zr-PIntermediate Alloy and Its Preparation Method:China,ZL200910016834.0[P].
[38]ZUO Min,JIANG Kun,LIU Xiang-fa.Refinement of Hypereutectic Al-Si Alloy by a New Al-Zr-P Master Alloy[J].Journal of Alloys and Compounds,2010,503(2):26-30.
[39]包国菊.Zr(RE)P在铝熔体中的反应合成与演变机制[D].济南:山东大学,2013.BAO Guo-ju.Reaction Synthesis and Evolution Mechanism of Zr(RE)P in Aluminum Melt[D].Jinan:Master's Dissertation of Shandong University,2013.
[40]ZHOU X L,WU Y Y,LI Y F,et al.Absorbing Formation Mechanism of Al P on Ti B2 Substrate and Their Application as High-efficiency Nucleating Agent in Al-45Si alloy[J].Journal of Alloys and Compounds,2017,693:853-858.
[41]XU C L,YANG Y F.Effect of Al-P-Ti-Ti C-Nd2O3Modifier on the Microstructure and Mechanical Properties of Hypereutectic Al-20 wt.%Si Alloy[J].Materials Science&Engineering A,2007,452/453(24):341-346.
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[47]卢绍龙,马幼平.过共晶Al-Si合金变质处理研究进展[J].轻合金加工技术,2009,37(8):5-8.LU Shao-long,MA You-ping.Research Progress of Modification of Hypereutectic Al-Si Alloy[J].Light Alloy Fabrication Technology,2009,37(8):5-8.
[2]《铸造有色金属及其熔炼》联合编写组.铸造有色合金及其熔炼[M].北京:国防工业出版社,1980.“Casting Nonferrous Metals and their Smelting”Joint Compiling Group.Casting Nonferrous Metals and Their Smelting[M].Beijing:National Defence Industry Press,1980.
[3]张俊红,任智森,赵群,等.变质工艺影响过共晶Al-Si合金初晶硅细化的研究[J].轻合金,2006(10):62-65.ZHANG Jun-hong,REN Zhi-sen,ZHAO Qun,et al.Effect of Modification Process on the Refinement of Primary Si in Hypereutectic Al-Si Alloy[J].Light Metals,2006(10):62-65.
[4]赵爱民,毛卫民,甄子胜,等.冷却速度对过共晶铝硅合金凝固组织和耐磨性能的影响[J].中国有色金属学报,2001,11(5):827-832.ZHAO Ai-min,MAO Wei-min,ZHEN Zi-sheng,et al.Effect of Cooling Rate on the Solidification Structure and Wear Resistance of Hypereutectic Al-Si Alloy[J].Chinese Journal of Nonferrous Metals,2001,11(5):827-832.
[5]张蓉,黄太文,刘林.过共晶Al-Si合金熔体中初生硅生长特性[J].中国有色金属学报,2004,14(2):262-266.ZHANG Rong,HUANG Tai-wen,LIU Lin.Growth Characterization of Primary Si in Hypereutectic Al-Si alloy[J].Chinese Journal of Nonferrous Metals,2004,14(2):262-266.
[6]HERNáNDEZ F C Robles,SOKOLOWSKI J H.Comparison Among Chemical and Electromagnetic Stirring and Vibration Melt Treatments for Al-Si Hypereutectic Alloys[J].Journal of Alloys and Compounds,2006,426(1/2):205-212.
[7]JIANG Q C,XU C L,LU M,et al.Effect of New Al-P-Ti-Ti C-Y Modifier on Primary Silicon in Hypereutectic Al-Si Alloys[J].Materials Letters,2005,59(6):624-628.
[8]MAENG D Y,LEE J H,WON C W,et al.The Effects of Processing Parameters on the Microstructure and Mechanical Properties of Modified B390 Alloy in Direct Squeeze Casting[J].Journal of Materials Processing Technology,2000,105(1/2):196-203.
[9]YOON S C,HONG S J,HONG S I,et al.Mechanical Properties of Equal Channel Angular Pressed Powder Extrudates of a Rapidly Solidified Hypereutectic Al-20 wt%Si Alloy[J].Materials Science and Engineering A,2007,449/450/451:966-970.
[10]APAYDIN N,SMITH R W.Microstructural Characterization of Rapid Solidified Al-Si Alloys[J].Materials Science and Engineering,1988,98:149-152.
[11]UZUN O,KARAASLAN T,GOGEBAKAN M,et al.Handness and Microstructural Characteristics of Rapidly Solidified Al-8-16wt.%Si Alloys[J].Journal of Alloys and Compounds,2004,376(1/2):149-157.
[12]MATSUURA K,KUDOH M,KINOSHITA H,et al.Precipitation of Si Particles in a Super-rapidly Solidified Al-Si Hypereutectic Alloy[J].Materials Chemistry and Physics,2003,81(2/3):393-395.
[13]FENG H K,YU S R,LI Y L,et al.Effect of Ultrasonic Treatment on Microstructures of Hypereutectic Al-Si Alloy.Journal of Materials Processing Technology,2008,208(1/2/3):330-335.
[14]LU D H,JIANG Y H,GUAN G S,et al.Refinement of Primary Si in Hypereutectic Al-Si alloy by Electromagnetic Stirring[J].Journal of Materials Processing Technology,2007,189(1/2/3):13-18.
[15]ABU-DHEIR N,KHRAISHEH M,SAITO K,et al.Silicon Morphology Modification in the Eutectic Al-Si Alloy Using Mechanical Mold Vibration[J].Materials Science and Engineering A,2005,393(1/2):109-117.
[16]ADDAMIANO A.On the Preparation of the Phosphides of Aluminum,Gallium and Indium[J].Journal of the American Chemical Society,1960,82(7):1537-1540.
[17]HO C R,CANTOR B.Heterogeneous Nucleation of Solidification of Si in Al-Si and Al-Si-P Alloys[J].Acta Metallurgica et Materialia,1995,43(8):3231-3246.
[18]CANTOR B.Impurity Effects on Heterogeneous Nucleation[J].Materials Science and Engineering A,1997,226/227/228:151-156.
[19]杨伏良,甘卫平,陈招科.高硅铝合金几种常见制备方法及其细化机理[J].材料导报,2005,19(5):42-45.YANG Fu-liang,GAN Wei-ping,CHEN Zhao-ke.Several Preparation Methods and Refinement Mechanism of High-Si Aluminium Alloys[J].Materials Review,2005,19(5):42-45.
[20]王泽华,毛协民,张金龙,等.Sr-PM复合变质过共晶铝硅合金[J].特种铸造及有色合金,2005,25(4):241-243.WANG Ze-hua,MAO Xie-min,ZHANG Jin-long,et al.Complex Modification of Hypereutectic Al-Si Alloy by Sr-PM[J].Special Casting&Nonferrous Alloys,2005,25(4):241-243.
[21]ZHANG H H,DUAN H L,SHAO G J,et al.Microstructure and Mechanical Properties of Hypereutectic Al-Si Alloy Modified with Cu-P[J].Rare Metals,2008,27(1):59-63.
[22]武玉英,刘相法,刘相俊,等.低熔点Cu-P基中间合金及其变质效果[J].特种铸造及有色合金,2004(3):69-70.WU Yu-ying,LIU Xiang-fa,LIU Xiang-jun,et al.A Low Melting Point Cu-P Based Master Alloy and Its Modification Efficiency[J].Special Casting&Nonferrous Alloys,2004(3):69-70.
[23]WOLFGANG S.A New Method for the Refinement of Primary Si of Hypereutectic Al-Si Alloys in Direct Chill and Ingot Casting[J].Light Metals,1993:815-820.
[24]赵永治,高泽生.过共晶Al-Si合金连续铸造中初晶硅细化的新方法[J].轻合金加工技术,1995,23(10):5-8.ZHAO Yong-zhi,GAO Ze-sheng.A New Method for Refinement of Silicon in the Continuous Casting of Eutectic Al-Si Alloy[J].Light Alloy Fabrication Technology,1995,23(10):5-8.
[25]王德满,郑子樵,石春生,等.熔铸法生产的磷变质剂对过共晶铝-硅合金组织和性能的影响[J].轻合金加工技术,1995,23(9):9-12.WANG De-man,ZHENG Zi-qiao,SHI Chun-sheng,et al.The Influence of Phosphorus Metamorphic Agent on the Microstructure and Properties of Eutectic Al-Si Alloy[J].Light Alloy Fabrication Technology,1995,23(9):9-12.
[26]王德满,赵海英,孙兆霞,等.一种新型过共晶Al-Si合金变质剂[J].轻金属,1997(7):50-53.WANG De-man,ZHAO Hai-ying,SUN Zhao-xia,et al.A New Modifier for Hypereutectic Al-Si Alloy[J].Light Metals,1997(7):50-53.
[27]KYFFIN W J,RAINFORTH W M,JONES H.The Formation of Aluminum Phosphide in Aluminum Melt Treated with an Al-Fe-P Inoculant Addition[J].Zeitschrift für Metallkunde,2001,92(4):396-398.
[28]KYFFIN W J,RAINFORTH W M,JONES H.Effect of Phosphorus Additions on the Spacing between Primary Silicon Particles in a Bridgman Solidified Hypereutectic Al-Si Alloy[J].Journal of Materials Science,2001,36(11):2667-2672.
[29]刘相法,齐广慧,韩延峰,等.Al-P中间合金变质剂在Al-Si活塞合金中的应用[J].内燃机配件,2001(6):14-17.LIU Xiang-fa,QI Guang-hui,HAN Yan-feng,et al.Application of Al-P Master Alloy in Al-Si Piston Alloy[J].Internal Combustion Engine Parts,2001(6):14-17.
[30]QIN J Y,ZUO Min,GU T,et al.The Featured Local Structural Units in Liquid Al80Si15P5 Alloy and Their Relationship with Si Modification[J].Journal of Alloys and Compounds,2010,492(1/2):525-528.
[31]朱向镇.Al-Si-X-P熔体中Al-P团簇演变行为与化学稳定性的研究[D].济南:山东大学,2016.ZHU Xiang-zhen.Study of Evolution and Chemistry Stability of Al-P Clusters in Al-Si-X-P melt[D].Jinan:Doctoral Dissertation of Shandong University,2009.
[32]ZHU X,JIANG W,LI M,et al.The Effect of Mg Adding Order on the Liquid Structure and Solidified Microstructure of the Al-Si-Mg-P Alloy:An Experiment and ab Initio Study[J].Metals,2015,5(1):40-51.
[33]乔进国.Al-P-Si中间合金及其变质处理技术的研究[D].济南:山东大学,2005.QIAO Jin-guo.Study of Al-P-Si Master Alloy and Its Modification Treatment[D].Jinan:Master's Dissertation of Shandong University,2005.
[34]ZUO Min,LIU Xiang-fa.Twin Growth Mechanism of Al P Hexagonal Platelets in an Al-Si Melt[J].Crystal Growth&Design,2010,10:2443-2446.
[35]刘相法,侯静,李冲,等.一种铝-镁-磷中间合金及其制备方法:中国,ZL201110264218.4[P].LIU Xiang-fa,HOU Jing,LI Chong,et al.An Al-Mg-PIntermediate Alloy and Its Preparation Method:China,ZL201110264218.4[P].
[36]侯静.Al-P中间合金对含Si镁合金细化与变质行为的研究[D].济南:山东大学,2012.HOU Jing.Study of Refinement and Modification Effect of Al-P Master Alloy on Magnesium Alloy with Si Containing[D].Jinan:Master's Dissertation of Shandong University,2012.
[37]刘相法,左敏,姜琨,等.一种铝-锆-磷中间合金及其制备方法:中国,ZL200910016834.0[P].LIU Xiang-fa,ZUO Min,JIANG Kun,et al.An Al-Zr-PIntermediate Alloy and Its Preparation Method:China,ZL200910016834.0[P].
[38]ZUO Min,JIANG Kun,LIU Xiang-fa.Refinement of Hypereutectic Al-Si Alloy by a New Al-Zr-P Master Alloy[J].Journal of Alloys and Compounds,2010,503(2):26-30.
[39]包国菊.Zr(RE)P在铝熔体中的反应合成与演变机制[D].济南:山东大学,2013.BAO Guo-ju.Reaction Synthesis and Evolution Mechanism of Zr(RE)P in Aluminum Melt[D].Jinan:Master's Dissertation of Shandong University,2013.
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