Enhancement of oxygen evolution reaction activity and durability of Ba_(0.5)Sr_(0.5)Co_(0.8)Fe_(0.2)O_(3-δ) by CO_2 thermal treatment
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摘要
This work demonstrates that in situ formation of carbonate layer on the surface of Ba_(0.5)Sr_(0.5)Co_(0.8)Fe_(0.2)O_(3-δ)(BSCF)obtained by exposure to CO_2 during heating between 500℃ and 700℃ can provide enhanced oxygen evolution reaction(OER)performance and durability in an alkaline solution relative to the original BSCF.Three temperatures,i.e., 500℃,600℃,and 700℃ were chosen to perform the CO_2 thermal treatment,resulting into BSCF-500,BSCF-600,and BSCF-700 samples.The OER was enhanced in the order of BSCF-500 This work demonstrates that in situ formation of carbonate layer on the surface of Ba_(0.5)Sr_(0.5)Co_(0.8)Fe_(0.2)O_(3-δ)(BSCF)obtained by exposure to CO_2 during heating between 500℃ and 700℃ can provide enhanced oxygen evolution reaction(OER)performance and durability in an alkaline solution relative to the original BSCF.Three temperatures,i.e., 500℃,600℃,and 700℃ were chosen to perform the CO_2 thermal treatment,resulting into BSCF-500,BSCF-600,and BSCF-700 samples.The OER was enhanced in the order of BSCF-500
引文
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[18] J.I. Jung, S. Park, M.G. Kim, J. Cho,Adv. Energy Mater. 5(2016), 1501560.
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[20] E. Fabbri, M. Nachtegaal, T. Binninger, X. Cheng, B.J. Kim, J. Durst, F. Bozza, T.Graule, R. Sch?ublin, L. Wiles, M. Pertoso, N. Danilovic, K.E. Ayers, T.J. Schmidt,Nat. Mater. 16(2017)925–931.
[21] C.C. McCrory, S. Jung, J.C. Peters, T.F. Jaramillo, J. Am. Chem. Soc. 135(2013)16977–16987.
[22] T.Y. Ma, S. Dai, M. Jaroniec, S.Z. Qiao, J. Am. Chem. Soc. 136(2014)13925–13931.
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