Covalent organic frameworks derived hollow structured N-doped noble carbon for asymmetric-electrolyte Zn-air battery
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摘要
We report a relatively low-temperature molten salt strategy to prepare hollow structured N-doped noble carbon(h-NNC) with highly desirable features of ultra-large surface area(1957 m~2 g~(-1)) and high graphitization, endowing the h-NNC with high activity toward catalysis of oxygen reduction reaction in acidic medium. The h-NNC is applied as cathode catalyst of an asymmetrical-electrolyte Zn-air battery, which exhibits an open circuit voltage of 2.11 V, a power density up to 270 mW cm~(-2),and an energy density of 1279 W h kg~(-1), behaving advantages over the conventional Zn-air batteries.
We report a relatively low-temperature molten salt strategy to prepare hollow structured N-doped noble carbon(h-NNC) with highly desirable features of ultra-large surface area(1957 m~2 g~(-1)) and high graphitization, endowing the h-NNC with high activity toward catalysis of oxygen reduction reaction in acidic medium. The h-NNC is applied as cathode catalyst of an asymmetrical-electrolyte Zn-air battery, which exhibits an open circuit voltage of 2.11 V, a power density up to 270 mW cm~(-2),and an energy density of 1279 W h kg~(-1), behaving advantages over the conventional Zn-air batteries.
We report a relatively low-temperature molten salt strategy to prepare hollow structured N-doped noble carbon(h-NNC) with highly desirable features of ultra-large surface area(1957 m~2 g~(-1)) and high graphitization, endowing the h-NNC with high activity toward catalysis of oxygen reduction reaction in acidic medium. The h-NNC is applied as cathode catalyst of an asymmetrical-electrolyte Zn-air battery, which exhibits an open circuit voltage of 2.11 V, a power density up to 270 mW cm~(-2),and an energy density of 1279 W h kg~(-1), behaving advantages over the conventional Zn-air batteries.
引文
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22 Zhang G,Jin X,Li H,Wang L,Hu C,Sun X.Sci China Mater,2016,59:337-347
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24 Miura A,Rosero-Navarro C,Masubuchi Y,Higuchi M,Kikkawa S,Tadanaga K.Angew Chem Int Ed,2016,55:7963-7967
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26 Wu G,More KL,Johnston CM,Zelenay P.Science,2011,332:443-447
27 Gong K,Du F,Xia Z,Durstock M,Dai L.Science,2009,323:760-764
28 Wei W,Liang H,Parvez K,Zhuang X,Feng X,Müllen K.Angew Chem Int Ed,2014,53:1570-1574
29 Elumeeva K,Fechler N,Fellinger TP,Antonietti M.Mater Horiz,2014,1:588-594
30 Liang HW,Zhuang X,Brüller S,Feng X,Müllen K.Nat Commun,2014,5:4973
31 Wu G,Zelenay P.Acc Chem Res,2013,46:1878-1889
32 Malko D,Kucernak A,Lopes T.J Am Chem Soc,2016,138:16056-16068
33 Ryoo R,Joo SH,Kruk M,Jaroniec M.Adv Mater,2001,13:677-681
34 Liang C,Li Z,Dai S.Angew Chem Int Ed,2008,47:3696-3717
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36 Lv R,Cui T,Jun MS,Zhang Q,Cao A,Su DS,Zhang Z,Yoon SH,Miyawaki J,Mochida I,Kang F.Adv Funct Mater,2011,21:999-1006
37 Huang W,Wang Y,Luo G,Wei F.Carbon,2003,41:2585-2590
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39 Antonietti M,Oschatz M.Adv Mater,2018,30:1706836
40 Men Y,Siebenbürger M,Qiu X,Antonietti M,Yuan J.J Mater Chem A,2013,1:11887-11893
41 Kuhn P,Thomas A,Antonietti M.Macromolecules,2008,42:319-326
42 Kuhn P,Forget A,Su D,Thomas A,Antonietti M.J Am Chem Soc,2008,130:13333-13337
43 Liu X,Fechler N,Antonietti M.Chem Soc Rev,2013,42:8237-8265
44 Lin L,Ou H,Zhang Y,Wang X.ACS Catal,2016,6:3921-3931
45 Ding Y,Tang Y,Yang L,Zeng Y,Yuan J,Liu T,Zhang S,Liu C,Luo S.J Mater Chem A,2016,4:14307-14315
46 Ahn SH,Yu X,Manthiram A.Adv Mater,2017,29:1606534
47 Zhang J,Qu L,Shi G,Liu J,Chen J,Dai L.Angew Chem Int Ed,2015,55:2230-2234
48 Yang W,Liu X,Yue X,Jia J,Guo S.J Am Chem Soc,2015,137:1436-1439
49 Song H,Yang L,Tang Y,Yan D,Liu C,Luo S.Chem Eur J,2015,21:16631-16638
50 Liu Q,Wang Y,Dai L,Yao J.Adv Mater,2016,28:3000-3006
51 Zhang J,Zhou H,Zhu J,Hu P,Hang C,Yang J,Peng T,Mu S,Huang Y.ACS Appl Mater Interfaces,2017,9:24545-24554
52 Park J,Park M,Nam G,Lee J,Cho J.Adv Mater,2015,27:1396-1401
53 Cai P,Ci S,Zhang E,Shao P,Cao C,Wen Z.Electrochim Acta,2016,220:354-362
54 Wu X,Han X,Ma X,Zhang W,Deng Y,Zhong C,Hu W.ACS Appl Mater Interfaces,2017,9:12574-12583
2 Lee JS,Tai Kim S,Cao R,Choi NS,Liu M,Lee KT,Cho J.Adv Energy Mater,2011,1:34-50
3 Zhang J,Zhao Z,Xia Z,Dai L.Nat Nanotech,2015,10:444-452
4 Lee DU,Choi JY,Feng K,Park HW,Chen Z.Adv Energy Mater,2014,4:1301389
5 Cao R,Lee JS,Liu M,Cho J.Adv Energy Mater,2012,2:816-829
6 Cheng F,Chen J.Chem Soc Rev,2012,41:2172-2192
7 Wang ZL,Xu D,Xu JJ,Zhang XB.Chem Soc Rev,2014,43:7746-7786
8 Li L,Liu C,He G,Fan D,Manthiram A.Energy Environ Sci,2015,8:3274-3282
9 Cai P,Li Y,Chen J,Jia J,Wang G,Wen Z.ChemElectroChem,2018,5:589-592
10 Lukowski MA,Daniel AS,Meng F,Forticaux A,Li L,Jin S.J Am Chem Soc,2013,135:10274-10277
11 Yin Y,Han J,Zhang Y,Zhang X,Xu P,Yuan Q,Samad L,Wang X,Wang Y,Zhang Z,Zhang P,Cao X,Song B,Jin S.J Am Chem Soc,2016,138:7965-7972
12 Wang YJ,Zhao N,Fang B,Li H,Bi XT,Wang H.Chem Rev,2015,115:3433-3467
13 Zhang H,Hwang S,Wang M,Feng Z,Karakalos S,Luo L,Qiao Z,Xie X,Wang C,Su D,Shao Y,Wu G.J Am Chem Soc,2017,139:14143-14149
14 Ma J,Xiang Z,Zhang J.Sci China Chem,2018,61:592-597
15 Liu X,Park M,Kim MG,Gupta S,Wang X,Wu G,Cho J.Nano Energy,2016,20:315-325
16 Sun M,Zhang G,Liu H,Liu Y,Li J.Sci China Mater,2015,58:683-692
17 Cai P,Hong Y,Ci S,Wen Z.Nanoscale,2016,8:20048-20055
18 Yan D,Guo L,Xie C,Wang Y,Li Y,Li H,Wang S.Sci China Mater,2018,61:679-685
19 Cheng F,Zhang T,Zhang Y,Du J,Han X,Chen J.Angew Chem Int Ed,2013,52:2474-2477
20 Yi QF,Zhang YH,Liu XP,Yang YH.Sci China Chem,2014,57:739-747
21 Wen Z,Ci S,Zhang F,Feng X,Cui S,Mao S,Luo S,He Z,Chen J.Adv Mater,2012,24:1399-1404
22 Zhang G,Jin X,Li H,Wang L,Hu C,Sun X.Sci China Mater,2016,59:337-347
23 Zhou YX,Yao HB,Wang Y,Liu HL,Gao MR,Shen PK,Yu SH.Chem Eur J,2010,16:12000-12007
24 Miura A,Rosero-Navarro C,Masubuchi Y,Higuchi M,Kikkawa S,Tadanaga K.Angew Chem Int Ed,2016,55:7963-7967
25 Liang HW,Wei W,Wu ZS,Feng X,Müllen K.J Am Chem Soc,2013,135:16002-16005
26 Wu G,More KL,Johnston CM,Zelenay P.Science,2011,332:443-447
27 Gong K,Du F,Xia Z,Durstock M,Dai L.Science,2009,323:760-764
28 Wei W,Liang H,Parvez K,Zhuang X,Feng X,Müllen K.Angew Chem Int Ed,2014,53:1570-1574
29 Elumeeva K,Fechler N,Fellinger TP,Antonietti M.Mater Horiz,2014,1:588-594
30 Liang HW,Zhuang X,Brüller S,Feng X,Müllen K.Nat Commun,2014,5:4973
31 Wu G,Zelenay P.Acc Chem Res,2013,46:1878-1889
32 Malko D,Kucernak A,Lopes T.J Am Chem Soc,2016,138:16056-16068
33 Ryoo R,Joo SH,Kruk M,Jaroniec M.Adv Mater,2001,13:677-681
34 Liang C,Li Z,Dai S.Angew Chem Int Ed,2008,47:3696-3717
35 Zhu Y,Li L,Zhang C,Casillas G,Sun Z,Yan Z,Ruan G,Peng Z,Raji ARO,Kittrell C,Hauge RH,Tour JM.Nat Commun,2012,3:1225
36 Lv R,Cui T,Jun MS,Zhang Q,Cao A,Su DS,Zhang Z,Yoon SH,Miyawaki J,Mochida I,Kang F.Adv Funct Mater,2011,21:999-1006
37 Huang W,Wang Y,Luo G,Wei F.Carbon,2003,41:2585-2590
38 Wen Z,Ci S,Hou Y,Chen J.Angew Chem Int Ed,2014,53:6496-6500
39 Antonietti M,Oschatz M.Adv Mater,2018,30:1706836
40 Men Y,Siebenbürger M,Qiu X,Antonietti M,Yuan J.J Mater Chem A,2013,1:11887-11893
41 Kuhn P,Thomas A,Antonietti M.Macromolecules,2008,42:319-326
42 Kuhn P,Forget A,Su D,Thomas A,Antonietti M.J Am Chem Soc,2008,130:13333-13337
43 Liu X,Fechler N,Antonietti M.Chem Soc Rev,2013,42:8237-8265
44 Lin L,Ou H,Zhang Y,Wang X.ACS Catal,2016,6:3921-3931
45 Ding Y,Tang Y,Yang L,Zeng Y,Yuan J,Liu T,Zhang S,Liu C,Luo S.J Mater Chem A,2016,4:14307-14315
46 Ahn SH,Yu X,Manthiram A.Adv Mater,2017,29:1606534
47 Zhang J,Qu L,Shi G,Liu J,Chen J,Dai L.Angew Chem Int Ed,2015,55:2230-2234
48 Yang W,Liu X,Yue X,Jia J,Guo S.J Am Chem Soc,2015,137:1436-1439
49 Song H,Yang L,Tang Y,Yan D,Liu C,Luo S.Chem Eur J,2015,21:16631-16638
50 Liu Q,Wang Y,Dai L,Yao J.Adv Mater,2016,28:3000-3006
51 Zhang J,Zhou H,Zhu J,Hu P,Hang C,Yang J,Peng T,Mu S,Huang Y.ACS Appl Mater Interfaces,2017,9:24545-24554
52 Park J,Park M,Nam G,Lee J,Cho J.Adv Mater,2015,27:1396-1401
53 Cai P,Ci S,Zhang E,Shao P,Cao C,Wen Z.Electrochim Acta,2016,220:354-362
54 Wu X,Han X,Ma X,Zhang W,Deng Y,Zhong C,Hu W.ACS Appl Mater Interfaces,2017,9:12574-12583