铅同位素示踪技术在水环境中的应用研究综述
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- 英文论文题名：Review of the Lead Isotopic Application in Tracing Metal Pollution sources in Water Environment
- 论文作者：郝红 ; 高博 ; 陆瑾 ; 黄勇 ; 周怀东 ; 殷淑华 ; 郭太君
- 英文论文作者：Hao Hong ; Gao Bo ; Lu Jin ; Huang Yong ; Zhou Huaidong ; Yin Shuhua ; Guo Taijun ; Department of Water Environment ; China Institute of Water Resources and Hydropower Research ; Jilin Agricultural University College of Horticulture
- 年：2013
- 作者机构：中国水利水电科学研究院水环境研究所;吉林农业大学园艺学院;
- 论文关键词：水环境 ; 重金属污染 ; 铅同位素 ; 示踪技术
- 英文论文关键词：water environment ; heavy metals ; lead isotopes ; source tracing
- 会议召开时间：2013-12-26
- 会议录名称：2013年水资源生态保护与水污染控制研讨会论文集
- 语种：中文
- 分类号：X52;X143
- 学会代码：HJKP
- 会议名称：2013年水资源生态保护与水污染控制研讨会
- 会议地点：中国黑龙江哈尔滨
- 主办单位：中国环境科学学会、环境保护部环境规划院、哈尔滨工业大学、哈尔滨师范大学、中国科学院南京地理与湖泊研究所
- 学会名称：中国环境科学学会
- 页数：7
- 文件大小：966k
- 原文格式：D
- 会议级别：全国
摘要
水是自然界最重要组成之一,随着近代工业的快速发展,大量重金属元素被释放到水环境中,严重影响到水体中重金属的平衡,导致水环境中的表层沉积物、水、水生生物等出现重金属污染。近年来,铅同位素示踪技术被国内外专家及学者广泛认同,并利用这种技术对水环境中重金属染污源进行示踪研究。本文通过查阅近年来国内外有关铅同位素示踪技术的应用,阐述了铅同位素示踪技术的原理及方法,概述了铅同位素示踪技术在水环境中的研究进展。根据以往研究的存在的问题,对同位素示踪技术的发展趋势提出了建议和展望,为我国在水环境中重金属溯源研究中提供理论依据。
Water is one of the most important components in nature. With the rapid development of modern industry, a large number of heavy metals were released into the water environment. It is seriously affecting the water balance of the heavy metals and resulting into heavy metal pollution was occurred in surface sediments,water and aquatic organisms in water environment. In recent years, the lead isotopic tracer technique has been widely accepted by the researches and scholars in the world, and this technique was widely used in source identification of heavy metal pollution in water environment. The applications for the lead isotope tracer technique in recent years were reviewed and the theory and method of the technique was also introduced.Moreover, the research progress of the technique in water environment is summarized in this paper. According to the shortages and the existing problems of previous studies, we gave some suggestions of heavy pollution in water environment and discussed the development future of the stable isotopic technique. Finally, our suggestion is expected to be beneficial to provide theoretical evidences for the source identification study of heavy metal pollution in water environment in China.
Water is one of the most important components in nature. With the rapid development of modern industry, a large number of heavy metals were released into the water environment. It is seriously affecting the water balance of the heavy metals and resulting into heavy metal pollution was occurred in surface sediments,water and aquatic organisms in water environment. In recent years, the lead isotopic tracer technique has been widely accepted by the researches and scholars in the world, and this technique was widely used in source identification of heavy metal pollution in water environment. The applications for the lead isotope tracer technique in recent years were reviewed and the theory and method of the technique was also introduced.Moreover, the research progress of the technique in water environment is summarized in this paper. According to the shortages and the existing problems of previous studies, we gave some suggestions of heavy pollution in water environment and discussed the development future of the stable isotopic technique. Finally, our suggestion is expected to be beneficial to provide theoretical evidences for the source identification study of heavy metal pollution in water environment in China.
引文
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[3]吴龙华,张长波,章海波,等.铅稳定同位素在土壤污染物来源识别中的应用[J].环境科学,2009,30(1):227-230.
[4]黄勇,高博,王健康,等.新疆石河子城区道路尘土的铅污染和铅同位素示踪研究[J].岩矿测试,2013,32(4):632-637.
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[12]Cheng H F,Hu Y A.Lead(Pb)isotopic fingerprinting and its applications in lead pollution studies in China:A review[J].Environmental Pollution,2010,158:1-13.
[13]伊慧,伊观.铅稳定同位素在环境污染示踪中的应用和进展[J].广东微量元素科学,2007,14(5):1-5.
[14]余伟河,于瑞莲,胡恭任.铅锌镉同位素在土壤和沉积物重金属污染溯源研究中的应用进展[J].有色金属工程,2012,4:57-62.
[15]Eades L J,Farmer J G,Mackenzie A B,et al.Stable lead isotopic characterization of the historical record of environmental lead contamination in dated freshwater lake sediment cores from Northern and Central Scotland[J].The Science of the Total Environment,2002,292:55-67.
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[22]彭渤,唐晓燕,等.湘江入湖河段沉积物重金属污染及其Pb同位素地球化学示踪[J].地质学报,2011,85(2):282-299.
[23]Choi M S,Yi H I,Yang S Y,Lee C B,Cha H J.Identification of Pb sources in Yellow Sea sediments using stable Pb isotope ratios[J].Marine Chemistry,2007,107:255–274.
[24]Hao Y,Guo Z,Yang Z,Fan D,Fang M,Li X.Tracking historical lead pollution in the coastal area adjacent to the Yangtze River Estuary using lead isotopic compositions[J].Environmental Pollution,2008,156,1325–1331.
[25]Hu X,Wang C,Zou L M.Characteristics of heavy metals and Pb isotopic signatures in sediment cores collected from typical urban shallow lakes in Nanjing,China[J].Journal of Environmental Management,2010,10:1-7.
[26]Zhu L M,Guo L D,Gao Z Y,et al.Source and distribution of lead in the surface sediments from the South China Sea as derived from Pb isotopes[J].Marine Pollution Bulletin,2010,60:2144-2153.
[27]徐林波,高勤峰,董双林,等.靖海湾重金属污染及铅稳定同位素溯源研究[J].环境科学,2013,34(2):476-483.
[28]Gao B,Liang X R,Zhou H D,Tu X L.Lead isotopes as a tracer of Pb origin in the sediments from Beijiang River,South China[J].Water Science and Technology.2012,66(12):2613-2619.
[29]Alain C,Philippe N,Catherine G.Direct determination of lead isotope in rainwater using inductively coupled plasma mass spectrometry[J].Journal of Analytical Atomic Spectrometry,1998,13:1069-1073.
[30]Stephane Roy,Philippe Negrel.A Pb isotope and trace element study of rainwater from Massif Central(France)[J].Science of the Total Environment,2001,277:225-239.
[31]Moller P,Dulski P,Gerstenberger H,Morteani G,Fuganti A.Rare earth,yttrium and H,O,C,Sr,Nd and Pb isotope studies in mineral waters and corresponding rocks from NM-Bohemia,Czech Republic[J].Applied Geochemistry,1998,13(8):975-994.
[32]Siddle W C,Li P.Impact of submersible pumps on Pb constituents in residential wells[J].Environmental Geochemistry and Health,2008,30:1-9.
[33]Amy E K,Matthew K,Reuer,Nathalie F G,Edward A B.Lead concentrations and isotopes in corals and water near Bermuda,1780-2000[J].Earth and Planetary Science Letters,2009,283:93-100.
[34]Barta C,Markich S J,Baird D J,et al.The relative importance of water and food as cadmium sources to Daphnia Magana Straus[J].Aquatic Toxicology,2002,61:143-154.
[35]Roy I,Hare L.Relative importance of water and food as cadmium source to the predatory insect Sialius valata(Megaloptera)[J].Canadian Journal of Fisheries and Aquatic Sciences,1999,56:1143-1149.
[36]Ip C C M,Li X D,Zhang G,Farmer J G,Wai O W H,Li Y S.Over one hundred years of trace metal fluxes in the sediments of the Pearl River Estuary,South China[J].Environmental Pollution,2004,132:157-172.
[37]Ip C C M,Li X D,Zhang G,Wong C S C,Zhang W L.Heavy metal and Pb isotopic compositions of aquatic organisms in the Pearl River Estuary,South China[J].Environmental Pollution,2005,138:494-504.
[38]Ip C C M,Li X D,Zhang G,Wai O W H,Li Y S.Trace metal distribution in sediments of the Pearl River Estuary and the surrounding coastal area,south China[J].Environmental Pollution,2007,147:311-323.
[2]Sturges W T,Barrie L A.Lead 206/207 isotopes rations in atmosphere of North American as tracers of US and Canadian emissions[J].Nature,1987,329:144-146.
[3]吴龙华,张长波,章海波,等.铅稳定同位素在土壤污染物来源识别中的应用[J].环境科学,2009,30(1):227-230.
[4]黄勇,高博,王健康,等.新疆石河子城区道路尘土的铅污染和铅同位素示踪研究[J].岩矿测试,2013,32(4):632-637.
[5]Blaisjules M.Using isotopic tracers in lake sediments to assess atmospheric transport of lead in eastern Canada[J].Water,Air and Soil Pollution,1996,92(3/4):329-342.
[6]Bur T,Prost J L,Nguessan M,et al.Distribution and origin of lead in stream sediments from small agricultural catchments draining Miocene molassic deposits(SW France)[J].Applied Geochemistry,2009,24:1324-1338.
[7]朱赖民,张海生,陈立奇,等.Pb稳定同位素在示踪环境污染中的应用[J].环境科学研究,2002,15(1):27-30.
[8]武永锋,陈建华.铅同位素在环境地球化学中的应用与进展[J].微量元素与健康研究,2009,26(2):65-67.
[9]于瑞莲,胡恭任,袁星,等.同位素示踪技术在沉积物重金属污染溯源中的应用[J].地球与环境,2008,36(3):245-250.
[10]Komárek M,Ettler V,ChrastnyV,et al.Lead isotopes in environmental sciences:A review[J].Environment International,2008,34(4):562-577.
[11]肖敏.沉积物重金属污染源的铅同位素示踪研究[J].现代商业工业,2011,23:322-323.
[12]Cheng H F,Hu Y A.Lead(Pb)isotopic fingerprinting and its applications in lead pollution studies in China:A review[J].Environmental Pollution,2010,158:1-13.
[13]伊慧,伊观.铅稳定同位素在环境污染示踪中的应用和进展[J].广东微量元素科学,2007,14(5):1-5.
[14]余伟河,于瑞莲,胡恭任.铅锌镉同位素在土壤和沉积物重金属污染溯源研究中的应用进展[J].有色金属工程,2012,4:57-62.
[15]Eades L J,Farmer J G,Mackenzie A B,et al.Stable lead isotopic characterization of the historical record of environmental lead contamination in dated freshwater lake sediment cores from Northern and Central Scotland[J].The Science of the Total Environment,2002,292:55-67.
[16]Gallon C,Tessier A,Gobeil C,Carignan R.Historical perspective of industrial lead emission to the atmospherefrom a Canadian smelter.Environ Sci Technol 2006,40:741-7.
[17]Abi-Ghanem C,Chiffoleau J F,Bermond A,et al.Lead and its isotopes in the sediment of three sites on the Leabanese coast:identification of contamination sources and mobility[J].Applied Geochemistry,2009,24:1990-1999.
[18]Harlavan Y,Labin A A,Herut B.Tracing natural and anthropogenic Pb in sediments along the Mediterranean coast of Israel using Pb Isotopes[J].Environmental Science and Technology,2010,44(17):6576-6582.
[19]Angelidis M O,Radakovitch O,Veron A,et al.Anthropogenic metal contamination and sapropel imprints in deep Mediterranean sediments[J].Marine Pollution Bulletin,2011,62:1041-1052.
[20]Bird G,Brewer P A,Macklin M G,et al.Quantifying sediment-associated metal dispersal using Pb isotopes:Application of binary and multivariate mixing models at the catchment-scale[J].Environment Pollution,2010,158:2158-2169.
[21]Sun G X,Wang X J,Hu Q H,Using stable lead isotopes to trace heavy metal contamination sources in sediments of Xiangjiang and Lishui Rivers in China[J].Environmental Pollution,2011,159:3406-3410.
[22]彭渤,唐晓燕,等.湘江入湖河段沉积物重金属污染及其Pb同位素地球化学示踪[J].地质学报,2011,85(2):282-299.
[23]Choi M S,Yi H I,Yang S Y,Lee C B,Cha H J.Identification of Pb sources in Yellow Sea sediments using stable Pb isotope ratios[J].Marine Chemistry,2007,107:255–274.
[24]Hao Y,Guo Z,Yang Z,Fan D,Fang M,Li X.Tracking historical lead pollution in the coastal area adjacent to the Yangtze River Estuary using lead isotopic compositions[J].Environmental Pollution,2008,156,1325–1331.
[25]Hu X,Wang C,Zou L M.Characteristics of heavy metals and Pb isotopic signatures in sediment cores collected from typical urban shallow lakes in Nanjing,China[J].Journal of Environmental Management,2010,10:1-7.
[26]Zhu L M,Guo L D,Gao Z Y,et al.Source and distribution of lead in the surface sediments from the South China Sea as derived from Pb isotopes[J].Marine Pollution Bulletin,2010,60:2144-2153.
[27]徐林波,高勤峰,董双林,等.靖海湾重金属污染及铅稳定同位素溯源研究[J].环境科学,2013,34(2):476-483.
[28]Gao B,Liang X R,Zhou H D,Tu X L.Lead isotopes as a tracer of Pb origin in the sediments from Beijiang River,South China[J].Water Science and Technology.2012,66(12):2613-2619.
[29]Alain C,Philippe N,Catherine G.Direct determination of lead isotope in rainwater using inductively coupled plasma mass spectrometry[J].Journal of Analytical Atomic Spectrometry,1998,13:1069-1073.
[30]Stephane Roy,Philippe Negrel.A Pb isotope and trace element study of rainwater from Massif Central(France)[J].Science of the Total Environment,2001,277:225-239.
[31]Moller P,Dulski P,Gerstenberger H,Morteani G,Fuganti A.Rare earth,yttrium and H,O,C,Sr,Nd and Pb isotope studies in mineral waters and corresponding rocks from NM-Bohemia,Czech Republic[J].Applied Geochemistry,1998,13(8):975-994.
[32]Siddle W C,Li P.Impact of submersible pumps on Pb constituents in residential wells[J].Environmental Geochemistry and Health,2008,30:1-9.
[33]Amy E K,Matthew K,Reuer,Nathalie F G,Edward A B.Lead concentrations and isotopes in corals and water near Bermuda,1780-2000[J].Earth and Planetary Science Letters,2009,283:93-100.
[34]Barta C,Markich S J,Baird D J,et al.The relative importance of water and food as cadmium sources to Daphnia Magana Straus[J].Aquatic Toxicology,2002,61:143-154.
[35]Roy I,Hare L.Relative importance of water and food as cadmium source to the predatory insect Sialius valata(Megaloptera)[J].Canadian Journal of Fisheries and Aquatic Sciences,1999,56:1143-1149.
[36]Ip C C M,Li X D,Zhang G,Farmer J G,Wai O W H,Li Y S.Over one hundred years of trace metal fluxes in the sediments of the Pearl River Estuary,South China[J].Environmental Pollution,2004,132:157-172.
[37]Ip C C M,Li X D,Zhang G,Wong C S C,Zhang W L.Heavy metal and Pb isotopic compositions of aquatic organisms in the Pearl River Estuary,South China[J].Environmental Pollution,2005,138:494-504.
[38]Ip C C M,Li X D,Zhang G,Wai O W H,Li Y S.Trace metal distribution in sediments of the Pearl River Estuary and the surrounding coastal area,south China[J].Environmental Pollution,2007,147:311-323.