应用质子转移反应质谱法评价猪场恶臭
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- 英文论文题名：Odorant Measurement from Swine Production by Proton Transfer Reaction Mass Spectrometry
- 论文作者：刘德钊 ; 满尊 ; 费堡-安德森
- 英文论文作者：Liu Dezhao ; Man Zun ; Feilberg Anders ; Zhejiang University ; College of Biosystems and Food Science ; Aarhus University
- 年：2016
- 作者机构：浙江大学生物系统工程与食品科学学院;丹麦奥胡斯大学工学院;
- 论文关键词：质子转移反应质谱仪 ; 在线检测 ; 猪场 ; 恶臭评价
- 会议召开时间：2016-11-17
- 会议录名称：第六届全国恶臭污染测试与控制技术研讨会论文集
- 语种：中文
- 分类号：X831;S828;O657.63
- 学会代码：GJHB
- 会议名称：第六届全国恶臭污染测试与控制技术研讨会
- 会议地点：中国上海
- 主办单位：国家环境保护恶臭污染控制重点实验室
- 学会名称：国家环境保护恶臭污染控制重点实验室
- 页数：6
- 文件大小：983k
- 原文格式：D
- 会议级别：全国
摘要
质子转移反应质谱法在近年来在大气环境等领域得到了广泛应用。质子转移反应质谱法在测量低浓度VOCs方面具有在线、快速、灵敏度高等优势,因此在测量畜禽场低浓度恶臭方面具有较好的应用潜力。另外目前的欧洲标准方法暨动态恶臭嗅辩仪具有稳定性不足并受到采样方法的较大限制。而作为直接采样法的质子转移反应质谱仪法在集中式猪场恶臭的现场及离线测量应用表明了其较好的适用性,有望对恶臭测量标准方法起到良好的推动作用。
Proton Transfer Reaction Mass Spectrometry(PTR-MS) was widely applied during the past decade especially within the area of atmospheric environment.PTR-MS has the advantages of online,fast response and high sensitivity(and thus low detection limit) when measuring low concentrations of VOCs,and thus has a potential of being used for odorants quantification emitted from intensive animal production.The European standard method for odor measurement,namely the dynamic olfactometry,has apparent limitations especially on sampling.On the contrary,the usage of PTR-MS on odorants measurement with no sampling process demonstrated the applicability of the method and may help to build a new standard method for odor measurement.
Proton Transfer Reaction Mass Spectrometry(PTR-MS) was widely applied during the past decade especially within the area of atmospheric environment.PTR-MS has the advantages of online,fast response and high sensitivity(and thus low detection limit) when measuring low concentrations of VOCs,and thus has a potential of being used for odorants quantification emitted from intensive animal production.The European standard method for odor measurement,namely the dynamic olfactometry,has apparent limitations especially on sampling.On the contrary,the usage of PTR-MS on odorants measurement with no sampling process demonstrated the applicability of the method and may help to build a new standard method for odor measurement.
引文
[1]Wing,S.,Horton,R.A.,Marshall,S.W.,Thu,K.,Tajik,M.,Schinasi,L.and Schiffman,S.S.(2008).Air pollution and odor in communities near industrial swine operations.Environmental Health Perspectives,116(10),1362-1368.
[2]Nimmermark,S.(2011).Influence of odour concentration and individual odour thresholds on the hedonic tone of odour from animal production.Biosystems Engineering,108(3),211-219.
[3]Wing,S.and Wolf,S.(2000).Intensive livestock operations,health and quality of life among eastern North Carolina residents.Environmental health perspectives,108(3),233-238.
[4]Schiffman,S.S.,Studwell,C.E.,Landerman,L.R.,Berman,K.and Sundy,J.S.(2005).Symptomatic effects of exposure to diluted air sampled from a swine confinement atmosphere on healthy human subjects.Environmental Health Perspectives,113(5),567-576.
[5]包景岭,邹克华,王连生.恶臭环境管理与污染控制[M].北京:中国环境科学出版社,2009:3-4.
[6]张欢,包景岭,王元刚.恶臭污染评价分级方法[J].城市环境与城市生态.2011,24(3):37-39.
[7]Kristoffer E.N.Jonassen,Poul Pedersen,Anders L.Riis,Karen S?rensen,2012.Does the Choice of Olfactometric Laboratory Affect the Efficiency of Odour Abatement Technologies?Chemical Engineering Transaction,30,43-48.
[8]李龙,覃名翠,杨燕罡,陈文亮,徐可欣,恶臭在线检测技术.第五届全国恶臭污染测试与控制技术研讨会论文集,2014.
[9]李祚泳,彭荔红.于韦伯——费希纳拓广定律的环境空气质量标准[J].中国环境监测,2003,19(4):17-19.
[10]de Gouw,J.,Warneke,C.,2007.Measurements of volatile organic compounds in the earth’s atmosphere using proton-transfer-reaction mass spectrometry.Mass Spectrometry Reviews 26(2),223-257.
[11]Blake,R.S.,Monks,P.S.,Ellis,A.M.,2009.Proton-transfer reaction mass spectrometry.Chemical Reviews 109(3),861-896.
[12]Lindinger W,Hansel A,Jordan A.1998.On-line monitoring of volatile organic compounds at pptv levels by means of proton-transfer-reaction mass spectrometry(PTR-MS)—Medical applications,food control and environmental research.Int J Mass Spectrom173:191–241.
[13]Shaw,S.L.;Mitloehner,F.M.;Jackson,W.;Depeters,E.J.;Fadel,J.G.;Robinson,P.H.;Holzinger,R.;Goldstein,A.H.Volatile organic compound emissions from dairy cows and their waste as measured by proton-transfer-reaction mass spectrometry.Environ.Sci.Technol.2007,41(4),1310–1316.
[14]Feilberg,A.,Liu,D.,Adamsen,A.P.S.,Hansen,M.J.,Jonassen,K.,2010B.Odorant emissions from intensive pig production measured by online proton-transferreaction mass spectrometry.Environmental Science and Technology 44(15),5894-5900.
[15]Liu,D.;Feilberg,A.;Adamsen,A.P.S;Jonassen,K.E.N.The 593 effect of slurry treatment including ozonation on odorant reduction measured by in-situ PTR-MS.Atmos.Environ.2011,45,3786-3793.
[16]Hansen M.J.,Liu D.,Guldberg L.B.,Feilberg A.,2012.Application of proton-transfer-reaction mass spectrometry to the assessment of odorant removal in a biological air cleaner for pig production.Journal of Agricultural and Food Chemistry,60(10),2599-2606.
[17]Liu D.,Andreasen R.R.,Poulsen T.G.,Feilberg A.,2013.Experimental determination of mass transfer coefficients of volatile sulfur odorants in biofilter media measured by Proton-Transfer-Reaction Mass Spectrometry(PTR-MS).Chemical Engineering Journal,219,335-345.
[2]Nimmermark,S.(2011).Influence of odour concentration and individual odour thresholds on the hedonic tone of odour from animal production.Biosystems Engineering,108(3),211-219.
[3]Wing,S.and Wolf,S.(2000).Intensive livestock operations,health and quality of life among eastern North Carolina residents.Environmental health perspectives,108(3),233-238.
[4]Schiffman,S.S.,Studwell,C.E.,Landerman,L.R.,Berman,K.and Sundy,J.S.(2005).Symptomatic effects of exposure to diluted air sampled from a swine confinement atmosphere on healthy human subjects.Environmental Health Perspectives,113(5),567-576.
[5]包景岭,邹克华,王连生.恶臭环境管理与污染控制[M].北京:中国环境科学出版社,2009:3-4.
[6]张欢,包景岭,王元刚.恶臭污染评价分级方法[J].城市环境与城市生态.2011,24(3):37-39.
[7]Kristoffer E.N.Jonassen,Poul Pedersen,Anders L.Riis,Karen S?rensen,2012.Does the Choice of Olfactometric Laboratory Affect the Efficiency of Odour Abatement Technologies?Chemical Engineering Transaction,30,43-48.
[8]李龙,覃名翠,杨燕罡,陈文亮,徐可欣,恶臭在线检测技术.第五届全国恶臭污染测试与控制技术研讨会论文集,2014.
[9]李祚泳,彭荔红.于韦伯——费希纳拓广定律的环境空气质量标准[J].中国环境监测,2003,19(4):17-19.
[10]de Gouw,J.,Warneke,C.,2007.Measurements of volatile organic compounds in the earth’s atmosphere using proton-transfer-reaction mass spectrometry.Mass Spectrometry Reviews 26(2),223-257.
[11]Blake,R.S.,Monks,P.S.,Ellis,A.M.,2009.Proton-transfer reaction mass spectrometry.Chemical Reviews 109(3),861-896.
[12]Lindinger W,Hansel A,Jordan A.1998.On-line monitoring of volatile organic compounds at pptv levels by means of proton-transfer-reaction mass spectrometry(PTR-MS)—Medical applications,food control and environmental research.Int J Mass Spectrom173:191–241.
[13]Shaw,S.L.;Mitloehner,F.M.;Jackson,W.;Depeters,E.J.;Fadel,J.G.;Robinson,P.H.;Holzinger,R.;Goldstein,A.H.Volatile organic compound emissions from dairy cows and their waste as measured by proton-transfer-reaction mass spectrometry.Environ.Sci.Technol.2007,41(4),1310–1316.
[14]Feilberg,A.,Liu,D.,Adamsen,A.P.S.,Hansen,M.J.,Jonassen,K.,2010B.Odorant emissions from intensive pig production measured by online proton-transferreaction mass spectrometry.Environmental Science and Technology 44(15),5894-5900.
[15]Liu,D.;Feilberg,A.;Adamsen,A.P.S;Jonassen,K.E.N.The 593 effect of slurry treatment including ozonation on odorant reduction measured by in-situ PTR-MS.Atmos.Environ.2011,45,3786-3793.
[16]Hansen M.J.,Liu D.,Guldberg L.B.,Feilberg A.,2012.Application of proton-transfer-reaction mass spectrometry to the assessment of odorant removal in a biological air cleaner for pig production.Journal of Agricultural and Food Chemistry,60(10),2599-2606.
[17]Liu D.,Andreasen R.R.,Poulsen T.G.,Feilberg A.,2013.Experimental determination of mass transfer coefficients of volatile sulfur odorants in biofilter media measured by Proton-Transfer-Reaction Mass Spectrometry(PTR-MS).Chemical Engineering Journal,219,335-345.