New Applications of Hybrid Perovskites Beyond solar cells:Solar Battery and Resistive Random Access Memory Devices
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- 英文论文题名：New Applications of Hybrid Perovskites Beyond solar cells:Solar Battery and Resistive Random Access Memory Devices
- 论文作者：Miaoqiang Lyu ; Eunji Yoo ; Jung-Ho Yun ; Qiong Wang ; 王连洲
- 英文论文作者：Miaoqiang Lyu ; Eunji Yoo ; Jung-Ho Yun ; Qiong Wang ; Lianzhou Wang ; Nanomaterials Centre ; School of Chemical Engineering and AIBN ; the University of Queensland
- 年：2017
- 作者机构：澳大利亚昆士兰大学;
- 英文论文关键词：organic-inorganic perovskite solar cells ; memory devices ; solar battery ; lead-free perovskites
- 会议召开时间：2017-05-27
- 会议录名称：第四届新型太阳能电池学术研讨会论文集
- 英文会议录名称：Abstract Book of the 4th Conference on New Generation Solar Cells
- 语种：英文
- 分类号：TM914.4
- 学会代码：ZKYQ
- 会议名称：第四届新型太阳能电池学术研讨会
- 会议地点：中国北京
- 主办单位：中国可再生能源学会光化学专业委员会
- 学会名称：中国科学院物理研究所清洁能源实验室
- 页数：1
- 文件大小：460k
- 原文格式：D
- 会议级别：全国
摘要
Organic-inorganic hybrid perovskite materials have been demonstrated to be highly performed light absorbers for high efficient perovskite solar cells.In addition to solar cells applications,the materials have also demonstrated versatile functionalities in a number of fields.Herein,we give the first demonstration of remarkable resistive switching behaviour in organic-inorganic hybrid perovskite materials(CH_3NH_3PbI_(3-x)Cl_x),which can be applicable in the resistive random access memory(RRAM)devices.~1 The hybrid perovskite material with high crystallinity can be readily fabricated by a low-temperature,solutionprocessable method.The simply designed Au/CH_3NH_3PbI_(3-x)Cl_x/FTO structure exhibits remarkable resistive switching behaviour with excellent endurance(>100 cycles),long retention time(>10~4 s)with a very small on-off voltage of<1 V.The resistive switching behaviour of the organic-inorganic hybrid perovskite-based device is originated from the intrinsic dielectric and defect properties of the CH_3NH_3PbI_(3-x)Cl_x material,corresponding to the space charge limited conduction(SCLC)mechanism.By dissolving organolead perovskites in organic solvents,a new type of in-situ solar conversion and energy storage system,so called solar battery,is also demonstrated.~2,On another attempt,new types of lead-free hybrid perovskite solar cells is also studied.~3
Organic-inorganic hybrid perovskite materials have been demonstrated to be highly performed light absorbers for high efficient perovskite solar cells.In addition to solar cells applications,the materials have also demonstrated versatile functionalities in a number of fields.Herein,we give the first demonstration of remarkable resistive switching behaviour in organic-inorganic hybrid perovskite materials(CH_3NH_3PbI_(3-x)Cl_x),which can be applicable in the resistive random access memory(RRAM)devices.~1 The hybrid perovskite material with high crystallinity can be readily fabricated by a low-temperature,solutionprocessable method.The simply designed Au/CH_3NH_3PbI_(3-x)Cl_x/FTO structure exhibits remarkable resistive switching behaviour with excellent endurance(>100 cycles),long retention time(>10~4 s)with a very small on-off voltage of<1 V.The resistive switching behaviour of the organic-inorganic hybrid perovskite-based device is originated from the intrinsic dielectric and defect properties of the CH_3NH_3PbI_(3-x)Cl_x material,corresponding to the space charge limited conduction(SCLC)mechanism.By dissolving organolead perovskites in organic solvents,a new type of in-situ solar conversion and energy storage system,so called solar battery,is also demonstrated.~2,On another attempt,new types of lead-free hybrid perovskite solar cells is also studied.~3
Organic-inorganic hybrid perovskite materials have been demonstrated to be highly performed light absorbers for high efficient perovskite solar cells.In addition to solar cells applications,the materials have also demonstrated versatile functionalities in a number of fields.Herein,we give the first demonstration of remarkable resistive switching behaviour in organic-inorganic hybrid perovskite materials(CH_3NH_3PbI_(3-x)Cl_x),which can be applicable in the resistive random access memory(RRAM)devices.~1 The hybrid perovskite material with high crystallinity can be readily fabricated by a low-temperature,solutionprocessable method.The simply designed Au/CH_3NH_3PbI_(3-x)Cl_x/FTO structure exhibits remarkable resistive switching behaviour with excellent endurance(>100 cycles),long retention time(>10~4 s)with a very small on-off voltage of<1 V.The resistive switching behaviour of the organic-inorganic hybrid perovskite-based device is originated from the intrinsic dielectric and defect properties of the CH_3NH_3PbI_(3-x)Cl_x material,corresponding to the space charge limited conduction(SCLC)mechanism.By dissolving organolead perovskites in organic solvents,a new type of in-situ solar conversion and energy storage system,so called solar battery,is also demonstrated.~2,On another attempt,new types of lead-free hybrid perovskite solar cells is also studied.~3
引文
[1]Yoo,E,Lyu,M,Wang,L,et al,Adv.Mater.,2015,27(40),6170-6175
[2]Wang Q.,Yun,J.,Wang,L,et al,Adv.Energy Mater.,2015,5,1501418.
[3]Lyu M,Wang L,Adv.Energy Mater.,2017,DOI:10.1002/aenm.201602512
[2]Wang Q.,Yun,J.,Wang,L,et al,Adv.Energy Mater.,2015,5,1501418.
[3]Lyu M,Wang L,Adv.Energy Mater.,2017,DOI:10.1002/aenm.201602512