基于多光子吸收效应的激光脉冲平滑技术研究
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摘要
激光脉冲时间调制严重威胁聚变驱动器的运行安全甚至使点火失败,必须消除或有效抑制。谱域的抑制方法技术难度高或依赖于光谱的精确测量并仅适用于特定光谱,限制了在实际激光装置中的广泛使用。因此,能够在实际中灵活应用的脉冲时间调制平滑方法的研究具有重要意义。
本论文提出了基于多光子吸收效应平滑脉冲调制的新方法,开展了多光子吸收效应脉冲匀滑特性的研究,分析了多光子吸收材料参数对平滑效果的影响,论证了多光子吸收应用于整形脉冲时域调制平滑的可行性。
基于描述激光与多光子吸收体相互作用的耦合方程,系统研究了时空调制超高斯脉冲与多光子吸收体相互作用的动力学过程,获得了多光子吸收体脉冲时空平滑的主要物理规律。多光子吸收具有强度依赖性,相当于时空上强度分辨的透过率函数,能够有效平滑脉冲时空调制。伴随多光子吸收发生的激发态吸收能够降低脉冲空间调制但造成脉冲时间波形后沿塌陷,并减弱对时间调制的平滑作用。设计并开展了双光子吸收脉冲平滑的实验,验证了双光子吸收机制具有显著的脉冲平滑效果,并观测到了由激发态吸收导致脉冲后沿塌陷的现象。
脉冲平滑应用要求多光子吸收体的输出光束质量高、时空调制平滑能力强、能量透过率高。为获得多光子吸收平滑时空脉冲的最优表现并观察各参数的影响趋势,系统分析了多光子吸收截面、单重态三重态第一激发态吸收截面、单重态第一激发态驰豫时间以及参与多光子吸收过程的光子数对平滑效果和透过率的影响。
研究并论证了多光子吸收体平滑整形脉冲时间调制的可行性。建立了整形脉冲的时间波形预整形方法,以解决整形脉冲轮廓畸变的问题。将耦合方程简化为超越方程,并根据此方程以输出脉冲时间波形反演输入时间波形,通过预整形校正整形脉冲的轮廓畸变。定义了整形脉冲调制程度表征参数,利用该参数对整形脉冲调制的平滑效果进行了讨论。本论文的研究是对基于新型功能材料、新原理新机制的新型激光器件的一种探索,也是将激光脉冲精确控制向时域扩展的一种尝试。
Amplitude modulation might damage the optics, adversely affects the laser performance and eventually would make the inertial confinement fusion (ICF) failed, and thus needs to be eliminated or efficiently controlled. By spectrum resolved transfer functions of traditional elements, amplitude modulation could be alleviated effectively to a certain extent. However, these components just act on specific spectrum structure and the spectrum is usually complex. Meanwhile these components are costly for precision manufacture and accuracy control, and hence restrict these technologies for practical applications. Therefore, a flexible amplitude modulation suppressing method aiming at complex spectrum and practical applications is urgently demanding.
Suppression of amplitude modulation in time domain based on nonlinear absorption effect is proposed. The smoothing characteristics of multiphoton absorption are investigated. The effects of several parameters of multiphoton absorber on smoothing are analysed, the feasibility of modulation suppressing effect of two-photon absorber on shaped pulse is also demonstrated.
The theoretical model coupling the propagation equation with the rate equations is employed to study the dynamics of nonlinear absorbers interacting with spatiotemporal modulation pulse, and the main smoothing rules are abtained. Spatiotemporal modulation can be alleviated simultaneously by two-photon absorption because of its intensity dependent characteristic. The following excited stateabsorption can suppress spatial modulation but induce temporal distortion, and reduce the suppressing temporal modulation effect. The modulation smoothing effect of two-photon absorption is demonstrated experimently. The temporal shape distortion caused by the excited state absorption is also observed. In comparison with traditional methods in spectrum domain, this approach needs no detailed spectrum structure, leading to convenient design and manufacture in practice.
Different from traditional optical limiters, high beam quality, efficient amplitude modulation suppressing capability and high energy transmission are the general requirments in beam smoothing applications. In order to assess the ultimate performance of TPA on amplitude modulation suppressing and to see trends, the effects of several parameters such as ESA cross section, relaxation time of first singlet excited state, TPA cross section, molecules consentration and the photon numbers on the temporal pulse shape, modulation suppressing efficiency and transmittance are quantitatively analysised in detail.
The feasibility of modulation suppressing effect of two photon absorber on shaped pulse is studied. In order to eliminate the contour distortion of shaped pulse, we propose an analytic method to preshape the input pulse. By defining a characterization parameter for shaped pulse modulation, the modulation suppressing effect of two photon absorption on shaped pulse is evaluated. This thesis is an exploration of new laser element based on new material and new mechanism, also a try to expand the laser pulse control technology to time domain.
本论文提出了基于多光子吸收效应平滑脉冲调制的新方法,开展了多光子吸收效应脉冲匀滑特性的研究,分析了多光子吸收材料参数对平滑效果的影响,论证了多光子吸收应用于整形脉冲时域调制平滑的可行性。
基于描述激光与多光子吸收体相互作用的耦合方程,系统研究了时空调制超高斯脉冲与多光子吸收体相互作用的动力学过程,获得了多光子吸收体脉冲时空平滑的主要物理规律。多光子吸收具有强度依赖性,相当于时空上强度分辨的透过率函数,能够有效平滑脉冲时空调制。伴随多光子吸收发生的激发态吸收能够降低脉冲空间调制但造成脉冲时间波形后沿塌陷,并减弱对时间调制的平滑作用。设计并开展了双光子吸收脉冲平滑的实验,验证了双光子吸收机制具有显著的脉冲平滑效果,并观测到了由激发态吸收导致脉冲后沿塌陷的现象。
脉冲平滑应用要求多光子吸收体的输出光束质量高、时空调制平滑能力强、能量透过率高。为获得多光子吸收平滑时空脉冲的最优表现并观察各参数的影响趋势,系统分析了多光子吸收截面、单重态三重态第一激发态吸收截面、单重态第一激发态驰豫时间以及参与多光子吸收过程的光子数对平滑效果和透过率的影响。
研究并论证了多光子吸收体平滑整形脉冲时间调制的可行性。建立了整形脉冲的时间波形预整形方法,以解决整形脉冲轮廓畸变的问题。将耦合方程简化为超越方程,并根据此方程以输出脉冲时间波形反演输入时间波形,通过预整形校正整形脉冲的轮廓畸变。定义了整形脉冲调制程度表征参数,利用该参数对整形脉冲调制的平滑效果进行了讨论。本论文的研究是对基于新型功能材料、新原理新机制的新型激光器件的一种探索,也是将激光脉冲精确控制向时域扩展的一种尝试。
Amplitude modulation might damage the optics, adversely affects the laser performance and eventually would make the inertial confinement fusion (ICF) failed, and thus needs to be eliminated or efficiently controlled. By spectrum resolved transfer functions of traditional elements, amplitude modulation could be alleviated effectively to a certain extent. However, these components just act on specific spectrum structure and the spectrum is usually complex. Meanwhile these components are costly for precision manufacture and accuracy control, and hence restrict these technologies for practical applications. Therefore, a flexible amplitude modulation suppressing method aiming at complex spectrum and practical applications is urgently demanding.
Suppression of amplitude modulation in time domain based on nonlinear absorption effect is proposed. The smoothing characteristics of multiphoton absorption are investigated. The effects of several parameters of multiphoton absorber on smoothing are analysed, the feasibility of modulation suppressing effect of two-photon absorber on shaped pulse is also demonstrated.
The theoretical model coupling the propagation equation with the rate equations is employed to study the dynamics of nonlinear absorbers interacting with spatiotemporal modulation pulse, and the main smoothing rules are abtained. Spatiotemporal modulation can be alleviated simultaneously by two-photon absorption because of its intensity dependent characteristic. The following excited stateabsorption can suppress spatial modulation but induce temporal distortion, and reduce the suppressing temporal modulation effect. The modulation smoothing effect of two-photon absorption is demonstrated experimently. The temporal shape distortion caused by the excited state absorption is also observed. In comparison with traditional methods in spectrum domain, this approach needs no detailed spectrum structure, leading to convenient design and manufacture in practice.
Different from traditional optical limiters, high beam quality, efficient amplitude modulation suppressing capability and high energy transmission are the general requirments in beam smoothing applications. In order to assess the ultimate performance of TPA on amplitude modulation suppressing and to see trends, the effects of several parameters such as ESA cross section, relaxation time of first singlet excited state, TPA cross section, molecules consentration and the photon numbers on the temporal pulse shape, modulation suppressing efficiency and transmittance are quantitatively analysised in detail.
The feasibility of modulation suppressing effect of two photon absorber on shaped pulse is studied. In order to eliminate the contour distortion of shaped pulse, we propose an analytic method to preshape the input pulse. By defining a characterization parameter for shaped pulse modulation, the modulation suppressing effect of two photon absorption on shaped pulse is evaluated. This thesis is an exploration of new laser element based on new material and new mechanism, also a try to expand the laser pulse control technology to time domain.
引文
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