飞秒激光多维信息存储关键技术研究
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摘要
现代科技对数据容量需求的急速增长使超高密度信息存储技术成为当代信息技术领域重要的研究课题。多维信息存储改变了原有光存储技术依靠缩短激光波长和增加物镜数值孔径来提高存储密度的传统思路,在几何三维空间之外，选择其他可以影响数据写入和读取的物理特性参量建立独立的坐标系,可以将多重信息记录到存储介质的同一物理空间上,并实现独立的读取,从而增加信息存储的维度。多维信息存储技术可实现的存储容量大,控制灵活方便,已成为下一代光存储技术发展的重要方向之一。本文结合飞秒激光双光子吸收的三维高分辨优势和偶氮苯材料的光致异构取向重分布特性,发展了偏振多元多阶信息存储技术,并对其中的关键间题进行了理论和实验研究。
首先,介绍了偶氮苯的双光子光响应性质及机理,包括双光子光致异构、光致取向和光致取向烧孔等；对双光子光致异构速率方程和光致取向速率方程分别进行了描述；对于其中最重要的光致各向异性性质——光致双折射进行了理论分析和实验测量；对研究非线性光学特性的Z扫描方法进行了介绍,并对实验结果进行了分析。
其次,搭建了飞秒激光双光子偏振存储系统并实现了偏振多元信息存储；分别利用偏振透射光读出,偏光读出和反射式扫描共焦读出三种方式验证了利用飞秒激光实现可擦除的偏振多元存储的可行性：存储密度理论值可以达到250Gb/cm3;还对存储过程中曝光剂量对信息点强度和大小的影响进行了实验研究和理论分析,为写入参数的进一步优化提供依据。
另外,双偶氮苯poly(M2BAN-co-MMA)聚合物的偏振存储过程中,当曝光量超过特定阈值时,会出现灰阶低于背景的暗点。本文利用这一性质实现了偏振多阶信息存储：同时通过对与入光曝光时间的控制实现了9阶信息存储,并讨论了多阶信息存储中的影响因素；对偏振飞秒激光在双偶氮苯聚合物薄膜中诱导产生表面形貌进行了深入的理论模型研究和实验分析,结果表明电场梯度力模型可以很好的解释偏振激光引起的表面形貌；并且对不同曝光条件下的偏振存储进行了详细的讨论。
最后,论文进行了基于空间光调制器的三维并行存储技术的初步研究；详细介绍了空间光调制器的结构以及调制机理；设计了三维计算全息算法并在此基础上实现了多层图像的设计和重现,验证了三维动态并行数据存储的可行性；同时考虑了折射率失配引起的离焦和球差对三维动态并行存储的影响并提出在全息算法迭代过程中进行补偿,为下一步实现并行多维信息存储和高效高分辨跨尺度全息并行加工奠定了基础。
The urgently increasing requirement on data storage capacity makes the super-high density storage technology to be one of the most important research topics. Different from the traditional optical storage technologies which depends on shortening the laser wavelength and decreasing the objective numerical aperture to achieve higher storage density, multi-dimensional data storage introduces other parameters besides the geometric space that can influence the recording and reading process, builds individual coordinates, finally records multiplex information inside the identical space of storage medium. Recorded data can be individually read out. This technology has the advantage of super-high storage capacity and easy to control. It has become a promising candidate for next generation optical storage. In this dissertation, both the high resolution of two-photon absorption and photoinduced isomeric reorientation properties of azobenzene chromophores are combined to develop a novel polarization-multiplexed and multilevel data storage method. Some key issues of the multi-dimensional data storage are theoretically and experimentally investigated.
Firstly, the two-photon optical response property and mechanism of azobenzene polymer is introduced, including photoinduced isomerization, reorientation and orientational hole burning; The two-photon isomerization rate equation and reorientation rate equation are described; Furthermore, as the most important anisotropy character, photoinduced birefringence is theoretically analyzed and experimentally measured; Z scan technique, which is wildly used to characterize the material nonlinear optical properties, is introduced and the experimental result is analyzed.
Secondly, a femtosecond laser two-photon polarization storage system is built to achieve polarization multiplexed data storage; Transmission polarized light readout configuration, polarizing microscopy, and reflective scanning confocal microscopy setup are respectively used to read out the recorded bits, and the feasibility of erasable and rewritable polarization storage is confirmed; The storage density can reach as high as250Gb/cm3; The influence of exposure dose (e.g. exposure time, power) on the bits intensity and size is also investigated, providing a basis for the optimization of recording parameters.
Thirdly, when the exposure dose exceeds one threshold during the polarization recording in poly(M2BAN-co-MMA), dark dots will appear when perpendicular readout. This phenomenon is used to perform polarization multilevel storage; At the same time, nine-level storage is realized by modulating the exposure dose; Some influencing factors are discussed for multilevel storage; The surface deformation induced by polarized femtosecond laser is deeply studied; The optical-field gradient force model is applied to explain the surface deformation; Three-stage recording in polarization storage is discussed.
Finally, basic research on three-dimensional parallel recording based on spatial light modulator (SLM) is carried out; The structure and modulation mechanism of SLM are circumstantiated;3D computer generate hologram (CGH) algorithm is designed and multi-layer images reconstruction is performed based on this; The defocus and spherical aberration caused by refractive mismatch are considered and proposed to be compensated in the3D computer generate hologram algorithm; All the work lay a foundation for next step parallel multi-dimensional data storage and dynamic holographic parallel processing technology.
首先,介绍了偶氮苯的双光子光响应性质及机理,包括双光子光致异构、光致取向和光致取向烧孔等；对双光子光致异构速率方程和光致取向速率方程分别进行了描述；对于其中最重要的光致各向异性性质——光致双折射进行了理论分析和实验测量；对研究非线性光学特性的Z扫描方法进行了介绍,并对实验结果进行了分析。
其次,搭建了飞秒激光双光子偏振存储系统并实现了偏振多元信息存储；分别利用偏振透射光读出,偏光读出和反射式扫描共焦读出三种方式验证了利用飞秒激光实现可擦除的偏振多元存储的可行性：存储密度理论值可以达到250Gb/cm3;还对存储过程中曝光剂量对信息点强度和大小的影响进行了实验研究和理论分析,为写入参数的进一步优化提供依据。
另外,双偶氮苯poly(M2BAN-co-MMA)聚合物的偏振存储过程中,当曝光量超过特定阈值时,会出现灰阶低于背景的暗点。本文利用这一性质实现了偏振多阶信息存储：同时通过对与入光曝光时间的控制实现了9阶信息存储,并讨论了多阶信息存储中的影响因素；对偏振飞秒激光在双偶氮苯聚合物薄膜中诱导产生表面形貌进行了深入的理论模型研究和实验分析,结果表明电场梯度力模型可以很好的解释偏振激光引起的表面形貌；并且对不同曝光条件下的偏振存储进行了详细的讨论。
最后,论文进行了基于空间光调制器的三维并行存储技术的初步研究；详细介绍了空间光调制器的结构以及调制机理；设计了三维计算全息算法并在此基础上实现了多层图像的设计和重现,验证了三维动态并行数据存储的可行性；同时考虑了折射率失配引起的离焦和球差对三维动态并行存储的影响并提出在全息算法迭代过程中进行补偿,为下一步实现并行多维信息存储和高效高分辨跨尺度全息并行加工奠定了基础。
The urgently increasing requirement on data storage capacity makes the super-high density storage technology to be one of the most important research topics. Different from the traditional optical storage technologies which depends on shortening the laser wavelength and decreasing the objective numerical aperture to achieve higher storage density, multi-dimensional data storage introduces other parameters besides the geometric space that can influence the recording and reading process, builds individual coordinates, finally records multiplex information inside the identical space of storage medium. Recorded data can be individually read out. This technology has the advantage of super-high storage capacity and easy to control. It has become a promising candidate for next generation optical storage. In this dissertation, both the high resolution of two-photon absorption and photoinduced isomeric reorientation properties of azobenzene chromophores are combined to develop a novel polarization-multiplexed and multilevel data storage method. Some key issues of the multi-dimensional data storage are theoretically and experimentally investigated.
Firstly, the two-photon optical response property and mechanism of azobenzene polymer is introduced, including photoinduced isomerization, reorientation and orientational hole burning; The two-photon isomerization rate equation and reorientation rate equation are described; Furthermore, as the most important anisotropy character, photoinduced birefringence is theoretically analyzed and experimentally measured; Z scan technique, which is wildly used to characterize the material nonlinear optical properties, is introduced and the experimental result is analyzed.
Secondly, a femtosecond laser two-photon polarization storage system is built to achieve polarization multiplexed data storage; Transmission polarized light readout configuration, polarizing microscopy, and reflective scanning confocal microscopy setup are respectively used to read out the recorded bits, and the feasibility of erasable and rewritable polarization storage is confirmed; The storage density can reach as high as250Gb/cm3; The influence of exposure dose (e.g. exposure time, power) on the bits intensity and size is also investigated, providing a basis for the optimization of recording parameters.
Thirdly, when the exposure dose exceeds one threshold during the polarization recording in poly(M2BAN-co-MMA), dark dots will appear when perpendicular readout. This phenomenon is used to perform polarization multilevel storage; At the same time, nine-level storage is realized by modulating the exposure dose; Some influencing factors are discussed for multilevel storage; The surface deformation induced by polarized femtosecond laser is deeply studied; The optical-field gradient force model is applied to explain the surface deformation; Three-stage recording in polarization storage is discussed.
Finally, basic research on three-dimensional parallel recording based on spatial light modulator (SLM) is carried out; The structure and modulation mechanism of SLM are circumstantiated;3D computer generate hologram (CGH) algorithm is designed and multi-layer images reconstruction is performed based on this; The defocus and spherical aberration caused by refractive mismatch are considered and proposed to be compensated in the3D computer generate hologram algorithm; All the work lay a foundation for next step parallel multi-dimensional data storage and dynamic holographic parallel processing technology.
引文
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