基于遥感的浙江省大气SO_2时空动态与下垫面关系研究
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摘要
二氧化硫(Sulfur dioxide,SO2)作为大气中一种重要的痕量气体,是大气污染的主要成分之一,也是衡量人为大气污染的一个重要指标。大气遥感理论的发展为研究地球气候变化与大气环境提供了重要理论支持与技术手段。了解中国地区SO2分布及其变化对大气环境研究和空气质量控制等方面都有重要意义。浙江省作为全国发展最快的地区之一,已成为人类活动造成大气污染的典型区域。本文以中国浙江为例,采用经过Matlab与Arcgis预处理的2005年1月-2009年12月OMI传感器SO2大气边界层(planet Boundary Layer,pBL)柱浓度产品为主要数据源,结合时间序列MODIS-EVI数据获取的城市、农田和森林等土地利用信息,并辅助研究区气象站点监测数据,分析了浙江省大气边界层SO2的时空分布特征和变化趋势以及不同土地利用类型的SO2柱浓度差异。同时,以自然地理分区为依据,选取浙江省具有代表性的12个小城镇,研究了SO2柱浓度变化与地表植被覆盖率的关系。
     研究表明:在时间尺度上,SO2柱浓度随时间推移总体呈逐年下降的趋势,并且SO2柱浓度的变化存在明显的季节性特征,其中SO2柱浓度最高值出现在冬季,最低值出现在夏季,采用正弦模型拟合结果良好,拟合精度达到0.65。在空间上,浙江省大气SO2分布明显具有地域性特征。SO2浓度最高值分布在浙北平原地区,最低值分布在浙西南山区。此外,在不同土地利用类型上,城市用地作为人类活动最为强烈的地区,SO2浓度值显著高于森林、水体等其他土地利用类型。在浙江省12个小城镇中,植被覆盖率高的城镇SO2浓度显著低于植被覆盖率低的城镇,SO2浓度与地表植被覆盖率呈负相关。
     本文结果表明利用OMI SO2产品可以对特定区域大气SO2的时空动态变化进行分析,是进行区域环境遥感监测的有效手段。
Sulfur dioxide(SO2)is an important trace gas and one of the main atmospheric pollution components, and usually used as an indicator to monitor the environmental pollution. The development of theory in atmospheric remote sensing provides important theoretical support and technical means to study global climate change and atmospheric environment. Understanding the distribution of SO2 in China and its change has important significance on the atmospheric environmental research and air quality control. Being the developed district of China, Zhejiang Province is a typical region suffered from air pollutions as results of human activities. In this paper, OMI SO2 column density remotely sensed data processed by Matlab and Arcgis from 2005.1 to 2009.12 and the land use mapping using MODIS-EVI data, as well as to combine with SO2 ground measured data are get together, serve for analyzing the relationship between SO2 column densities and underlying surface of Zhejiang Province.
     The relationship between SO2 column density and vegetation coverage in 12 towns is also studied. The results indicated that the SO2 column densities in Zhejiang Province decreased from 2005 to 2009, and it showed distinct regional and seasonal variation characteristics. It has the highest concentration in winter while lowest in summer. The fitting accuracy of sinusoidal model reached to 0.65. It also presents zonal distribution and decreasing from northern to southern. Under the influence of the urbanization process, the highest SO2 column densities appeared at cities and metropolises which located in the Hangzhou-Jiaxing-Huzhou plain, northern area of Ningbo as well as the west and east of Zhejiang. Moreover the lowest column densities appeared at the forest areas which are in the south and west of Zhejiang. In addition, it has the higher SO2 column density over urban, cropland and water while lower values over forest. The result also showed that the higher SO2 column density appeared in towns which located in northern plain of Zhejiang province with lower vegetation coverage. SO2 concentration was negatively correlated with vegetation coverage.
     The results approved that the OMI SO2 column density remotely sensed data can be used in air quality monitoring at regional scale.
引文
[1]PhamM,MüllerJF,BrasseurGP,GranierC,MegieG.A3dmodelstudyoftheglobalsulphurcycle:Contributionsofanthropogenicandbiogenicsources[J].Atmosphericenvironment.1996,30(10-11):1815-1822.
    [2]吴鹏鸣.环境监测原理与应用[M]:化学工业出版社;1991.
    [3]张斌才.大气边界层SO2空间分布的OMI数据分析[D]:西北师范大学;2009.
    [4]郭培章,孙广宣,马晓民.中国工业可持续发展研究[M]:经济科学出版社;2002.
    [5]吴忠标,李伟,王莉红.城市大气环境概论.北京:化学工业出版社;2003.
    [6]蒋益民.湖南省城市与森林的大气湿沉降化学及其作用机理[D]:湖南大学;2005.
    [7]陶福绿,冯宗炜.中国南方生态系统的酸沉降临界负荷[J].中国环境科学.1999,19(001):14-17.
    [8]周琴.大气中二氧化硫的污染及防治对策[J].内蒙古环境保护.2002,14(003):12-13.
    [9]陈翠芝,陈伟国.城市主要大气污染物与呼吸系统疾病相关性浅析[J].上海环境科学.1994,13(009):27-30.
    [10]王自发,高超,谢付莹.中国酸雨模式研究回顾与所面临的挑战[J].自然杂志.2007,29(2):78-82.
    [11]杨舵,王淑民,桑修诚.乌鲁木齐市SO2浓度的分布及其可能原因[J].气象.2000,26(004):29-32.
    [12]高书然,李郁竹.空气污染的天气形势分析和预报[J].气象.1982,1:33-35.
    [13]田英.贵阳市严重大气二氧化硫污染的气象条件[J].贵州气象.1995,19(005):4-16.
    [14]朱蓉,徐大海.Capps预报方法研究[J].气象.2001,27(006):10-16.
    [15]孔斌.大连市冬季大气中二氧化硫浓度与天气型的相关性及其预报[J].辽宁气象.1995,(002):19-22.
    [16]于鹏,郭素荣.大气污染物浓度级别的统计与诊断判据[J].青岛大学学报:工程技术版.2000,15(002):72-74.
    [17]王庆梅.大气污染预报技术及有关防治对策的研究[J].中国环境监测.1999,15(002):56-58.
    [18]尚可政,付有智.兰州城区冬季空气污染预报方法研究[J].兰州大学学报:自然科学版.1998,34(004):165-170.
    [19]尚可政,祁斌.兰州冬季空气污染与地面气象要素的关系[J].甘肃科学学报.1999,11(001):1-5.
    [20]王建华,郭素荣.青岛市空气污染统计预报方法研究[J].青岛大学学报:工程技术版.1999,14(004):60-62.
    [21]佟华,邵德民.一个模拟SO2浓度分布的数值模式研究[J].南京气象学院学报.2001,24(003):371-377.
    [22]安俊岭,王自发,黄美元,陶树旺,程新金,叶红.区域空气质量数值预报模型[J].气候与环境研究.1999,4(3):244-251.
    [23]范引琪.石家庄市主要大气污染的数值预报[J].气象.2001,27(004):7-11.
    [24]汤洁,林年丰,赵凤琴.城市大气环境污染预警方法研究[J].城市环境.2001,6:1-3.
    [25]LinGY.Oxidantpredictionbydiscriminantanalysisinthesouthcoastairbasinofcalifornia[J].AtmosphericEnvironment(1967).1982,16(1):135-143.
    [26]AngellJK,SeidelD,BenjeyWG.Airresourceslaboratory[J].BulletinoftheAmericanMeteorologicalSociety.2002,83(4):521-536.
    [27]HooyberghsJ,MensinkC,DumontG,FierensF,BrasseurO.Aneuralnetworkforecastfordailyaveragepm10concentrationsinbelgium[J].Atmosphericenvironment.2005,39(18):3279-3289.
    [28]江静蓉,徐亦钢.城市植物叶片含硫量与大气SO2污染关系及其在污染状况[J].环境科学.1992,13(001):71-74.
    [29]蒋高明.植物硫含量法监测大气污染数量模型[J].中国环境科学.1995,15(003):208-214.
    [30]刘荣坤,李世承.二氧化硫对蓖麻叶质膜透性,叶绿素含量和花粉生长的影响[J].1982.
    [31]孙宝盛,单金林,邵青.环境分析监测理论与技术.北京:化学工业出版社;2004.
    [32]韩永志.统计学在理化检验中的应用:第六讲正态分布及其检验[J].理化检验:化学分册.2000,36(002):94-95.
    [33]孙红梅,彭慰先,孙桂娟.二氧化硫光谱检测技术[J].环境监测管理与技术.2004,16(003):6-8.
    [34]BurrowsJP,WeberM,BuchwitzM,RozanovV,Ladsttter-WeienmayerA,RichterA,DeBeekR,HoogenR,BramstedtK,EichmannKU.Theglobalozonemonitoringexperiment(gome):Missionconceptandfirstscientificresults[J].JournaloftheAtmosphericSciences.1999,56(2).
    [35]NeeckSP,ScoleseCJ,BordiF.Eosam-1[C]//.1998:2.
    [36]马立杰,黄海军,龚建明,崔迎春,张志珣.对流层污染测量仪(mopitt)原理及其应用[J].海洋科学.2006,30(002):81-84.
    [37]AumannHH,ChahineMT.Airs/amsu/hsboneospm-1instrumentperfromanceandproductgeneration[J].TheEarthObserver.1999,11(2).
    [38]DesnosYL,BuckC,GuijarroJ,LevriniG,SuchailJL,TorresR,LaurH,ClosaJ,RosichB.Theenvisatadvancedsyntheticapertureradarsystem[C].2000.
    [39]BovensmannH,BurrowsJP,BuchwltzM,FrerickI,NolS,RozanovVV,ChanceKV,GoedeAPH.Sciamachy:Missionobjectivesandmeasurementmodes[J].JournaloftheAtmosphericSciences.1999,56:127-150.
    [40]张兴赢,张鹏,方宗义,邱红,李晓静,张艳.应用卫星遥感技术监测大气痕量气体的研究进展[J].气象.2007,33(007):3-14.
    [41]KrotkovNA,CarnSA,KruegerAJ,BhartiaPK,YangK.Bandresidualdifferencealgorithmforretrievalofso2fromtheauraozonemonitoringinstrument(omi)[J].IEEEtransactionsongeoscienceandremotesensing.2006,44(5):1259-1266.
    [42]冯砚青.中国酸雨状况和自然成因综述及防治对策探究[J].云南地理环境研究.2004,16(001):25-28.
    [43]杨国福.利用modis遥感技术监测浙江省森林火燃料湿度的时空动态[D]:浙江林学院;2009.
    [44]刘安兴,张正寿,丁冬良.浙江林业自然资源(森林卷).In:北京:中国农业科学技术出版社;2002.
    [45]ZhengGUO,JiangH,ChenJ,ChengM,WangB,JiangZ.Therelationshipbetweenatmosphericso2columndensityandlanduseinzhejiang,china[J].
    [46]童笑柳.浙江省情概览[J].资料通讯.2005,(001):15-20.
    [47]TorresO,DecaeR,VeefkindP,deLeeuwG.Omiaerosolretrievalalgorithm[J].OMIAlgorithmTheoreticalBasisDocument.2002,3:47–71.
    [48]AhmadSP,LeveltPF,BhartiaPK,HilsenrathE,LeppelmeierGW,JohnsonJE.Atmosphericproductsfromtheozonemonitoringinstrument(omi)[C]//.2003:619-630.
    [49]DiL,YangW,DengM,DengD,McDonaldK.Theprototypicalnasahdf-eoswebgissoftwaresuite(nwgiss)[C]//.2001.
    [50]潘虹梅,李凤全,王俊荆,曹志纯.基于API方法的城市大气污染评价[J].环境科学与管理.2008,33(002):178-180.
    [51]VogelmannJE,SohlT,HowardSM.Regionalcharacterizationoflandcoverusingmultiplesourcesofdata[J].PhotogrammetricEngineeringandRemoteSensing.1998,64(1):45-57.
    [52]HansenMC,DeFriesRS,TownshendJRG,SohlbergR.Globallandcoverclassificationat1kmspatialresolutionusingaclassificationtreeapproach[J].InternationalJournalofRemoteSensing.2000,21(6):1331-1364.
    [53]GuoZ,JiangH,ChenJ,ChengM,JiangZ.Themethodsresearchofderivingbambooinformationbasedonikonosimage[C]//.2009:74982D.
    [54]齐瑾.利用sciamachy/envisat资料开展中国区域NO2反演试验研究[D].北京:中国科学院;2007.
    [55]徐永明,刘勇洪,魏鸣,吕晶晶.基于modis数据的长江三角洲地区土地覆盖分类[J].地理学报.2007,62(006):640-648.
    [56]DeFriesRS,HansenM,TownshendJRG,SohlbergR.Globallandcoverclassificationsat8kmspatialresolution:Theuseoftrainingdataderivedfromlandsatimageryindecisiontreeclassifiers[J].InternationalJournalofRemoteSensing.1998,19(16):3141-3168.
    [57]DeFriesRS,ChanJCW.Multiplecriteriaforevaluatingmachinelearningalgorithmsforlandcoverclassificationfromsatellitedata[J].RemoteSensingofEnvironment.2000,74(3):503-515.
    [58]KloditzC,BoxtelA,CarfagnaE,DeursenW.Estimatingtheaccuracyofcoarsescaleclassificationusinghighscaleinformation[J].Photogrammetricengineeringandremotesensing.1998,64(2):127-132.
    [59]BolesSH,XiaoX,LiuJ,ZhangQ,MunkhtuyaS,ChenS,OjimaD.Landcovercharacterizationoftemperateeastasiausingmulti-temporalvegetationsensordata[J].RemoteSensingofEnvironment.2004,90(4):477-489.
    [60]WeatherheadEC,ReinselGC,CheangWK,TiaoGC,MengXL,ChoiD,KellerT,DeLuisiJ,WuebblesDJ,KerrJB.Factorsaffectingthedetectionoftrends-statisticalconsiderationsandapplicationstoenvironmentaldata[J].JournalofGeophysicalResearch.1998,103(D14):17,149-117,161.
    [61]朱珊.浙江省小城镇发展差异研究[D]:浙江大学;2005.
    [62]MartinRV,ChanceK,JacobDJ,KurosuTP,SpurrRJD,BucselaE,GleasonJF,PalmerPI,BeyI,FioreAM.Animprovedretrievaloftroposphericnitrogendioxidefromgome[J].J.Geophys.Res.2002,107(10.1029):9-1.
    [63]闫文德,田大伦,项文化,黄志宏.城市林地与非林地大气SO2季节动态变化[J].生态学报.2006,26(005):1367-1374.
    [64]魏可染.金昌市大气二氧化硫污染现状分析及控制对策研究[D]:兰州大学;2008.

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