四苯乙烯衍生物与大环主体在主客体相互作用下的聚集诱导发光
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摘要
具有聚集诱导发光性质化合物的发展不仅很大程度上解决了传统有机分子发色团在高浓度、固态或者薄膜等形式的聚集状态下荧光猝灭的问题,而且扩展了有机发色团在荧光探针、传感器以及细胞成像等方面的应用。其中,四苯乙烯及其衍生物作为具有聚集诱导发光性质的典型化合物已被广泛应用在材料化学、生物化学等相关研究领域。受此启发,超分子化学家也将这类具有聚集诱导发光性质的四苯乙烯及其衍生物作为研究对象引入到超分子化学的领域,特别是利用大环主体与四苯乙烯客体通过主客体相互作用有效地限制了荧光客体分子的分子内转动或运动,增强了这类超分子体系的发光强度,并为其在刺激响应性传感器、智能探针等方面提供了新思路。本文总结了近年来涉及四苯乙烯衍生物与大环主体通过主客体相互作用形成聚集诱导发光超分子体系的发展,并按照大环主体进行分类简要介绍其应用。
The compounds with aggregation-induced emission(AIE) property have been widely developed to solve aggregation-caused quenching(ACQ) problem of organic luminophores at high concentration, in the solid state, or in the form of thin film. Therefore, AIE compounds are useful for a number of applications, such as fluorescent probes and receptors, and cell imaging. Tetraphenylethene(TPE) and its derivatives, as typical compounds with AIE property, have been widely applied in materials chemistry, biochemistry, and other related fields. Inspired from AIE, TPE has been also introduced into the field of supramolecular chemistry by supramolecular chemists. Especially, given their ability to restrict the intramolecular rotation or motion of TPE molecules, macrocyclic hosts can form host-guest complexes or supramolecular polymers with TPE via host-guest interactions, which results in enhancement in the AIE effect of guests. Hence, AIE of TPE derivatives with macrocycles via host-guest interaction also provides a new approach to develop the applications in stimuli-responsive sensors and probes. This review mainly focuses on summarizing the research progress of host-guest complexes between macrocycles and TPE, and comments on the bright future of AIE behaviors of the supramolecular systems involving host-guest interactions.
The compounds with aggregation-induced emission(AIE) property have been widely developed to solve aggregation-caused quenching(ACQ) problem of organic luminophores at high concentration, in the solid state, or in the form of thin film. Therefore, AIE compounds are useful for a number of applications, such as fluorescent probes and receptors, and cell imaging. Tetraphenylethene(TPE) and its derivatives, as typical compounds with AIE property, have been widely applied in materials chemistry, biochemistry, and other related fields. Inspired from AIE, TPE has been also introduced into the field of supramolecular chemistry by supramolecular chemists. Especially, given their ability to restrict the intramolecular rotation or motion of TPE molecules, macrocyclic hosts can form host-guest complexes or supramolecular polymers with TPE via host-guest interactions, which results in enhancement in the AIE effect of guests. Hence, AIE of TPE derivatives with macrocycles via host-guest interaction also provides a new approach to develop the applications in stimuli-responsive sensors and probes. This review mainly focuses on summarizing the research progress of host-guest complexes between macrocycles and TPE, and comments on the bright future of AIE behaviors of the supramolecular systems involving host-guest interactions.
引文
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