液相中气泡上升行为与界面传质:实验研究与数值计算
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摘要
在工业生产过程中,气泡在液相中的上升行为及气液界面的传质行为极为常见。本文针对不同条件下气泡上升过程的实验研究方法以及数值计算方法进行了总结。从实验与数值计算的角度,综述了单气泡上升过程的影响因素、多气泡上升过程聚并与破裂的现象和机理以及工业装置中气液两相流型和气泡特性,并对传质模型进行了归纳,主要关注了气侧-界面传质模型的研究现状。综述结果表明:当前对于单气泡上升行为的研究较为充分,而对于多气泡的行为机理的研究尚需深入。此外,受到研究手段的限制,进行气侧-界面传质模型研究具有一定挑战性。针对当前的相关研究进展和存在的问题,对今后气泡上升行为和传质行为的研究提出以下建议,即开展气泡聚并与破裂可控性研究,强化对气侧-界面传质过程的研究,包括泡内流体行为可视化研究和相关传质模型的建立。
In the industrial processes,rising behavior of bubbles in the liquid and mass transfer on the gas-liquid interface are very common.In this paper,experimental methods and numerical simulation methods are summarized under different conditions.In terms of experiments and numerical simulations,impact factors of single bubble rising behavior,phenomenon and mechanism of coalescence and break up for multiple bubbles,bubble flow pattern and properties in industrial devices,and mass transfer model,especially for gas-interface mass transfer model,are summed up.The results show that the studies about single bubble behavior are sufficient while for the multiple bubbles,more works need to be done.Besides,it is challenging to establish gas-interface mass transfer model due to the limit of research tools.According to the relative research progress and problems,the following suggestions about the future research directions conducting controllability study of coalescence and break up for bubbles,and strengthening of research on gas-interface mass transfer including the research of visualization of the internal flow and convective mass transfer in bubbles.
In the industrial processes,rising behavior of bubbles in the liquid and mass transfer on the gas-liquid interface are very common.In this paper,experimental methods and numerical simulation methods are summarized under different conditions.In terms of experiments and numerical simulations,impact factors of single bubble rising behavior,phenomenon and mechanism of coalescence and break up for multiple bubbles,bubble flow pattern and properties in industrial devices,and mass transfer model,especially for gas-interface mass transfer model,are summed up.The results show that the studies about single bubble behavior are sufficient while for the multiple bubbles,more works need to be done.Besides,it is challenging to establish gas-interface mass transfer model due to the limit of research tools.According to the relative research progress and problems,the following suggestions about the future research directions conducting controllability study of coalescence and break up for bubbles,and strengthening of research on gas-interface mass transfer including the research of visualization of the internal flow and convective mass transfer in bubbles.
引文
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[8]邹晓燕,姚克俭.被动式DMFC阳极通道气泡行为的实验研究[J].化工进展, 2011, 30(7):1444-1449.ZOU Xiaoyan, YAO Kejian. Experimental investigation onbubbling behavior in anode channel of passive DMFC[J].Chemical Industry and Engineering Progress, 2011, 30(7):1444-1449.
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[12] SANADA T, SATO A, SHIROTA M, et al. Motion and coalescenceof a pair of bubbles rising side by side[J]. Chemical EngineeringScience, 2009, 64(11):2659-2671.
[13] LEGENDRE D, ZEVENHOVEN R. Detailed experimental studyon the dissolution of CO2and air bubbles rising in water[J].Chemical Engineering Science, 2017, 158:552-560.
[14] AOKI J, HAYASHI K, TOMIYAMA A. Mass transfer from singlecarbon dioxide bubbles in contaminated water in a vertical pipe[J].International Journal of Heat and Mass Transfer, 2015, 83:652-658.
[15] BOHM L, BREHMER M, KRAUME M. Comparison of the singlebubble ascent in a newtonian and a non-newtonian liquid:aphenomenological PIV study[J]. Chemie Ingenieur Technik, 2016,88(1/2):93-106.
[16] POURTOUSI M, GANESAN P, KAZEMZADEH A, et al. Methanebubble formation and dynamics in a rectangular bubble column:aCFD study[J]. Chemometrics and Intelligent Laboratory Systems,2015, 147:111-120.
[17]许联锋,陈刚,李建中,等.粒子图像测速技术研究进展[J].力学进展, 2003, 33(4):533-540.XU Lianfeng, CHEN Gang, LI Jianzhong, et al. Progress in theresearch of particle image velocimetry[J]. Advances in Mechanics,2003, 33(4):533-540.
[18] FUNFSCHILLING D, LI H Z. Flow of non-Newtonian fluidsaround bubbles:PIV measurements and birefringence visualisation[J]. Chemical Engineering Science, 2001, 56:1137-1141.
[19] SAITO T, TORIU M. Effects of a bubble and the surroundingliquid motions on the instantaneous mass transfer across the gas-liquid interface[J]. Chemical Engineering Journal, 2015, 265:164-175.
[20] HUANG J, SAITO T. Influences of gas-liquid interfacecontamination on bubble motions, bubble wakes, andinstantaneous mass transfer[J]. Chemical Engineering Science,2017, 157:182-199.
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