Fenton及类Fenton法氧化垃圾渗滤液研究进展
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摘要
综述了Fenton与类Fenton氧化垃圾渗滤液的研究进展。Fenton法对垃圾渗滤液中难去除有机物尤其是腐殖酸有良好的降解效果。引入光、电、微波、超声波等的类Fenton法减少了药剂用量,提升了去除效果,非均相Fenton实现了催化剂的循环使用。并对Fenton及类Fenton法处理垃圾渗滤液的研究方向进行了展望。
The research progress of Fenton and Fenton-like oxidized landfill leachate in recent years was reviewed. The Fenton method had a good degradation effect on refractory organic matter,especially humic acid, in landfill leachate. The Fenton-like method, which introduced light, electricity, microwave, ultrasonic, etc., reduced the amount of the agents and improved the removal effect. The heterogeneous Fenton realized the recycling of the catalyst. Finally, the research direction of Fenton and Fenton-like treatment of landfill leachate was prospected.
The research progress of Fenton and Fenton-like oxidized landfill leachate in recent years was reviewed. The Fenton method had a good degradation effect on refractory organic matter,especially humic acid, in landfill leachate. The Fenton-like method, which introduced light, electricity, microwave, ultrasonic, etc., reduced the amount of the agents and improved the removal effect. The heterogeneous Fenton realized the recycling of the catalyst. Finally, the research direction of Fenton and Fenton-like treatment of landfill leachate was prospected.
引文
[1] XU Y,XUE X,DONG L,et al.Long-term dynamics of leachate production,leakage from hazardous waste landfill sites and the impact on groundwater quality and human health[J].Waste Management,2018,82:156-166.
[2] BADERNA D,CALONI F,BENFENATI E. Investigating landfill leachate toxicity in vitro:A review of cell models and endpoints[J].Environment International,2019,122:21-30.
[3]王恒.电化学法处理垃圾渗沥液反渗透浓缩液的实验研究[D].青岛:青岛理工大学,2015.
[4]刘占孟,徐礼春,赵杰峰,等.新型高级氧化技术处理垃圾渗滤液的研究进展[J].水处理技术,2018,44(1):7-12+25.
[5] YANG D,JAMES D E.Treatment of landfill leachate by the Fenton process[J].Water Research,2006,40(20):3683-3694.
[6] UMAR M,AZIZ H A,YUSOFF M S. Trends in the use of Fenton,electro-Fenton and photo-Fenton for the treatment of landfill leachate[J].Waste Management,2010,30(11):2113-2121.
[7]刘静,王杰,孙金诚,等.Fenton及改进Fenton氧化处理难降解有机废水的研究进展[J].水处理技术,2015,41(2):6-10+16.
[8] SINGA P K,ISA M H,HO Y-C,et al.Treatment of hazardous waste landfill leachate using Fenton oxidation process[J].E3S Web of Conferences,2018,34:02034.
[9] SUBRAMANIAM R,GANG D D,NIE J,et al.Application of response surface methodology for optimization of treatment for an Aged Landfill leachate using Fenton's oxidation reagent[J].Environmental Engineering Science,2017,34(10):731-739.
[10] ROUDI A M,CHELLIAPAN S,WAN W H M,et al.Prediction and optimization of the Fenton process for the treatment of landfill leachate using an artificial neural network[J].Water,2018,10(5):595.
[11] HE R,TIAN B-H,ZHANG Q-Q,et al.Effect of Fenton oxidation on biodegradability,biotoxicity and dissolved organic matter distribution of concentrated landfill leachate derived from a membrane process[J].Waste Management,2015,38:232-239.
[12] JUNG C,DENG Y,ZHAO R,et al.Chemical oxidation for mitigation of UV-quenching substances(UVQS)from municipal landfill leachate:Fenton process versus ozonation[J].Water Research,2017,108:260-270.
[13] XU J,LONG Y,SHEN D,et al.Optimization of Fenton treatment process for degradation of refractory organics in pre-coagulated leachate membrane concentrates[J].Journal of Hazardous Materials,2017,323:674-680.
[14] AFTAB B,SHIN H-S,HUR J.Exploring the fate and oxidation behaviors of different organic constituents in landfill leachate upon Fenton oxidation processes using EEM-PARAFAC and2D-COS-FTIR[J].Journal of Hazardous Materials,2018,354:33-41.
[15]郑艳芬.改进的Fenton法处理难降解有机废水应用进展[J].中国环境管理干部学院学报,2017,27(3):78-81.
[16] POURAN S R,AZIZ A A,DAUD W M A W.Review on the main advances in photo-Fenton oxidation system for recalcitrant wastewaters[J].Journal of Industrial and Engineering Chemistry,2015,21:53-69.
[17] CLARIZIA L,RUSSO D,DI SOMMA I,et al.Homogeneous photo-Fenton processes at near neutral p H:a review[J].Applied Catalysis B:Environmental,2017,209:358-371.
[18] SEIBERT D,DIEL T,WELTER J B,et al. Performance of photo-Fenton process mediated by Fe(III)-carboxylate complexes applied to degradation of landfill leachate[J].Journal of Environmental Chemical Engineering,2017,5(5):4462-4470.
[19] LAK M G,SABOUR M R,GHAFARI E,et al.Energy consumption and relative efficiency improvement of Photo-Fenton Optimization by RSM for landfill leachate treatment,a case study[J].Waste Management,2018,79:58-70.
[20]赵庆良,黄慧彬,丁晶,等.电Fenton技术的研究现状及应用进展[J].工业水处理,2018,38(2):6-11.
[21] FERNANDES A,LABIADH L,CIR ACO L,et al.Electro-Fenton oxidation of reverse osmosis concentrate from sanitary landfill leachate:Evaluation of operational parameters[J].Chemosphere,2017,184:1223-1229.
[22] HU Y,LU Y,LIU G,et al.Effect of the structure of stacked electro-Fenton reactor on treating nanofiltration concentrate of landfill leachate[J].Chemosphere,2018,202:191-197.
[23] HASSAN M,POUS N,XIE B,et al.Influence of iron species on integrated microbial fuel cell and electro-Fenton process treating landfill leachate[J].Chemical Engineering Journal,2017,328:57-65.
[24] WANG D,HOU H,HU J,et al.A bio-electro-Fenton system with a facile anti-biofouling air cathode for efficient degradation of landfill leachate[J].Chemosphere,2019,215:173-181.
[25] TRIPATHY B K,KUMAR M.Suitability of microwave and microwave-coupled systems for landfill leachate treatment:an overview[J].Journal of Environmental Chemical Engineering,2017,5(6):6165-6178.
[26] ZHANG A,GU Z,CHEN W,et al.Removal of refractory organic pollutants in reverse-osmosis concentrated leachate by microwave Fenton process[J].Environmental Science and Pollution Research,2018,25(29):28907-28916.
[27]孙俊良.超声波处理对淀粉性质及其酶解产物分子特性的影响[J].河南科技学院学报(自然科学版),2010,38(2):81-86.
[28] BABUPONNUSAMI A,MUTHUKUMAR K.A review on Fenton and improvements to the Fenton process for wastewater treatment[J].Journal of Environmental Chemical Engineering,2014,2(1):557-572.
[29] JOSHI S M,GOGATE P R.Treatment of landfill leachate using different configurations of ultrasonic reactors combined with advanced oxidation processes[J].Separation and Purification Technology,2019,211:10-18.
[30] NIDHEESH P.Heterogeneous Fenton catalysts for the abatement of organic pollutants from aqueous solution:a review[J].Rsc Advances,2015,5(51):40552-40577.
[31] SRUTHI T,GANDHIMATHI R,RAMESH S,et al.Stabilized landfill leachate treatment using heterogeneous Fenton and electro-Fenton processes[J].Chemosphere,2018,210:38-43.
[32] KIM D-G,KO S-O.Cu@Fe3O4core-shell nanoparticle-catalyzed oxidative degradation of the antibiotic oxytetracycline in pretreated landfill leachate[J].Chemosphere,2018,191:639-650.
[33] MA C,HE Z,JIA S,et al.Treatment of stabilized landfill leachate by Fenton-like process using Fe3O4particles decorated Zr-pillared bentonite[J].Ecotoxicology and Environmental Safety,2018,161:489-496.
[34] ZHA F,YAO D,HU Y,et al.Integration of US/Fe2+and photoFenton in sequencing for degradation of landfill leachate[J].Water Science and Technology,2016,73(2):260-266.
[35] ASAITHAMBI P,BEYENE D,ALEMAYEHU E.Treatment of landfill leachate waste using sono(US)and photo(UV)based advanced oxidation processes:Studies on various operating parameters[J].Deslination and Water Treatment,2017,94:147-155.
[36] BAIJU A,GANDHIMATHI R,RAMESH S,et al.Combined heterogeneous Electro-Fenton and biological process for the treatment of stabilized landfill leachate[J].Journal of Environmental Management,2018,210:328-337.
[37] WANG Z,LI J,TAN W,et al.Removal of COD from landfill leachate by advanced Fenton process combined with electrolysis[J].Separation and Purification Technology,2019,208:3-11.
[38] CHEN W,ZHANG A,GU Z,et al.Enhanced degradation of refractory organics in concentrated landfill leachate by Fe0/H2O2coupled with microwave irradiation[J].Chemical Engineering Journal,2018,354:680-691.
[2] BADERNA D,CALONI F,BENFENATI E. Investigating landfill leachate toxicity in vitro:A review of cell models and endpoints[J].Environment International,2019,122:21-30.
[3]王恒.电化学法处理垃圾渗沥液反渗透浓缩液的实验研究[D].青岛:青岛理工大学,2015.
[4]刘占孟,徐礼春,赵杰峰,等.新型高级氧化技术处理垃圾渗滤液的研究进展[J].水处理技术,2018,44(1):7-12+25.
[5] YANG D,JAMES D E.Treatment of landfill leachate by the Fenton process[J].Water Research,2006,40(20):3683-3694.
[6] UMAR M,AZIZ H A,YUSOFF M S. Trends in the use of Fenton,electro-Fenton and photo-Fenton for the treatment of landfill leachate[J].Waste Management,2010,30(11):2113-2121.
[7]刘静,王杰,孙金诚,等.Fenton及改进Fenton氧化处理难降解有机废水的研究进展[J].水处理技术,2015,41(2):6-10+16.
[8] SINGA P K,ISA M H,HO Y-C,et al.Treatment of hazardous waste landfill leachate using Fenton oxidation process[J].E3S Web of Conferences,2018,34:02034.
[9] SUBRAMANIAM R,GANG D D,NIE J,et al.Application of response surface methodology for optimization of treatment for an Aged Landfill leachate using Fenton's oxidation reagent[J].Environmental Engineering Science,2017,34(10):731-739.
[10] ROUDI A M,CHELLIAPAN S,WAN W H M,et al.Prediction and optimization of the Fenton process for the treatment of landfill leachate using an artificial neural network[J].Water,2018,10(5):595.
[11] HE R,TIAN B-H,ZHANG Q-Q,et al.Effect of Fenton oxidation on biodegradability,biotoxicity and dissolved organic matter distribution of concentrated landfill leachate derived from a membrane process[J].Waste Management,2015,38:232-239.
[12] JUNG C,DENG Y,ZHAO R,et al.Chemical oxidation for mitigation of UV-quenching substances(UVQS)from municipal landfill leachate:Fenton process versus ozonation[J].Water Research,2017,108:260-270.
[13] XU J,LONG Y,SHEN D,et al.Optimization of Fenton treatment process for degradation of refractory organics in pre-coagulated leachate membrane concentrates[J].Journal of Hazardous Materials,2017,323:674-680.
[14] AFTAB B,SHIN H-S,HUR J.Exploring the fate and oxidation behaviors of different organic constituents in landfill leachate upon Fenton oxidation processes using EEM-PARAFAC and2D-COS-FTIR[J].Journal of Hazardous Materials,2018,354:33-41.
[15]郑艳芬.改进的Fenton法处理难降解有机废水应用进展[J].中国环境管理干部学院学报,2017,27(3):78-81.
[16] POURAN S R,AZIZ A A,DAUD W M A W.Review on the main advances in photo-Fenton oxidation system for recalcitrant wastewaters[J].Journal of Industrial and Engineering Chemistry,2015,21:53-69.
[17] CLARIZIA L,RUSSO D,DI SOMMA I,et al.Homogeneous photo-Fenton processes at near neutral p H:a review[J].Applied Catalysis B:Environmental,2017,209:358-371.
[18] SEIBERT D,DIEL T,WELTER J B,et al. Performance of photo-Fenton process mediated by Fe(III)-carboxylate complexes applied to degradation of landfill leachate[J].Journal of Environmental Chemical Engineering,2017,5(5):4462-4470.
[19] LAK M G,SABOUR M R,GHAFARI E,et al.Energy consumption and relative efficiency improvement of Photo-Fenton Optimization by RSM for landfill leachate treatment,a case study[J].Waste Management,2018,79:58-70.
[20]赵庆良,黄慧彬,丁晶,等.电Fenton技术的研究现状及应用进展[J].工业水处理,2018,38(2):6-11.
[21] FERNANDES A,LABIADH L,CIR ACO L,et al.Electro-Fenton oxidation of reverse osmosis concentrate from sanitary landfill leachate:Evaluation of operational parameters[J].Chemosphere,2017,184:1223-1229.
[22] HU Y,LU Y,LIU G,et al.Effect of the structure of stacked electro-Fenton reactor on treating nanofiltration concentrate of landfill leachate[J].Chemosphere,2018,202:191-197.
[23] HASSAN M,POUS N,XIE B,et al.Influence of iron species on integrated microbial fuel cell and electro-Fenton process treating landfill leachate[J].Chemical Engineering Journal,2017,328:57-65.
[24] WANG D,HOU H,HU J,et al.A bio-electro-Fenton system with a facile anti-biofouling air cathode for efficient degradation of landfill leachate[J].Chemosphere,2019,215:173-181.
[25] TRIPATHY B K,KUMAR M.Suitability of microwave and microwave-coupled systems for landfill leachate treatment:an overview[J].Journal of Environmental Chemical Engineering,2017,5(6):6165-6178.
[26] ZHANG A,GU Z,CHEN W,et al.Removal of refractory organic pollutants in reverse-osmosis concentrated leachate by microwave Fenton process[J].Environmental Science and Pollution Research,2018,25(29):28907-28916.
[27]孙俊良.超声波处理对淀粉性质及其酶解产物分子特性的影响[J].河南科技学院学报(自然科学版),2010,38(2):81-86.
[28] BABUPONNUSAMI A,MUTHUKUMAR K.A review on Fenton and improvements to the Fenton process for wastewater treatment[J].Journal of Environmental Chemical Engineering,2014,2(1):557-572.
[29] JOSHI S M,GOGATE P R.Treatment of landfill leachate using different configurations of ultrasonic reactors combined with advanced oxidation processes[J].Separation and Purification Technology,2019,211:10-18.
[30] NIDHEESH P.Heterogeneous Fenton catalysts for the abatement of organic pollutants from aqueous solution:a review[J].Rsc Advances,2015,5(51):40552-40577.
[31] SRUTHI T,GANDHIMATHI R,RAMESH S,et al.Stabilized landfill leachate treatment using heterogeneous Fenton and electro-Fenton processes[J].Chemosphere,2018,210:38-43.
[32] KIM D-G,KO S-O.Cu@Fe3O4core-shell nanoparticle-catalyzed oxidative degradation of the antibiotic oxytetracycline in pretreated landfill leachate[J].Chemosphere,2018,191:639-650.
[33] MA C,HE Z,JIA S,et al.Treatment of stabilized landfill leachate by Fenton-like process using Fe3O4particles decorated Zr-pillared bentonite[J].Ecotoxicology and Environmental Safety,2018,161:489-496.
[34] ZHA F,YAO D,HU Y,et al.Integration of US/Fe2+and photoFenton in sequencing for degradation of landfill leachate[J].Water Science and Technology,2016,73(2):260-266.
[35] ASAITHAMBI P,BEYENE D,ALEMAYEHU E.Treatment of landfill leachate waste using sono(US)and photo(UV)based advanced oxidation processes:Studies on various operating parameters[J].Deslination and Water Treatment,2017,94:147-155.
[36] BAIJU A,GANDHIMATHI R,RAMESH S,et al.Combined heterogeneous Electro-Fenton and biological process for the treatment of stabilized landfill leachate[J].Journal of Environmental Management,2018,210:328-337.
[37] WANG Z,LI J,TAN W,et al.Removal of COD from landfill leachate by advanced Fenton process combined with electrolysis[J].Separation and Purification Technology,2019,208:3-11.
[38] CHEN W,ZHANG A,GU Z,et al.Enhanced degradation of refractory organics in concentrated landfill leachate by Fe0/H2O2coupled with microwave irradiation[J].Chemical Engineering Journal,2018,354:680-691.