季铵化木质素与纳米二氧化钛协同稳定的双重pH响应性Pickering乳液
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摘要
利用季铵化木质素与TiO2纳米颗粒复合作为乳化剂,以正癸烷为油相,制备具有pH响应性的O/W型Pickering乳液.该乳液在6.0 pH-Responsive oil-in-water Pickering emulsions using n-decane as oil phase were prepared by mixing quaternized lignin(QAL)and titanium dioxidenanoparticles as emulsifiers.The emulsions stabilized by 0.5 wt%TiO_2 neat nanoparticles are extremely unstable due to the strong hydrophilic properties of the nanoparticles.However,when TiO_2 nanoparticles are dispersed in neutral solution containing 0.1 wt%QAL,all the emulsifier particles can be applied onto the n-decane/water interface,which greatly improves the stability of the emulsions and the droplet size ranges from 20μm to 60μm.Meanwhile,emulsions stabilized by QAL and TiO_2 nanoparticles show outstanding pH-responsive properties,which are stable in the range of 6.0
引文
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22Li S,Li Z,Zhang Y,Liu C,Yu G,Li B,Mu X,Peng H.ACS Sustain Chem Eng,2017,5(5):4214-4222
23Zhou Mingsong(周明松),Xu Ruilin(许锐林),Wang Wenli(王文利),Pang Yuxia(庞煜霞),Qiu Xueqing(邱学青).Acta Polymerica Sinica(高分子学报),2015,(12):1414-1420
24Yi H,Yang Y,Gu X,Huang J,Wang C.J Mater Chem A,2015,3(26):13749-13757
25Silmore K S,Gupta C,Washburn N R.J Colloid Interface Sci,2016,466:91-100
26Wei Z,Yang Y,Yang R,Wang C.Green Chem,2012,14(11):3230-3236
27Qian Y,Zhang Q,Qiu X,Zhu S.Green Chem,2014,16(12):4963-4968
28Li Yuanyuan(李圆圆),Yang Dongjie(杨东杰),Qiu Xueqing(邱学青).Chemical Journal of Chinese Universities(高等学校化学学报),2017,38(5):880-887
29Li Y,Qiu X,Qian Y,Xiong W,Yang D.Chem Eng J,2017,327:1176-1183
30Cai C,Zhan X,Zeng M,Lou H,Pang Y,Yang J,Yang D,Qiu X.Green Chem,2017,19(22):5479-5487
31Ye F,Miao M,Jiang B,Campanella O H,Jin Z,Zhang T.Food Chem,2017,229:152-8
32Lu J,Zhou W,Chen J,Jin Y,Walters K B,Ding S.RSC Adv,2015,5(13):9416-9424
33Yi C,Yang Y,Zhu Y,Liu N,Liu X,Luo J,Jiang M.Langmuir,2012,28(25):9211-9222
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36Nowotny M K,Sheppard L R,Bak T,Nowotny J.J Phys Chem C,2008,112(14):5275-5300
37González E,Bonnefond A,Barrado M,Casado Barrasa A M,Asua J M,Leiza J R.Chem Eng J,2015,281:209-217
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39Hao Y,Liu Y,Yang R,Zhang X,Liu J,Yang H.Chinese Chem Lett,2018,29(6):778-782
40Chen Y,Li W,Zhang X.Colloid J,2011,73(2):267-274
41Yang Dongjie(杨东杰),Bai Mengxian(白孟仙),Hu Wenli(胡文莉),Yan Mingfang(严明芳),Qiu Xueqing(邱学青).Journal of Chemical Engineering of Chinese Universities(高校化学工程学报),2012,(5):748-754
42Yang Dongjie(杨东杰),Guo Wenyuan(郭闻源),Zen Weimei(曾伟媚),Qiu Xueqing(邱学青).Acta Polymerica Sinica(高分子学报),2014,(3):333-340