聚乙烯醇与纳米抗菌材料的复合研究进展
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摘要
对聚乙烯醇(PVA)与纳米抗菌材料的复合工艺及研究现状进行综述。通过收集文献,以近几年来国内外学者对PVA与纳米抗菌材料复合的研究论文作为依据,对其复合工艺及研究中难点进行分析和总结,综述PVA与多种不同纳米抗菌材料的复合工艺、实验结果及应用。对PVA与不同的纳米抗菌材料的复合研究结果总结发现,PVA易与其他纳米抗菌颗粒复合形成纳米复合薄膜从而赋予其抗菌性能,同时改善纯PVA膜的水溶性,提高其机械性能。PVA与纳米抗菌材料形成的复合膜具有优异的抑菌性,现已被广泛应用于食品保鲜和医药等方面。
Reviewed the research progress in nano-antibacterial materials loaded on polyvinyl alcohol( PVA) composite. According to the collection of literatures,the research papers of domestic and foreign scholars on the composites of PVA and nano antibacterial materials in recent years were taken as the basis.The compound technology and research key point were analyzed and summarized. It reviewed the compound technology,experimental results and application of PVA and nano antibacterial materials. The composite research results of PVA and different nano-antibacterial materials were summarized and found that the nanocomposite films could enhance the anti-bacterial property of the composites and improve the water solubility and mechanical properties. This form of PVA with nano-antibacterial composite films could gain excellent antimicrobial activity and have been extensively used in medical and food fresh keeping.
Reviewed the research progress in nano-antibacterial materials loaded on polyvinyl alcohol( PVA) composite. According to the collection of literatures,the research papers of domestic and foreign scholars on the composites of PVA and nano antibacterial materials in recent years were taken as the basis.The compound technology and research key point were analyzed and summarized. It reviewed the compound technology,experimental results and application of PVA and nano antibacterial materials. The composite research results of PVA and different nano-antibacterial materials were summarized and found that the nanocomposite films could enhance the anti-bacterial property of the composites and improve the water solubility and mechanical properties. This form of PVA with nano-antibacterial composite films could gain excellent antimicrobial activity and have been extensively used in medical and food fresh keeping.
引文
[1]李少香,雷芸娜,王佳平.聚乙烯醇膜的研究进展[J].涂层与防护,2018,39(8):44-48.
[2]杜运鹏.纳米改性聚乙烯醇(PVA)抗氧复合包装薄膜的制备及对鲜切山药保鲜的应用[D].上海:上海海洋大学,2017.
[3]范方方,刘琨.膨润土/壳聚糖/PVA保鲜膜对芒果保鲜效果的影响[J].食品科技,2017,42(3):54-59.
[4]LIU B,XU H,ZHAO H,et al.Preparation and characterization of intelligent starch/PVA films for simultaneous colorimetric indication and antimicrobial activity for food packaging applications[J].Carbohydr Polym,2017,157:842-849.
[5]LIU H Q,ZHANG G Z,LI H J.Preparation and properties of GO-PVA composite hydrogel with oriented structure[C]//Advances in Materials,Machinery,Electronics(AMME 2017).Penang,Malaysia,2017,1808:030009.
[6]晓铭.国内外聚乙烯醇的供需现状及未来发展趋势[J].乙醛醋酸化工,2018(3):4-7.
[7]THONG C C,TEO D C L,NG C K.Application of polyvinyl alcohol(PVA)in cement-based composite materials:A review of its engineering properties and microstructure behavior[J].Constr Build Mater,2016,107(6):172-180.
[8]MAJD S A,KHORASGANI M R,MOSHTAGHIAN S J,et al.Application of chitosan/PVA nano fiber as a potential wound dressing for streptozotocin-induced diabetic rats[J].Int J Biol Macromol,2016,92(11):1162-1168.
[9]ARUNKUMAR T,MURUGESAN D,RAJ K,et al.Effect of nano-coated Cu O absorbers with PVA sponges in solar water desalting system[J].Appl Therm Eng,2018,148(10):1416-1424.
[10]张群.载Zn O纳米纤维复合膜的制备及其抗菌性能的研究[D].合肥:安徽农业大学,2012.
[11]张志杰.PVA基纳米Ag复合静电纺丝纤维的制备及抗菌性能研究[D].开封:河南大学,2017.
[12]蔡晴,隋刚,于运花,等.功能性纳米纤维的静电纺丝制备及其生物医学应用研究[J].高分子通报,2013(4):18-35.
[13]王雪芳,王鸿博,傅佳佳,等.Ti O2/聚乳酸复合纳米纤维膜对草莓保鲜效果的研究[J].食品工业科技,2014,35(20):366-368.
[14]SARWAR M S,MBK N,JAHAN Z,et al.Preparation and characterization of PVA/nanocellulose/Ag nanocomposite films for antimicrobial food packaging[J].Carbohydr Polym,2018,184(24):453-464.
[15]封强锁.PAAm/PVA互穿网络水凝胶的制备及Cu纳米粒子的组装[D].西安:陕西师范大学,2012.
[16]SWAROOP K,FRANCIS S,SOMASHEKARAPPA H M.Gamma irradiation synthesis of Ag/PVA hydrogels and its antibacterial activity[J].Mater Today Proc,2016,3(6):1792-1798.
[17]曾晓峰.含纳米银的壳聚糖/聚乙烯醇敷料的研究[D].广州:华南理工大学,2011.
[18]何晓伟.Ag/PVA纳米复合纤维膜的制备及抗菌性能研究[D].郑州:中原工学院,2011.
[19]FRAGAL V H,CELLET T S,PEREIRA G M,et al.Covalently-layers of PVA and PAA and in situ formed Ag nanoparticles as versatile antimicrobial surfaces[J].Int J Biol Macromol,2016,91(10):329-337.
[20]LEE K S,KIM C H,JEONG S W,et al.Ultrasonic fabrication of flexible antibacterial Zn O nanopillar array film[J].Colloids Surf B,2018,170(10):172-178.
[21]SHAFIE Z M H M,AHMAD A L.Juxtaposition of PESbased hollow fiber membrane:Antifouling and antibacterial potential of Li Cl mediated PVA-Zn O blend[J].J Ind Eng Chem,2018,62(12):273-283.
[22]HAMZA A M,ALHTHEAL E D,SHAKIR A K.Enhancement the efficiency of Zn O nanofiber mats antibacterial using novel PVA/Ag nanoparticles[J].Energy Procedia,2017,119(8):615-621.
[23]SHALUMON K T,ANULEKHA K H,NAIR S V,et al.Sodium alginate/poly(vinyl alcohol)/nano Zn O composite nanofibers for antibacterial wound dressings[J].Int J Biol Macromol,2011,49(3):247-254.
[24]XU J,ZHANG Y,GUTHA Y,et al.Antibacterial property and biocompatibility of chtosan/poly(vinyl alcohol)/Zn O(CS/PVA/Zn O)beads as an efficient adsorbent for Cu(II)removal from aqueous solution[J].Colloids Surf B,2017,156(8):340-348.
[25]ZHANG L L,BAI H,LIU L,et al.Dimension induced intrinsic physio-electrical effects of nanostructured Ti O2on its antibacterial properties[J].Chem Eng J,2018,334(1):1309-1315.
[26]LEONG H J,OH S G.Preparation of antibacterial Ti O2,particles by hybridization with azelaic acid for applications in cosmetics[J].J Ind Eng Chem,2018,18(66):242-247.
[27]唐艳军,刘晓峰,夏军,等.Ti O2/壳聚糖纳米复合涂料制备及其在抗菌纸中的应用[J].功能材料,2012,43(17):2416-2420.
[28]张浩,袁军座.用于光催化抗菌涂料的纳米Ti O2的制备及改性方法[J].材料保护,2013,46(4):44-47.
[29]龙门,马磊,宋野,等.纳米Fe3+/Ti O2改性聚乙烯醇基紫胶复合膜对鸡蛋的保鲜效果[J].农业工程学报,2014,30(20):313-324.
[30]王志栋.聚乙烯醇/蒙脱土/二氧化钛复合薄膜的研究[D].青岛:青岛科技大学,2007.
[31]DHANASEKAR M,JENEFER V,NAMBIAR R B,et al.Ambient light antimicrobial activity of reduced graphene oxide supported metal doped Ti O2nanoparticles and their PVA based polymer nanocomposite films[J].Mater Res Bull,2018,97(8):238-243.
[32]潘晓勇,杜岩岩,陈伟,等.载银纳米二氧化钛在抗菌塑料中的应用研究进展[J].工程塑料应用,2012,40(11):101-105.
[33]LIAN Z,ZHANG Y,ZHAO Y.Nano-Ti O2particles and high hydrostatic pressure treatment for improving functionality of polyvinyl alcohol and chitosan composite films and nano-Ti O2migration from film matrix in food simulants[J].Innov Food Sci Emerg Technol,2016,33(3):145-153.
[34]LIN D,HUANG Y,LIU Y,et al.Physico-mechanical and structural characteristics of starch/polyvinyl alcohol/nano-titania photocatalytic antimicrobial composite films[J].Food Sci Technol,2018,96(10):704-712.
[35]王晓丹.聚乙烯醇/功能化氧化石墨烯纳米复合材料的制备及其性能研究[D].南京:南京师范大学,2011.
[36]胡承功,王孙琳,徐珍珍.PVA-Cu(Ⅱ)、PVA-Hg(Ⅱ)配合物功能纤维的制备及抗菌性能研究[J].化工新型材料,2017(3):184-185.
[37]雷艳雄.PVA基复合包装材料纳米Si O2改性及其对咸鸭蛋保鲜效果的影响[D].南京:南京农业大学,2011.
[38]尹月玲.PVA基复合材料纳米Si O2改性及对松花蛋涂膜保鲜包装效能影响的研究[D].南京:南京农业大学,2011.
[39]EWALDZ E,PATEL R,BANERJEE M,et al.Material selection in electrospinning microparticles[J].Polymer,2018,153(16):529-537.
[40]POORMOHAMMADIAN S J,DARVISHI P,DEZFULI AM G.Investigating the structural effect of electrospun nanofibrous polymeric films on water vapor transmission[J].Chin J Chem Eng,2018,(4):2-10.
[41]GUEL M L,JIMENEZ L D,HERNáNDEZ D A.Ultrasound-assisted sol-gel synthesis of Zr O2[J].Ultrason Sonochem,2017,35(6):514-517.
[42]NAJAFI A,GOLESTANI-FARD F,REZAIE H R.Sol-gel synthesis and characterization of B4C nanopowder[J].Ceram Int,2018,44(17):21386-21394.
[2]杜运鹏.纳米改性聚乙烯醇(PVA)抗氧复合包装薄膜的制备及对鲜切山药保鲜的应用[D].上海:上海海洋大学,2017.
[3]范方方,刘琨.膨润土/壳聚糖/PVA保鲜膜对芒果保鲜效果的影响[J].食品科技,2017,42(3):54-59.
[4]LIU B,XU H,ZHAO H,et al.Preparation and characterization of intelligent starch/PVA films for simultaneous colorimetric indication and antimicrobial activity for food packaging applications[J].Carbohydr Polym,2017,157:842-849.
[5]LIU H Q,ZHANG G Z,LI H J.Preparation and properties of GO-PVA composite hydrogel with oriented structure[C]//Advances in Materials,Machinery,Electronics(AMME 2017).Penang,Malaysia,2017,1808:030009.
[6]晓铭.国内外聚乙烯醇的供需现状及未来发展趋势[J].乙醛醋酸化工,2018(3):4-7.
[7]THONG C C,TEO D C L,NG C K.Application of polyvinyl alcohol(PVA)in cement-based composite materials:A review of its engineering properties and microstructure behavior[J].Constr Build Mater,2016,107(6):172-180.
[8]MAJD S A,KHORASGANI M R,MOSHTAGHIAN S J,et al.Application of chitosan/PVA nano fiber as a potential wound dressing for streptozotocin-induced diabetic rats[J].Int J Biol Macromol,2016,92(11):1162-1168.
[9]ARUNKUMAR T,MURUGESAN D,RAJ K,et al.Effect of nano-coated Cu O absorbers with PVA sponges in solar water desalting system[J].Appl Therm Eng,2018,148(10):1416-1424.
[10]张群.载Zn O纳米纤维复合膜的制备及其抗菌性能的研究[D].合肥:安徽农业大学,2012.
[11]张志杰.PVA基纳米Ag复合静电纺丝纤维的制备及抗菌性能研究[D].开封:河南大学,2017.
[12]蔡晴,隋刚,于运花,等.功能性纳米纤维的静电纺丝制备及其生物医学应用研究[J].高分子通报,2013(4):18-35.
[13]王雪芳,王鸿博,傅佳佳,等.Ti O2/聚乳酸复合纳米纤维膜对草莓保鲜效果的研究[J].食品工业科技,2014,35(20):366-368.
[14]SARWAR M S,MBK N,JAHAN Z,et al.Preparation and characterization of PVA/nanocellulose/Ag nanocomposite films for antimicrobial food packaging[J].Carbohydr Polym,2018,184(24):453-464.
[15]封强锁.PAAm/PVA互穿网络水凝胶的制备及Cu纳米粒子的组装[D].西安:陕西师范大学,2012.
[16]SWAROOP K,FRANCIS S,SOMASHEKARAPPA H M.Gamma irradiation synthesis of Ag/PVA hydrogels and its antibacterial activity[J].Mater Today Proc,2016,3(6):1792-1798.
[17]曾晓峰.含纳米银的壳聚糖/聚乙烯醇敷料的研究[D].广州:华南理工大学,2011.
[18]何晓伟.Ag/PVA纳米复合纤维膜的制备及抗菌性能研究[D].郑州:中原工学院,2011.
[19]FRAGAL V H,CELLET T S,PEREIRA G M,et al.Covalently-layers of PVA and PAA and in situ formed Ag nanoparticles as versatile antimicrobial surfaces[J].Int J Biol Macromol,2016,91(10):329-337.
[20]LEE K S,KIM C H,JEONG S W,et al.Ultrasonic fabrication of flexible antibacterial Zn O nanopillar array film[J].Colloids Surf B,2018,170(10):172-178.
[21]SHAFIE Z M H M,AHMAD A L.Juxtaposition of PESbased hollow fiber membrane:Antifouling and antibacterial potential of Li Cl mediated PVA-Zn O blend[J].J Ind Eng Chem,2018,62(12):273-283.
[22]HAMZA A M,ALHTHEAL E D,SHAKIR A K.Enhancement the efficiency of Zn O nanofiber mats antibacterial using novel PVA/Ag nanoparticles[J].Energy Procedia,2017,119(8):615-621.
[23]SHALUMON K T,ANULEKHA K H,NAIR S V,et al.Sodium alginate/poly(vinyl alcohol)/nano Zn O composite nanofibers for antibacterial wound dressings[J].Int J Biol Macromol,2011,49(3):247-254.
[24]XU J,ZHANG Y,GUTHA Y,et al.Antibacterial property and biocompatibility of chtosan/poly(vinyl alcohol)/Zn O(CS/PVA/Zn O)beads as an efficient adsorbent for Cu(II)removal from aqueous solution[J].Colloids Surf B,2017,156(8):340-348.
[25]ZHANG L L,BAI H,LIU L,et al.Dimension induced intrinsic physio-electrical effects of nanostructured Ti O2on its antibacterial properties[J].Chem Eng J,2018,334(1):1309-1315.
[26]LEONG H J,OH S G.Preparation of antibacterial Ti O2,particles by hybridization with azelaic acid for applications in cosmetics[J].J Ind Eng Chem,2018,18(66):242-247.
[27]唐艳军,刘晓峰,夏军,等.Ti O2/壳聚糖纳米复合涂料制备及其在抗菌纸中的应用[J].功能材料,2012,43(17):2416-2420.
[28]张浩,袁军座.用于光催化抗菌涂料的纳米Ti O2的制备及改性方法[J].材料保护,2013,46(4):44-47.
[29]龙门,马磊,宋野,等.纳米Fe3+/Ti O2改性聚乙烯醇基紫胶复合膜对鸡蛋的保鲜效果[J].农业工程学报,2014,30(20):313-324.
[30]王志栋.聚乙烯醇/蒙脱土/二氧化钛复合薄膜的研究[D].青岛:青岛科技大学,2007.
[31]DHANASEKAR M,JENEFER V,NAMBIAR R B,et al.Ambient light antimicrobial activity of reduced graphene oxide supported metal doped Ti O2nanoparticles and their PVA based polymer nanocomposite films[J].Mater Res Bull,2018,97(8):238-243.
[32]潘晓勇,杜岩岩,陈伟,等.载银纳米二氧化钛在抗菌塑料中的应用研究进展[J].工程塑料应用,2012,40(11):101-105.
[33]LIAN Z,ZHANG Y,ZHAO Y.Nano-Ti O2particles and high hydrostatic pressure treatment for improving functionality of polyvinyl alcohol and chitosan composite films and nano-Ti O2migration from film matrix in food simulants[J].Innov Food Sci Emerg Technol,2016,33(3):145-153.
[34]LIN D,HUANG Y,LIU Y,et al.Physico-mechanical and structural characteristics of starch/polyvinyl alcohol/nano-titania photocatalytic antimicrobial composite films[J].Food Sci Technol,2018,96(10):704-712.
[35]王晓丹.聚乙烯醇/功能化氧化石墨烯纳米复合材料的制备及其性能研究[D].南京:南京师范大学,2011.
[36]胡承功,王孙琳,徐珍珍.PVA-Cu(Ⅱ)、PVA-Hg(Ⅱ)配合物功能纤维的制备及抗菌性能研究[J].化工新型材料,2017(3):184-185.
[37]雷艳雄.PVA基复合包装材料纳米Si O2改性及其对咸鸭蛋保鲜效果的影响[D].南京:南京农业大学,2011.
[38]尹月玲.PVA基复合材料纳米Si O2改性及对松花蛋涂膜保鲜包装效能影响的研究[D].南京:南京农业大学,2011.
[39]EWALDZ E,PATEL R,BANERJEE M,et al.Material selection in electrospinning microparticles[J].Polymer,2018,153(16):529-537.
[40]POORMOHAMMADIAN S J,DARVISHI P,DEZFULI AM G.Investigating the structural effect of electrospun nanofibrous polymeric films on water vapor transmission[J].Chin J Chem Eng,2018,(4):2-10.
[41]GUEL M L,JIMENEZ L D,HERNáNDEZ D A.Ultrasound-assisted sol-gel synthesis of Zr O2[J].Ultrason Sonochem,2017,35(6):514-517.
[42]NAJAFI A,GOLESTANI-FARD F,REZAIE H R.Sol-gel synthesis and characterization of B4C nanopowder[J].Ceram Int,2018,44(17):21386-21394.