Novel FeMnCoCrAl high entropy alloy family is introduced for the first time.
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Single BCC phase solid solution form at equiatomic and non-equiatomic compositions.
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Ab-initio predictions of BCC phase stability agree with experiments.
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Equiatomic thin film and as-cast bulk HEA exhibit similar structure and properties.
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Combinatorial alloy design approach would enable accelerated exploration of HEAs.
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