Photocatalytic hydrogen evolution by iridium(III)-rhodium(III) system: Effect of the free ligand addition

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Photocatalytic hydrogen evolution by iridium(III)-rhodium(III) system: Effect of the free ligand addition

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作者：D.B. Vasilchenko^a ; ^c ; S.V. Tkachev^a ; A. Yu. Kurenkova^b ; ^c ; E.A. Kozlova^b ; ^c ; ^{kozlova@catalysis.ru" class="auth_mail" title="E-mail the corresponding author} ; D.V. Kozlov^b ; ^c
关键词：Catalyst design ; Hydrogen evolution ; Rhodium ; Iridium ; Pyridine derivatives
刊名：International Journal of Hydrogen Energy
出版年：2016
出版时间：30 January 2016
年：2016
卷：41
期：4
页码：2592-2597
全文大小：583 K

文摘

•: New homogeneous Rh–Ir systems are efficient for photohydrogen production.
•: Prolonged irradiation causes reduction of Rh to metal state and low activity.
•: Addition of free ligands stabilizes system from decomposition.
•: Quantum yield of 80% achieved by the stabilized systems.

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