Thermodynamic and mass transfer modeling of carbon dioxide absorption into aqueous 2-piperidineethanol

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Thermodynamic and mass transfer modeling of carbon dioxide absorption into aqueous 2-piperidineethanol

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作者：Brent J. Sherman^a ; ^{brentjsherman@utexas.edu" class="auth_mail" title="E-mail the corresponding author} ; Arlinda F. Ciftja^b ; Gary T. Rochelle^a ; ^{gtr@che.utexas.edu" class="auth_mail" title="E-mail the corresponding author}
关键词：Separations ; CO2 capture ; eNRTL ; Wetted-wall column ; Hindered amine ; Carbamate stability
刊名：Chemical Engineering Science
出版年：2016
出版时间：22 October 2016
年：2016
卷：153
期：Complete
页码：295-307
全文大小：2381 K

文摘

•: Liquid film mass transfer coefficient is most sensitive to the carbamate reaction.
•: Carbamate reaction rate follows same trend as unhindered amines.
•: 2PE forms a more stable carbamate than AMP.
•: Bicarbonate reaction rate is ten times faster than for an analogous tertiary amine.
•: The PFO assumption applies at low temperature, lean loading conditions.

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