Transition metal-modified mesoporous Mg-Al mixed oxides: Stable base catalysts for the synthesis of diethyl carbonate from ethyl carbamate and ethanol

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Transition metal-modified mesoporous Mg-Al mixed oxides: Stable base catalysts for the synthesis of diethyl carbonate from ethyl carbamate and ethanol

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作者：Dengfeng Wang^a ; Xuelan Zhang^a ; ^b ; ^{mhszxl@sxicc.ac.cn" class="auth_mail" title="E-mail the corresponding author} ; Chunli Liu^a ; TingTing Cheng^a ; Wei Wei^b ; Yuhan Sun^b
关键词：Diethyl carbonate ; Ethyl carbamate ; Ethanol ; Hydrotalcite ; Transition metal ; Mixed oxide
刊名：Applied Catalysis A: General
出版年：2015
出版时间：25 September 2015
年：2015
卷：505
期：Complete
页码：478-486
全文大小：3303 K

文摘

•: Tunable basicity of calcined hydrotalcites with mesoporous structure obtained by modifying with transition metal cations.
•: Effective synthesis of diethyl carbonate achieved over Mn²⁺ modified calcined hydrotalcites.
•: Good correlation between catalytic activity and both moderate and strong basicity.
•: Mn²⁺ modified calcined hydrotalcites presented high catalytic stability.

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