Deep oxidative desulfurization of dibenzothiophene using a flower-like WO<sub>3</sub>·H<sub>2</sub>O catalyst in an organic biphasic system

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Deep oxidative desulfurization of dibenzothiophene using a flower-like WO₃·H₂O catalyst in an organic biphasic system

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作者：Xin Xiao ; ^{xiaox@scnu.edu.cn" class="auth_mail" title="E-mail the corresponding author} ; Huan Zhong ; Chunxia Zheng ; Mingli Lu ; Xiaoxi Zuo ; Junmin Nan ; ^{jmnan@scnu.edu.cn" class="auth_mail" title="E-mail the corresponding author}
关键词：Desulfurization ; WO3· ; H2O ; Dibenzothiophene ; Organic biphasic system ; Catalytic oxidation mechanism
刊名：Chemical Engineering Journal
出版年：2016
出版时间：15 November 2016
年：2016
卷：304
期：Complete
页码：908-916
全文大小：2722 K

文摘

•: Flower-like WO₃·H₂O was conveniently synthesized by a low-temperature oil bath route.
•: The as-prepared WO₃·H₂O has excellent catalytic oxidative desulfurization activity for DBT.
•: The as-prepared catalyst is stable during the reaction and retain its high activity after recycled.
•: A simultaneous adsorption-oxidation-extraction mechanism was proposed based on experiments and DFT calculations.

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