Plasmonic Perovskite Light-Emitting Diodes Based on the Ag–CsPbBr3 System

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• 作者：Xiaoli ZhangBing Xu ; Weigao Wang ; Sheng Liu ; Yuanjin Zheng ; Shuming Chen ; Kai Wang ; Xiao Wei Sun
• 刊名：ACS Applied Materials & Interfaces
• 出版年：2017
• 出版时间：February 8, 2017
• 年：2017
• 卷：9
• 期：5
• 页码：4926-4931
• 全文大小：386K
• ISSN：1944-8252

文摘

The enhanced luminescence through semiconductor–metal interactions suggests the great potential of device performance improvement via properly tailored plasmonic nanostructures. Surface plasmon enhanced electroluminescence in an all-inorganic CsPbBr₃ perovskite light-emitting diode (LED) is fabricated by decorating the hole transport layer with the synthesized Ag nanorods. An increase of 42% and 43.3% in the luminance and efficiency is demonstrated for devices incorporated with Ag nanorods. The device with Ag introduction indicates identical optoelectronic properties to the controlled device without Ag nanostructures. The increased spontaneous emission rate caused by the Ag-induced plasmonic near-field effect is responsible for the performance enhancement. Therefore, the plasmonic Ag–CsPbBr₃ nanostructure studied here provides a novel strategy on the road to the future development of perovskite LEDs.