Substituent groups from aromatic dicarboxylates modulated structural diversification in the assembly of Co(II) complexes based on the bis-pyridyl-bis-amide ligands

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• 作者：XiuLi Wang (14784)
  Bao Mu (14784)
  HongYan Lin (14784)
  Song Yang (14784)
  GuoCheng Liu (14784)
  AiXiang Tian (14784)
  JuWen Zhang (14784)
  
• 关键词：coordination polymer ; bis ; pyridyl ; bis ; amide ligand ; hydrothermal reaction ; fluorescent property
• 刊名：SCIENCE CHINA Chemistry
• 出版年：2013
• 出版时间：May 2013
• 年：2013
• 卷：56
• 期：5
• 页码：557-566
• 全文大小：1542KB
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• 作者单位：XiuLi Wang (14784)
  Bao Mu (14784)
  HongYan Lin (14784)
  Song Yang (14784)
  GuoCheng Liu (14784)
  AiXiang Tian (14784)
  JuWen Zhang (14784)
  
  14784. Department of Chemistry, Bohai University, Jinzhou, 121000, China
  
• ISSN：1869-1870

文摘

Four coordination polymers based on two bis-pyridyl-bis-amide ligands and three aromatic dicarboxylates with different substituent groups, namely, [Co(3-bpcb)1.5(NPH)(H2O)]·4H2O (1), [Co(3-bpcb)(NIPH)] (2), [Co(3-bpcb)0.5(5-H2AIP)]·2H2O (3), [Co(3-bpcd)0.5(5-H2AIP)(H2O)]·2H2O (4) [3-bpcb = N,N-bis(3-pyridinecarboxamide)-1,4-benzene, 3-bpcd = N,N-bis(3 pyridine)cyclohexane-1,4-dicarboxamide, H2NPH = 3-nitrophthalic acid, H2NIPH = 5-nitroisophthalic acid, 5-H4AIP = 5-aminoisophthalic acid] have been synthetized under hydrothermal conditions. Complex 1 displays a one dimensional (1D) chain based on the binuclear [Co2(NPH)2] units and 3-bpcb ligands, which is extended into a three dimensional (3D) supramolecular framework through hydrogen bonding and π-π stacking interactions. In complex 2, the (3,5)-connected two dimensional (2D) layers are constructed from 1D Co-NIPH chains and bidentate-bridging 3-bpcb ligands. Complex 3 is a 2D double layer based on Co-5-H2AIP 2D layers and 3-bpcb pillars. Complex 4 also displays a 2D network, which is constructed from the Co-5-H2AIP 1D double chains and 3-bpcd ligands. Finally, complexes 2-4 are extended into 3D supramolecular frameworks by hydrogen bonding or π-π stacking interactions. The substituent groups of dicarboxylates play an important role in the assembly and structures of the title complexes. In addition, the fluorescent properties of complexes 1-strong class="a-plus-plus">4 and the electrochemical behaviors of 3 and 4 at room temperature have been investigated.