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Spectral studies to increase the efficiency and stability of laser dyes by charge-transfer reactions for using in solar cells: charge-transfer complexes of Ponceau S with p-chloranil, chloranilic and picric acids
- 作者:M. S. Al-Amoudi ; Mahmoud Salman ; M. M. Al-Majthoub…
- 关键词:Ponceau S ; π ; acceptors ; Charge ; transfer ; Thermal analysis ; Fluorescence spectra
- 刊名:Research on Chemical Intermediates
- 出版年:2015
- 出版时间:May 2015
- 年:2015
- 卷:41
- 期:5
- 页码:3089-3108
- 全文大小:755 KB
- 参考文献:1. Refat, MS, Grabchev, I, Chovelon, J-M, Ivanova, G (2006) Spectrochim. Acta A64: pp. 345
2. Refat, MS, Teleb, SM, Grabchev, I (2005) Spectrochim. Acta A61: pp. 205 ss="external" href="http://dx.doi.org/10.1016/j.saa.2004.04.017" target="_blank" title="It opens in new window">CrossRef 3. Refat, MS, El-Didamony, AM, Grabchev, I (2006) Spectrochim. Acta A 67: pp. 58-65 ss="external" href="http://dx.doi.org/10.1016/j.saa.2006.06.035" target="_blank" title="It opens in new window">CrossRef 4. Refat, MS, Aqeel, SM, Grabchev, I (2004) Can. J. Anal. Sci. Spectr. 49: pp. 258 5. Z. Rappoport, J. Chem. Soc., (1963) 4498 6. Z. Rappoport, A. Horowitz, J. Chem. Soc., (1964) 1348 7. Pilho, VC, Campos, F, Correa, R, Yunes, R, Nunes, R (2003) Quim. Nova 26: pp. 230 ss="external" href="http://dx.doi.org/10.1590/S0100-40422003000200016" target="_blank" title="It opens in new window">CrossRef 8. Angadi, M, Gosztola, D, Wasielievski, M (1998) J. Appl. Phys. 118: pp. 6187 ss="external" href="http://dx.doi.org/10.1063/1.367491" target="_blank" title="It opens in new window">CrossRef 9. Lee, S, Zu, Y, Hermann, A, Geerts, Y, Mullen, K, Bard, A (1999) J. Am. Chem. Soc. 121: pp. 3513 ss="external" href="http://dx.doi.org/10.1021/ja984188m" target="_blank" title="It opens in new window">CrossRef 10. Andric, G, Boas, J, Bond, A, Fallon, G, Ghiggino, K, Hogan, C, Hutchison, J, Lee, M, Langford, S, Pilbrow, J, Troup, G, Woodwar, C (2004) Aust. J. Chem. 57: pp. 1011 ss="external" href="http://dx.doi.org/10.1071/CH04130" target="_blank" title="It opens in new window">CrossRef 11. Gosztola, D, Niemezyk, P, Svek, W, Lukas, A, Wasielievski, M (2004) J. Phys. Chem. A 104: pp. 6545 ss="external" href="http://dx.doi.org/10.1021/jp000706f" target="_blank" title="It opens in new window">CrossRef 12. Takenaka, S, Yamashita, K, Takagi, M, Uno, Y, Kondo, H (2000) Anal. Chem. 72: pp. 1334 ss="external" href="http://dx.doi.org/10.1021/ac991031j" target="_blank" title="It opens in new window">CrossRef 13. Yamashita, K, Takagi, M, Kondo, H, Takenaka, S (2002) Anal. Biochem. 306: pp. 188 ss="external" href="http://dx.doi.org/10.1006/abio.2002.5822" target="_blank" title="It opens in new window">CrossRef 14. Barros, T, Brochsztain, S, Troskano, V, Filho, PB, Politi, MJ (1997) J. Photochem. Photobiol. 111: pp. 97 ss="external" href="http://dx.doi.org/10.1016/S1010-6030(97)00205-0" target="_blank" title="It opens in new window">CrossRef 15. Wiederrecht, G, Wasielievski, M (1998) J. Am. Chem. Soc. 120: pp. 3231 ss="external" href="http://dx.doi.org/10.1021/ja974033z" target="_blank" title="It opens in new window">CrossRef 16. Alp, S, Erten, S, Karapirem, C, Koz, B, Doroshenko, A, Icli, S (2000) J. Photochem. Photobiol. A. Chem. 135: pp. 103 ss="external" href="http://dx.doi.org/10.1016/S1010-6030(00)00306-3" target="_blank" title="It opens in new window">CrossRef 17. Usun, D, Ozser, M, Yunes, K, Icil, H, Demuth, M (2003) J. Photochem. Photobiol. A. Chem. 156: pp. 45 ss="external" href="http://dx.doi.org/10.1016/S1010-6030(02)00436-7" target="_blank" title="It opens in new window">CrossRef 18. Skoog, DA (1985) Principle of Instrumental Analysis. Saunders, New York 19. Benesi, HA, Hildebrand, JH (1949) J. Am. Chem. Soc. 71: pp. 2703-2704 ss="external" href="http://dx.doi.org/10.1021/ja01176a030" target="_blank" title="It opens in new window">CrossRef 20. Abu-Eittah, R, Al-Sugeir, F (1976) Can. J. Chem. 54: pp. 3705-3712 ss="external" href="http://dx.doi.org/10.1139/v76-532" target="_blank" title="It opens in new window">CrossRef 21. Leve, ABP (1985) Inorganic Electronic Spectroscopy. Elsevier, Amsterdam 22. Tsubomura, H, Lang, RP (1961) J. Am. Chem. Soc. 83: pp. 2085-2092 ss="external" href="http://dx.doi.org/10.1021/ja01470a013" target="_blank" title="It opens in new window">CrossRef 23. Rathone, R, Lindeman, SV, Kochi, JK (1997) J. Am. Chem. Soc. 119: pp. 9393 ss="external" href="http://dx.doi.org/10.1021/ja9720319" target="_blank" title="It opens in new window">CrossRef 24. Aloisi, G, Pignataro, S (1972) J. Chem. Soc., Faraday. Trans. 69: pp. 534 ss="external" href="http://dx.doi.org/10.1039/f19736900534" target="_blank" title="It opens in new window">CrossRef 25. Briegleb, G (1960) Z. Angew. Chem. 72: pp. 401 ss="external" href="http://dx.doi.org/10.1002/ange.19600721203" target="_blank" title="It opens in new window">CrossRef 26. Briegleb, G, Angew, Z (1964) Chem. 76: pp. 326-341 27. Martin, AN, Swarbrick, J, Cammarata, A (1969) Physical Pharmacy. Lee and Febiger, Philadelphia 28. Mostafa, SI (1999) Trans. Met. Chem. 24: pp. 306 ss="external" href="http://dx.doi.org/10.1023/A:1006944124791" target="_blank" title="It opens in new - 刊物类别:Chemistry and Materials Science
- 刊物主题:Chemistry
Catalysis Physical Chemistry Inorganic Chemistry
- 出版者:Springer Netherlands
- ISSN:1568-5675
文摘
Charge-transfer complexes formed from the reaction of Ponceau S dye with some π-acceptors such as tetrachloro-p-benzoquinone (p-chloranil; p-Chl), 2,5-dichloro-3,6-dihydroxybenzoquinone (chloranilic acid; CLA) and 2,4,6-trinitrophenol (picric acid; PA) have been studied in methanol at 25?°C. The final reaction products have been isolated and characterized using UV–Vis, mid-infrared, Raman laser, fluorescence spectra, and thermal stability measurements (TG/DTG), as well as elemental analysis of carbon, hydrogen, and nitrogen elements. The photometric titration curves for the reactions indicated that the data obtained refer to 1:2 Ponceau S charge-transfer complexes [(Pon)(p-Chl)2sub>], [(Pon)(CLA)2sub>], and [(Pon)(PA)2sub>] being formed. The infrared and Raman laser spectra interpreted the mode of charge-transfer interactions associated with the hydrogen bonding existing between two protons (–OH) of the S(=O)2sub>–OH group: a sulfonyl hydroxide Ponceau S donor and the acidic central position of acceptors for –C=O and –OH in the p-Chl and both CLA and PA, respectively. The activation parameters ΔE, ΔH, ΔS and ΔG were obtained from the DTG diagrams by using the Coats–Redfern method. The fluorescence efficiency data of free Ponceau S dye and the [(Pon)(acceptor)2sub>] charge-transfer complexes have been checked and are discussed.
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